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We present high-resolution single crystal time-of-flight neutron scattering measurements on the candidate quantum spin liquid pyrochlore Tb2Ti2O7 at low temperature and in a magnetic field. At ~70 mK and in zero field, Tb2Ti2O7 reveals…

Strongly Correlated Electrons · Physics 2013-04-16 K. Fritsch , K. A. Ross , Y. Qiu , J. R. D. Copley , T. Guidi , R. I. Bewley , H. A. Dabkowska , B. D. Gaulin

Elastic and inelastic neutron scattering studies have been carried out on the pyrochlore magnet Ho2Ti2O7. Measurements in zero applied magnetic field show that the disordered spin ice ground state of Ho2Ti2O7 is characterized by a pattern…

Strongly Correlated Electrons · Physics 2016-08-05 J. P. Clancy , J. P. C. Ruff , S. R. Dunsiger , Y. Zhao , H. A. Dabkowska , J. S. Gardner , Y. Qiu , J. R. D. Copley , T. Jenkins , B. D. Gaulin

Intensity distribution of the neutron magnetic scattering has been taken in the reciprocal space of a single crystal of the "spin ice" system Ho2Ti2O7 at the elastic energy position in the temperature (T) region between 0.4 K and 50 K. The…

We present an interpretation of zero field diffuse neutron scattering and of high field magnetisation data at very low temperature in the frustrated pyrochlore system Tb2Ti2O7. This material has antiferromagnetic exchange interactions and…

Strongly Correlated Electrons · Physics 2013-12-16 P. Bonville , A. Gukasov , I. Mirebeau , S. Petit

Structural disorder in the magnetically frustrated pyrochlore system leads to intriguing magnetic states. We present the thermodynamic behavior and short range magnetic correlations in Tb$_{2}$Zr$_{2}$O$_{7}$ and…

Strongly Correlated Electrons · Physics 2026-04-16 Sujata Singh , Leon Carstens , M. Duc Le , R. Klingeler , C. S. Yadav

The pyrochlore material Yb2Ti2O7 displays unexpected quasi-two-dimensional (2D) magnetic correlations within a cubic lattice environment at low temperatures, before entering an exotic disordered ground state below T=265mK. We report neutron…

Strongly Correlated Electrons · Physics 2012-02-13 K. A. Ross , L. R. Yaraskavitch , M. Laver , J. S. Gardner , J. A. Quilliam , S. Meng , J. B. Kycia , D. K. Singh , H. A. Dabkowska , B. D. Gaulin

We report neutron scattering studies of the spin correlations of the geometrically frustrated pyrochlore Tb2Mo2O7 using single crystal samples. This material undergoes a spin-freezing transition below Tg~24 K, similar to Y2Mo2O7, and has…

Strongly Correlated Electrons · Physics 2009-11-13 D. K. Singh , J. S. Helton , S. Chu , T. H. Han , C. J. Bonnoit , S. Chang , H. J. Kang , J. W. Lynn , Y. S. Lee

We report vibrating coil magnetometry of the spin ice system Ho2Ti2O7 down to ~0.04 K for magnetic fields up to 5 T applied parallel to the [111] axis. History dependent behavior emerges below T*_0 ~ 0.6 K near zero magnetic field, in…

Strongly Correlated Electrons · Physics 2012-06-25 C. Krey , S. Legl , S. R. Dunsiger , M. Meven , J. S. Gardner , J. M. Roper , C. Pfleiderer

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

By means of neutron scattering techniques we have investigated the frustrated pyrochlore magnet Ho_2Sn_2O_7, which was found to show a ferromagnetic spin-ice behavior below T \simeq 1.4 K by susceptibility measurements. High-resolution…

Disordered Systems and Neural Networks · Physics 2007-05-23 Hiroaki Kadowaki , Yoshinobu Ishii , Kazuyuki Matsuhira , Yukio Hinatsu

