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We report comparative experimental and theoretical studies of second and third harmonic generation from a 20nm-thick indium tin oxide layer in proximity of the epsilon-near-zero condition. Using a tunable OPA laser we record both spectral…

High quality factor optical nanostructures provide great opportunity to enhance nonlinear optical processes such as third harmonic generation. However, the field enhancement in these high quality factor structures is typically accompanied…

Optics · Physics 2023-11-22 Claudio U. Hail , Lior Michaeli , Harry A. Atwater

Third-harmonic generation can be realized via both $\chi^{(3)}$ and cascaded $\chi^{(2)}$ nonlinear processes in a triply-resonant microcavity. It is still unknown how these processes interfere with each other and the optimization of the…

Optics · Physics 2018-11-14 Ming Li , Chang-Ling Zou , Chun-Hua Dong , Dao-Xin Dai

We study second and third harmonic generation in centrosymmetric semiconductors at visible and UV wavelengths in bulk and cavity environments. Second harmonic generation is due to a combination of symmetry breaking, the magnetic portion of…

Aluminum nitride and silicon nitride have recently emerged as important nonlinear optical materials in integrated photonics respectively for their quadratic and cubic optical nonlinearity. A composite aluminum nitride and silicon nitride…

Optics · Physics 2017-12-04 Joshua B. Surya , Xiang Guo , Chang-Ling Zou , Hong X. Tang

We propose a new concept to generate efficient one-third harmonic light from an unseeded third harmonic process in optical fibers. Our concept is based on the dynamic constant (Hamiltonian) of the nonlinear third harmonic generation in…

Whispering-gallery-mode microcavities are known to have high optical quality factor, making them suitable for nonlinear optical interactions. Here, third-harmonic generation is observed using a relatively small radius wedge silicon oxide…

Efficient third-order nonlinearities of the Zinc Oxide and Al-doped Zinc Oxide were studied by Third Harmonic Generation (Third Harmonic Generation) Maker fringes to establish the effect Aluminum of Aluminum doping(Al-doping) on the cubic…

Materials Science · Physics 2023-05-01 Calford Otieno

Black phosphorus has been the subject of growing interest due to its unique band structure that is both layer dependent and anisotropic. While many have studied the linear optical response of black phosphorus, the nonlinear response has…

Materials Science · Physics 2016-11-16 Nathan Youngblood , Ruoming Peng , Andrei Nemilentsau , Tony Low , Mo Li

Nonlinear optical phenomena are at the heart of various technological domains such as high-speed data transfer, optical logic applications, and emerging fields such as non-reciprocal optics and photonic time crystal design. However,…

Improving the conversion efficiency is critical for advancing nonlinear photonic devices, enabling applications in ultrafast optics, quantum light sources, and high-resolution imaging. Herein, we present a bilayer waveguide integrated with…

Optics · Physics 2025-08-21 Xin Huang , Qi Lin , Sheng-Xuan Xia , Xiang Zhai , Gui-Dong Liu

Organic cavity polaritons are bosonic quasi-particles that arise from the strong interaction between organic molecular excitons and photons within microcavities. The spectral dispersion of third harmonic generation near resonance with the…

Optics · Physics 2018-10-08 Bin Liu , Michael Crescimanno , Robert J. Twieg , Kenneth D. Singer

Notwithstanding its long history, the study of nonlinear optics from metal surfaces is still an active field of research. For instance, in view of the presence of absorption questions remain concerning the possibility of significantly…

Nonlinear metasurfaces have become prominent tools for controlling and engineering light at the nanoscale. Usually, the polarization of the total generated third harmonic is studied. However, diffraction orders may present different…

We present a comprehensive tensorial characterization of second-harmonic generation from silicon nitride films with varying composition. The samples were fabricated using plasma-enhanced chemical vapor deposition, and the material…

Optical materials with centrosymmetry, such as silicon and germanium, are unfortunately absent of second-order nonlinear optical responses, hindering their developments in efficient nonlinear optical devices. Here, a design with an array of…

Optics · Physics 2022-06-17 C. Fang , Q. Yang , Q. Yuan , L. Gu , X. Gan , Y. Shao , Y. Liu , G. Han , Y. Hao

Harmonic generation in underdense spatially homogeneous plasma is generally expected to be inefficient: in an unmagnetized uniform plasma the fundamental and its harmonics cannot be phase-matched, resulting in third-harmonic generation…

Plasma Physics · Physics 2026-01-21 S. Cao , M. R. Edwards

Optical properties of periodic arrays of nanoholes of a triangular shape with experimentally realizable parameters are examined in both linear and nonlinear regimes. Utilizing fully vectorial three-dimensional approach based on the…

Mesoscale and Nanoscale Physics · Physics 2020-03-18 Elena Drobnyh , Maxim Sukharev

Understanding how light interacts at the nanoscale with metals, semiconductors, or ordinary dielectrics is pivotal if one is to properly engineer nano-antennas, filters and, more generally, devices that aim to harness the effects of new…

Classical nonlocality in conducting nanostructures has been shown to dramatically alter the linear optical response, by placing a fundamental limit on the maximum field enhancement that can be achieved. This limit directly extends to all…

Mesoscale and Nanoscale Physics · Physics 2013-11-14 Cristian Ciracì , Michael Scalora , David R. Smith
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