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Electron microscopy techniques such as electron energy-loss spectroscopy (EELS) facilitate the spatio-spectral characterization of plasmonic nanostructures. In this work, a time-dependent perspective is presented, which significantly…

Historically, the field of plasmonics has been relying on the framework of classical electrodynamics, with the local-response approximation of material response being applied even when dealing with nanoscale metallic structures. However,…

Electron energy loss spectroscopy (EELS) can be used to probe plasmon excitations in nanostructured materials with atomic-scale spatial resolution. For structures smaller than a few nanometers quantum effects are expected to be important,…

Mesoscale and Nanoscale Physics · Physics 2013-01-03 Kirsten Andersen , Karsten W. Jacobsen , Kristian S. Thygesen

Understanding light-matter interactions using localized surface plasmons (LSPs) is of fundamental interest in classical and quantum plasmonics and has a wide range of applications. In order to understand the spatial properties of LSPs,…

Mesoscale and Nanoscale Physics · Physics 2016-03-22 Rong-Chun Ge , Stephen Hughes

Recently, two reports have demonstrated the amazing possibility to probe vibrational excitations from nanoparticles with a spatial resolution much smaller than the corresponding free-space phonon wavelength using electron energy loss…

Materials Science · Physics 2017-12-13 Hugo Lourenço-Martins , Mathieu Kociak

Excitation of localized surface plasmons (LSPs) of metal nanoparticles (NPs) residing on a flat metal film has attracted great attentions recently due to the enhanced electromagnetic (EM) fields found to be higher than the case of NPs on a…

Optics · Physics 2015-07-02 Anran Li , Sivan Isaacs , Ibrahim Abdulhalim , Shuzhou Li

Electron energy loss spectroscopy (EELS) is often utilized to characterize localized surface plasmon modes supported by plasmonic antennas. However, the spectral resolution of this technique is only mediocre, and it can be rather difficult…

The optical properties of metallic nanoparticles are dominated by localized surface plasmons (LSPs). Their properties only depend on the constituting material, the size and shape of the nano-object as well as its surrounding medium. In…

We demonstrate spatially-resolved measurements of spontaneous and stimulated electron-photon interactions in nanoscale optical near fields using electron energy-loss spectroscopy (EELS), cathodoluminescence spectroscopy (CL), and…

The role of metallic nanostructures in nanophotonics is expected to expand if ways to electrically manipulate their optical resonances at high speed can be identified. Here, we capitalize on electrically-driven surface acoustic waves and…

We investigate surface plasmons from a solid-state standpoint and highlight their ultra electron density sensitivity. When a surface plasmon is excited on a planar gold film by an evanescent wave from 625 nm incident light, only a minute…

Optics · Physics 2023-07-12 Wei Liu , Meng Li , Yu Niu , Ziren Luo

We theoretically investigated electron energy loss spectroscopy (EELS) of ultraviolet surface plasmon modes in aluminum nanodisks. Using full-wave simulations, we studied the impact of diameter on the resonant modes of the nanodisks. We…

In electron energy-loss spectroscopy (EELS) of individual silver nanoparticles encapsulated in silicon nitride, we observe besides the usual dipole resonance an additional surface plasmon (SP) resonance corresponding to higher angular…

Electron energy loss spectroscopy (EELS) has been established as a powerful analytical technique for investigating the oxidation state, band structure, and dielectric properties of materials with exceptional spatial resolution. Inspired by…

Among the many potential applications of topological insulator materials, their broad potential for the development of novel tunable plasmonics at THz and mid-infrared frequencies for quantum computing, terahertz detectors, and spintronic…

Mesoscale and Nanoscale Physics · Physics 2023-05-09 Helena La , Abel Brokkelkamp , Stijn van der Lippe , Jaco ter Hoeve , Juan Rojo , Sonia Conesa-Boj

We study strongly confined plasmons in ultrathin gold and silver films by simulating electron energy-loss spectroscopy (EELS). Plasmon dispersion relations are directly retrieved from the energy- and momentum-resolved loss probability under…

Mesoscale and Nanoscale Physics · Physics 2020-05-06 A. Rodríguez Echarri , Enok Johannes Haahr Skjølstrup , Thomas G. Pedersen , F. Javier García de Abajo

Electron energy-loss spectroscopy (EELS) offers a window to view nanoscale properties and processes. When performed in a scanning transmission electron microscope, EELS can simultaneously render images of nanoscale objects with…

Mesoscale and Nanoscale Physics · Physics 2016-09-26 Charles Cherqui , Niket Thakkar , Guoliang Li , Jon P. Camden , David Masiello

One fundamental motivation to know the dispersive, or frequency dependent characteristics of localized surface plasmons (LSPs) supported by elliptical shaped particles wrapped with graphene sheet, as well as their scattering characteristics…

Optics · Physics 2021-11-24 Mauro Cuevas , Ricardo A. Depine

Acoustic-graphene-plasmons (AGPs) are highly confined electromagnetic modes, carrying large momentum and low loss in the mid-infrared/Terahertz spectra. Owing to their ability to confine light to extremely small dimensions, they bear great…

Plasmonics, the science and technology of the interaction of light with metallic objects, is fundamentally changing the way we can detect, generate and manipulate light. Although the field is progressing swiftly, thanks to the availability…

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