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To examine the insulating mechanism of 5$d$ transition metal oxide Sr$_2$IrO$_4$, we study the ground state properties of a three-orbital Hubbard model with a large relativistic spin-orbit coupling on a square lattice. Using a variational…

Strongly Correlated Electrons · Physics 2014-09-22 Hiroshi Watanabe , Tomonori Shirakawa , Seiji Yunoki

A series of polycrystalline samples of Sr2-xIrO4 have been synthesized by a solid-state reaction method. The crystal structure of this doped system can be explained on the basis of the extended nature of 5d electrons and strontium vacancies…

Strongly Correlated Electrons · Physics 2016-11-09 Jimei Kong , S. L. Liu , Jie Cheng , Haiyun Wang , Xing ao Li , Z. H. Wang

The temperature-dependent behavior of magnetic domains plays an essential role in the magnetic properties of materials, leading to widespread applications. However, experimental methods to access the three-dimensional (3D) magnetic domain…

We report a high frequency/high magnetic field electron spin resonance (HF-ESR) spectroscopy study in the sub-THz frequency domain of the two representatives of the family of magnetic topological insulators…

Strongly Correlated Electrons · Physics 2022-02-03 A. Alfonsov , K. Mehlawat , A. Zeugner , A. Isaeva , B. Büchner , V. Kataev

Metamagnetism in antiferromagnets exhibits distinct critical behaviors and dynamics when invoking spin reversal and rotation. Here we show a 0.05% anisotropic strain suffices to in-situ modulate the metamagnetic critical field of the Mott…

Strongly Correlated Electrons · Physics 2020-07-24 H. Zhang , L. Hao , J. Yang , J. Mutch , Z. Liu , Q. Huang , K. Noordhoek , A. F. May , J. -H. Chu , J. W. Kim , P. J. Ryan , H. D. Zhou , Jian Liu

A spin-orbital superexchange Hamiltonian in a Mott insulator with $t_{2g}$ orbital degeneracy is investigated. More specifically, we focus on a spin ferromagnetic state of the model and study a collective behavior of orbital angular…

Strongly Correlated Electrons · Physics 2009-11-11 G. Khaliullin , S. Okamoto

Electrical control of structural and physical properties is a long-sought, but elusive goal of contemporary science and technology. We demonstrate that a combination of strong spin-orbit interactions (SOI) and a canted antiferromagnetic…

Strongly Correlated Electrons · Physics 2018-01-08 G. Cao , J. Terzic , H. D. Zhao , H. Zheng , L. E. De Long , Peter S. Riseborough

Sr2IrO4 exhibits a novel insulating state assisted by spin-orbit interactions. A series of polycrystalline samples of Sr2-xIrO4 have been synthesized. It is found that deep Sr-vacancies of Sr2-xIrO4 greatly reduce the rotation of IrO6…

Strongly Correlated Electrons · Physics 2016-11-01 Xuanyong Sun , S. L. Liu , Haiyun Wang , Bin Li , Jie Cheng , Z. H. Wang

The electronic and magnetic properties of monoclinic double perovskite Sr$_2$CeIrO$_6$ were examined based on both experiments and first-principles density functional theory calculations. From the calculations we conclude that…

Materials Science · Physics 2016-07-13 Sudipta Kanungo , Kailash Mogare , Binghai Yan , Claudia Felser , Martin Jansen

We report point-contact measurements of anisotropic magnetoresistance (AMR) in a single crystal of antiferromagnetic (AFM) Mott insulator Sr2IrO4. The point-contact technique is used here as a local probe of magnetotransport properties on…

Mesoscale and Nanoscale Physics · Physics 2014-12-03 Cheng Wang , Heidi Seinige , Gang Cao , Jian-Shi Zhou , John B. Goodenough , Maxim Tsoi

We have used Raman scattering to investigate the magnetic excitations and lattice dynamics in the prototypical spin-orbit Mott insulators Sr2IrO4 and Sr3Ir2O7. Both compounds exhibit pronounced two-magnon Raman scattering features with…

Strongly Correlated Electrons · Physics 2016-04-06 H. Gretarsson , N. H. Sung , M. Hoeppner , B. J. Kim , B. Keimer , M. Le Tacon

The insulating iron compounds Eu$_2$SrFe$_2$O$_6$ and Sr$_3$Fe$_2$O$_4$Cl$_2$ have high-temperature antiferromagnetic (AF) order despite their different layered structures. Here we carry out density functional calculations and Monte Carlo…

Strongly Correlated Electrons · Physics 2022-08-18 Di Lu , Ke Yang , Lu Liu , Guangyu Wang , Hua Wu

CoO has an odd number of electrons in its unit cell, and therefore is expected to be metallic. Yet, CoO is strongly insulating owing to significant electronic correlations, thus classifying it as a Mott insulator. We investigate the…

Time-of-flight inelastic neutron scattering measurements on Sr2IrO4 single crystals were performed to access the spin Hamiltonian in this canonical Jeff=1/2 spin-orbital Mott insulator. The momentum of magnetic scattering at all inelastic…

Strongly Correlated Electrons · Physics 2018-12-12 S. Calder , D. M. Pajerowski , M. B. Stone , A. F. May

Applying the correlated electronic structure method based on density functional theory plus the Hubbard $U$ interaction, we have investigated the tetragonal scheelite structure Mott insulator KOsO$_4$, whose $e_g^1$ configuration should be…

Strongly Correlated Electrons · Physics 2014-12-10 Young-Joon Song , Kyo-Hoon Ahn , K. -W. Lee , W. E. Pickett

In this work, we present a comprehensive study of the low energy optical magnetic response of the skyrmionic Mott insulator Cu$_2$OSeO$_3$ via high resolution time-domain THz spectroscopy. In zero field, a new magnetic excitation not…

Strongly Correlated Electrons · Physics 2017-07-03 N. J. Laurita , G. G. Marcus , B. A. Trump , J. Kindervater , M. B. Stone , T. M. McQueen , C. L. Broholm , N. P. Armitage

Antiferromagnetic (AFM) spintronics, where magneto-transport is governed by an antiferromagnet instead of a ferromagnet, opens fascinating new perspectives for both fundamental research and device technology, owing to their intrinsic…

Materials Science · Physics 2021-10-26 Haowen Wang , Wei Wang , Ni Hu , Tianci Duan , Songliu Yuan , Shuai Dong , Chengliang Lu , Jun-Ming Liu

The low-frequency dynamical response of an Anderson insulator is dominated by so-called Mott resonances: hybridization of pairs of states close in energy, but separated spatially. We study the effect of interaction on Mott resonances in the…

Mesoscale and Nanoscale Physics · Physics 2017-02-02 D. A. Ivanov , M. V. Feigel'man

The effect of isoelectronic substitution within single crystals of (Sr1-xCax)2-yIrO4+z is explored. The nominal n=1 Ruddlesden-Popper phase with y=0, z=0 remains stable from x=0 until x=0.11, where the antiferromagnet spin-orbit Mott…

Materials Science · Physics 2016-11-23 Xiang Chen , Stephen D. Wilson

We present a multi-frequency Electron Spin Resonance (ESR) study in the range of 4 GHz to 420 GHz of the quasi-one-dimensional, non-dimerized, quarter-filled Mott insulators, delta-(EDT-TTF-CONMe_2)_2X (X=AsF_6, Br). In the high temperature…

Strongly Correlated Electrons · Physics 2010-07-15 Bálint Náfrádi , Areta Olariu , László Forró , Cécile Mézière , Patrick Batail , András Jánossy