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Related papers: Hidden order in hexagonal RMnO3 multiferroics

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Antiferroelectrics are emerging as advanced functional materials and are fertile ground for unusual electric effects. For example, they enhance the recoverable energy density in energy storage applications and give rise to large…

An explanation is given for the charge order, orbital order and insulating state observed in half-doped manganese oxides, such as Nd$_{1/2}$Sr$_{1/2}$MnO$_{3}$. The competition between the kinetic energy of the electrons and the magnetic…

Strongly Correlated Electrons · Physics 2009-10-31 Jeroen van den Brink , Giniyat Khaliullin , Daniel Khomskii

With a combined ab initio density functional and model Hamiltonian approach we establish that in the recently discovered multiferroic phase of the manganite Sr$_{1/2}$Ba$_{1/2}$MnO$_{3}$ the polar distortion of Mn and O ions is stabilized…

Materials Science · Physics 2015-03-09 Gianluca Giovannetti , Sanjeev Kumar , Carmine Ortix , Massimo Capone , Jeroen van den Brink

We have studied the influence of antiferromagnetic ordering on the local dielectric moments of the MnO_5 and LuO_7 polyhedra by measuring neutron powder diffraction patterns of LuMnO_3 at temperatures near T_N. We show that the coupling is…

Strongly Correlated Electrons · Physics 2009-11-10 Bas B. Van Aken , Thomas T. M. Palstra

We performed magnetic and ferroelectric measurements, associated with Landau theory and symmetry analysis, in order to clarify the situation of the YMnO3 system, a classical example of type I multiferroics. We found that the only magnetic…

Strongly Correlated Electrons · Physics 2015-06-16 Kiran Singh , Marie-Bernadette Lepetit , Charles Simon , Natalia Bellido , Stephane Pailhes , Julien Varignon , Abin De Muer

We consider the orbital ordering in LaMnO3 and similar systems, proceeding from the band picture. We show that for the realistic magnetic structure of A-type there exists a complete nesting betweeen two e_g-bands. As a result there occurs…

Strongly Correlated Electrons · Physics 2009-11-10 D. V. Efremov , D. I. Khomskii

We report resonant X-ray scattering measurements on the orbitally-degenerate triangular metallic antiferromagnet 2H-AgNiO2 to probe the spontaneous transition to a triple-cell superstructure at temperatures below 365 K. We observe a strong…

Strongly Correlated Electrons · Physics 2015-05-19 G. L. Pascut , R. Coldea , P. G. Radaelli , A. Bombardi , G. Beutier , I. I. Mazin , M. D. Johannes , M. Jansen

We present a new member of the multiferroic oxides, Lu$_2$MnCoO$_6$, which we have investigated using X-ray diffraction, neutron diffraction, specific heat, magnetization, electric polarization, and dielectric constant measurements. This…

Multiferroic materials have received an astonishing attention in the last decades due to expectations that potential coupling between distinct ferroic orders could inspire new applications and new device concepts. As a result, a new…

Materials Science · Physics 2015-10-14 Josep Fontcuberta

It is argued that both transitions observed in 50%-doped manganites, at the N\'{e}el temperature ($T_{\rm N}$) and the so-called charge ordering temperature ($T_{\rm CO}$), are magnetic. $T_{\rm N}$ corresponds to the order-disorder…

Strongly Correlated Electrons · Physics 2007-05-23 I. V. Solovyev

Neutron powder diffraction and single crystal x-ray resonant magnetic scattering measurements suggest that Dy plays an active role in enhancing the ferroelectric polarization in multiferroic DyMnO3 above TNDy = 6.5 K. We observe the…

Strongly Correlated Electrons · Physics 2007-05-23 O. Prokhnenko , R. Feyerherm , E. Dudzik , S. Landsgesell , N. Aliouane , L. C. Chapon , D. N. Argyriou

An effective model is developed to explain the phase diagram and the mechanism of magnetoelectric coupling in multiferroics, $RMn_2O_5$. We show that the nature of magnetoelectric coupling in $RMn_2O_5$ is a coupling between two Ising-type…

Strongly Correlated Electrons · Physics 2009-11-13 Chen Fang , Jiangping Hu

We have found a remarkable increase (up to 60 %) of the dielectric constant with the onset of magnetic order at 42 K in the metastable orthorhombic structures of YMnO3 and HoMnO3 that proves the existence of a strong magneto-dielectric…

Strongly Correlated Electrons · Physics 2009-11-10 B. Lorenz , Y. Q. Wang , Y. Y. Sun , C. W. Chu

Magnetically hidden order is a hypernym for electronic ordering phenomena that are visible to macroscopic thermodynamic probes but whose microscopic symmetry cannot be revealed with conventional neutron or x-ray diffraction. In a handful of…

Strongly Correlated Electrons · Physics 2024-08-29 F. Mazza , P. Y. Portnichenko , S. Avdoshenko , P. Steffens , M. Boehm , Eun Sang Choi , M. Nikolo , X. Yan , A. Prokofiev , S. Paschen , D. S. Inosov

On the basis of group theory and the first-principles calculations, we investigate high-rank multipole orderings in URu2Si2, which have been proposed as a genuine primary order parameter in the hidden order phase below 17.5K. We apply…

Materials Science · Physics 2015-01-07 Michi-To Suzuki , Hiroaki Ikeda

YCrO3 which has a monoclinic structure, shows weak ferromagnetism below 140 K (TN) and a ferroelectric transition at 473 K accompanied by hysteresis. We have determined the structure and energetics of YCrO3 with ferromagnetic and…

Materials Science · Physics 2007-05-23 Claudy Rayan Serrao , Asish K. Kundu , S. B. Krupanidhi , Umesh V. Waghmare , C. N. R. Rao

The heavy fermion intermetallic compound URu2Si2 exhibits a "hidden-order" phase below the temperature of 17.5 K, which supports both anomalous metallic behavior and unconventional superconductivity. While these individual phenomena have…

By performing first-principles calculations, we systematically explore the effect of epitaxial strain on the structure and properties of multiferroic TbMnO3. We show that, although the unstrained bulk TbMnO3 displays a non-collinear…

Materials Science · Physics 2015-05-20 Yusheng Hou , Jihui Yang , Xingao Gong , Hongjung Xiang

Solids with strong electron correlations generally develop exotic phases of electron matter at low temperatures. Among such systems, the heavy-fermion semi-metal URu2Si2 presents an enigmatic transition at To = 17.5 K to a `hidden order'…

Strongly Correlated Electrons · Physics 2009-07-25 A. F. Santander-Syro , M. Klein , F. L. Boariu , A. Nuber , P. Lejay , F. Reinert

We show that the improper ferroelectric phase transition in the multiferroic hexagonal manganites displays the same symmetry-breaking characteristics as those proposed in early-universe theories. We present an analysis of the Kibble-Zurek…

Materials Science · Physics 2021-03-09 S. M. Griffin , M. Lilienblum , K. Delaney , Y. Kumagai , M. Fiebig , N. A. Spaldin