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We used a local susceptibility approach in extensive polarized neutron diffraction studies of the spin liquid \tbti. For a magnetic field applied along the [110] and [111] directions, we found that, at high temperature, all Tb moments are…

Strongly Correlated Electrons · Physics 2015-05-13 Arsen Gukasov , Huibo Cao , Isabelle Mirebeau , Pierre Bonville

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

High resolution X-ray powder-diffraction experiments on a well-characterized polycrystalline sample of the spin liquid Tb2Ti2O7 reveal that it shows normal positive thermal-expansion above 4 K, which does not agree with the intriguing…

Strongly Correlated Electrons · Physics 2011-12-14 Kazuki Goto , Hiroshi Takatsu , Tomohiro Taniguchi , Hiroaki Kadowaki

We investigated the possibility of temperature dependent lattice distortions in the pyrochlore compound Tb$_{2}$Ti$_{2}$O$_{7}$ by measuring the internal magnetic field distribution, using muon spin resonance, and comparing it to the…

Strongly Correlated Electrons · Physics 2015-06-25 Oren Ofer , Amit Keren , Chris Baines , Jason S. Gardner

The antiferromagnetic pyrochlore material NaCaCo$_2$F$_7$ is a thermal spin liquid over a broad temperature range (~ 140 K down to $T_F = 2.4 $K), in which magnetic correlations between Co$^{2+}$ dipole moments explore a continuous manifold…

Strongly Correlated Electrons · Physics 2017-04-26 K. A. Ross , J. M. Brown , R. J. Cava , J. W. Krizan , S. E. Nagler , J. A. Rodriguez-Rivera , M. B. Stone

The frustrated pyrochlore antiferromagnet Gd$_{2}$Ti$_{2}$O$_{7}$ has an unusual partially-ordered magnetic structure at the lowest measurable temperatures. This structure is currently believed to involve four magnetic propagation vectors…

Neutron scattering experiments on frustrated fcc - antiferromagnet HoB$_{12}$ have been performed above T$_{N}$ = 7.4 K. Diffuse scattering patterns indicate that above Neel temperature correlations between neighboring magnetic moments of…

Strongly Correlated Electrons · Physics 2007-05-23 K. Siemensmeyer , K. Flachbart , S. Gabani , S. Matas , Y. Paderno , N. Shitsevalova

We present time-of-fight neutron-scattering measurements on single crystals of $La_{2-x}Ba_{x}CuO_{4}$ (LBCO) with 0 $\leq$ x $\leq$ 0.095 and $La_{2-x}Sr_{x}CuO_{4}$ (LSCO) with x = 0.08 and 0.11. This range of dopings spans much of the…

We interpret recent measurements of the zero field muon relaxation rate in the frustrated magnetic pyrochlore Dy$_2$Ti$_2$O$_7$ as resulting from the quantum diffusion of muons in the substance. In this scenario, the plateau observed at low…

Strongly Correlated Electrons · Physics 2015-06-04 P. Quémerais , P. McClarty , R. Moessner

The insulating magnetic pyrochlore Ce$_2$Zr$_2$O$_7$ has gained attention as a quantum spin ice candidate with dipole-octupole character arising from the crystal electric field ground state doublet for the Ce$^{3+}$ ion. This permits both…

Strongly Correlated Electrons · Physics 2025-05-01 E. M. Smith , R. Schäfer , J. Dudemaine , B. Placke , B. Yuan , Z. Morgan , F. Ye , R. Moessner , O. Benton , A. D. Bianchi , B. D. Gaulin

The spin-liquid phase of two highly frustrated pyrochlore magnets Gd2Ti2O7 and Gd2Sn2O7 is probed using electron spin resonance in the temperature range 1.3 - 30 K. The deviation of the absorption line from the paramagnetic position \nu…

Strongly Correlated Electrons · Physics 2013-05-29 S. S. Sosin , L. A. Prozorova , A. I. Smirnov , P. Bonville , G. Jasmin - Le Bras , O. A. Petrenko

In this paper, we illustrate how polarized neutron scattering can be used to isolate the spin-spin correlations of modes forming flat bands in a frustrated magnetic system hosting a classical spin liquid phase. In particular, we explain why…

We have investigated polycrystalline samples of the zigzag chain system BaTb$_2$O$_4$ with a combination of magnetic susceptibility, heat capacity, neutron powder diffraction, and muon spin relaxation measurements. Despite the onset of…

Strongly Correlated Electrons · Physics 2015-10-27 A. A. Aczel , L. Li , V. O. Garlea , J. -Q. Yan , F. Weickert , V. S. Vapf , R. Movshovich , M. Jaime , P. J. Baker , V. Keppens , D. Mandrus

We investigate low-temperature spin correlations in the metallic frustrated magnet \beta-MnCo. Single-crystal polarised-neutron scattering experiments reveal the persistence of highly-structured magnetic diffuse scattering and the absence…

The very low temperature properties of two pyrochlore compounds, Yb2Ti2O7 and Gd2Sn2O7, were investigated using an ensemble of microscopic and bulk techniques. In both compounds, a first order transition is evidenced, as well as spin…

We present here a neutron diffraction study, both in zero field and as a function of magnetic field, of the magnetic structure of the tetragonal intermetallic \eun\ on a single crystalline sample. This material is known to undergo a cascade…

Strongly Correlated Electrons · Physics 2016-06-29 X. Fabreges , A. Gukasov , P. Bonville , A. Maurya , A. Thamizhavel , S. K. Dhar

We have studied the neutron diffuse scattering in the relaxor PMN. The diffuse scattering appears around the Burns temperature (~620K), indicating its origin from the polar nanoregions (PNR). While the relative diffuse intensities are…

Materials Science · Physics 2009-11-07 K. Hirota , Z. -G. Ye , S. Wakimoto , P. M. Gehring , G. Shirane

The Ising triangular lattice remains the classic test-case for frustrated magnetism. Here we report neutron scattering measurements of short range magnetic order in CuMnO$_2$, which consists of a distorted lattice of Mn$^{3+}$ spins with…

Strongly Correlated Electrons · Physics 2020-08-13 Simon A. J. Kimber , Andrew Wildes , Hannu Mutka , Jan-Willem G. Bos , Dimitri N. Argyriou

Neutron scattering measurements show the ferromagnetic XY pyrochlore Yb2Ti2O7 to display strong quasi-two dimensional (2D) spin correlations at low temperature, which give way to long range order (LRO) under the application of modest…

Strongly Correlated Electrons · Physics 2010-02-08 K. A. Ross , J. P. C. Ruff , C. P. Adams , J. S. Gardner , H. A. Dabkowska , Y. Qiu , J. R. D. Copley , B. D. Gaulin

The temperature evolution of the crystal and magnetic structures of ferroelectric sulfide AgCrS2 have been investigated by means of neutron scattering. AgCrS2 undergoes at TN = 41.6 K a first-order phase transition, from a paramagnetic…

Materials Science · Physics 2015-05-19 Francoise Damay , Christine Martin , Vincent Hardy , Gilles André , Sylvain Petit , Antoine Maignan