Tb2Ti2O7 is a pyrochlore antiferromagnet that has dynamical spins and only short-range correlations even at 50 mK; the lowest temperature explored so far, which is much smaller than the scale set by the Curie-Weiss temperature T_{CW}~14 K.…

Statistical Mechanics · Physics 2009-12-16 Hamid R. Molavian , Paul A. McClarty , Michel J. P. Gingras

We have studied magnetically frustrated Tb$_2$Sn$_2$O$_7$ by neutron diffraction and high resolution energy-resolved neutron scattering. At 0.1 K, we observe short range magnetic correlations with a typical scale of 4 \AA, close to the near…

Strongly Correlated Electrons · Physics 2009-11-13 I. Mirebeau , H. Mutka , P. Bonville , A. Apetrei , A. Forget

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

The anisotropic spin glass transition, in which spin freezing is observed only along the c-axis in pseudobrookite Fe$_2$TiO$_5$, has long been perplexing because the Fe$^{3+}$ moments (d$^5$) are expected to be isotropic. Recently, neutron…

Disordered Systems and Neural Networks · Physics 2023-01-18 Yu Li , P. G. LaBarre , D. M. Pajerowski , A. P. Ramirez , S. Rosenkranz , D. Phelan

Neutron scattering, a.c. magnetic susceptibility and specific heat studies have been carried out on polycrystalline Dy2Zr2O7. Unlike the pyrochlore spin ice Dy2Ti2O7, Dy2Zr2O7 crystallizes into the fluorite structure and the magnetic Dy3+…

Disordered Systems and Neural Networks · Physics 2019-07-01 J. G. A. Ramon , C. W. Wang , L. Ishida , P. L. Bernardo , M. M. Leite , F. M. Vichi , J. S. Gardner , R. S. Freitas

We have studied the field-dependent ac magnetic susceptibility of single crystals of Dy2Ti2O7 spin ice along the [111] direction in the temperature range 1.8 K - 7 K. Our data reflect the onset of local spin ice order in the appearance of…

Strongly Correlated Electrons · Physics 2015-06-12 M. J. Matthews , C. Castelnovo , R. Moessner , S. A. Grigera , D. Prabhakaran , P. Schiffer

The magnetocaloric effect of polycrystalline samples of pure and Y-doped dipolar spin ice Dy2Ti2O7 was investigated at temperatures from nominally 0.3 K to 6 K and in magnetic fields of up to 2 T. As well as being of intrinsic interest, it…

Soft Condensed Matter · Physics 2015-06-25 M. Orendac , J. Hanko , E. Cizmar , A. Orendacova , M. Shirai , S. T. Bramwell

Recent elastic and inelastic neutron scattering studies of the highly frustrated pyrochlore antiferromagnet Tb2Ti2O7 have shown some very intriguing features that cannot be modeled by the local <111> classical Ising model, naively expected…

Disordered Systems and Neural Networks · Physics 2007-05-23 Ying-Jer Kao , Matthew Enjalran , Adrian Del Maestro , Hamid R. Molavian , Michel J. P. Gingras

We have probed the low temperature magnetic behavior of the ordered spin ice material Tb2Sn2O7 through ac magnetic susceptibility measurements of both the pure material and samples with small percentages of Ti substituted on the Sn…

Strongly Correlated Electrons · Physics 2012-11-27 M. L. Dahlberg , M. J. Matthews , P. Jiramongkolchai , R. J. Cava , P. Schiffer

The thermodynamic properties of the pyrochlore Yb2Ti2O7 material are calculated using the numericallinked-cluster (NLC) calculation method for an effective anisotropic-exchange spin-1/2 Hamiltonian with parameters recently determined by…

Strongly Correlated Electrons · Physics 2014-04-11 N. R. Hayre , K. A. Ross , R. Applegate , T. Lin , R. R. P. Singh B. D. Gaulin , M. J. P. Gingras
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