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Related papers: Hidden order in hexagonal RMnO3 multiferroics

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The improper ferroelectricity in YMnO$_3$ and other related multiferroic hexagonal manganites are known to cause topologically protected ferroelectric domains that give rise to rich and diverse physical phenomena. The local structure and…

Hexagonal manganites are multiferroic materials with two highly-dissimilar phase transitions: a ferroelectric transition (from P63/mmc to P63cm) at a temperature higher than 1000 K and an antiferromagnetic transition at TN=65 - 130 K.…

Strongly Correlated Electrons · Physics 2018-02-20 Hasung Sim , Jaehong Jeong , Haeri Kim , S-W Cheong , Je-Geun Park

The controversy regarding the ferroelectric behavior of hexagonal InMnO$_3$ is resolved by using a combination of x-ray diffraction (XRD), piezoresponse force microscopy (PFM), second harmonic generation (SHG), and density functional theory…

Materials Science · Physics 2013-05-30 Yu Kumagai , Alexei A. Belik , Martin Lilienblum , Naëmi Leo , Manfred Fiebig , Nicola A. Spaldin

Translation domains differing in the phase but not in the orientation of the corresponding order parameter are resolved in two types of multiferroics. Hexagonal (h-) YMnO$_3$ is a split-order-parameter multiferroic in which commensurate…

Strongly Correlated Electrons · Physics 2010-08-20 D. Meier , N. Leo , T. Jungk , E. Soergel , P. Becker , L. Bohaty , M. Fiebig

Magnetic order of the manganese and rare-earth lattices according to different symmetry representations is observed in multiferroic hexagonal (h-) DyMnO$_3$ by optical second harmonic generation and neutron diffraction. The incompatibility…

Strongly Correlated Electrons · Physics 2012-08-08 C. Wehrenfennig , D. Meier , Th. Lottermoser , Th. Lonkai , J. -U. Hoffmann , N. Aliouane , D. N. Argyriou , M. Fiebig

Structural features of ferroic domains are fundamentally important for the understanding of microstructure and physical properties of ferroic materials, and they are also of technological significance for information storage and electronic…

Materials Science · Physics 2012-05-22 J. Q. Li , J. Li , H. X. Yang , H. F. Tian , S-W. Cheong , C. Ma , S. Zhang , Y. G. Zhao

Trimerization-polarization domains in ferroelectric hexagonal YMnO$_3$ were resolved in all three spatial dimensions by piezoresponse force microscopy. Their topology is dominated by electrostatic effects with a range of 100 unit cells and…

Materials Science · Physics 2015-05-27 Tobias Jungk , Ákos Hoffmann , Manfred Fiebig , Elisabeth Soergel

InMnO$_3$ is a peculiar member of the hexagonal manganites h-RMnO$_3$ (where R is a rare earth metal element), showing crystalline, electronic and magnetic properties at variance with the other compounds of the family. We have studied high…

Materials Science · Physics 2015-03-19 X. Fabrèges , I. Mirebeau , S. Petit , P. Bonville , A. A. Belik

Hexagonal Dy(0.5)Y(0.5)MnO3, a multiferroic rare-earth manganite with geometrically frustrated antiferromagnetism, has been investigated with single-crystal neutron diffraction measurements. Below 3.4 K magnetic order is observed on both…

Strongly Correlated Electrons · Physics 2011-08-29 Joel S. Helton , Deepak K. Singh , Harikrishnan S. Nair , Suja Elizabeth

As the result of the high-temperature improper ferroelectric transition occurring in YMnO3 and other hexagonal manganites a striking domain pattern was observed: an emergence of six domains of alternating polarization from one point in a…

Strongly Correlated Electrons · Physics 2014-01-31 Bruno Mettout , Pierre Toledano , Martin Lilienblum , Manfred Fiebig

Magnetic monopoles and toroidal order are compelling features that have long been theorized but remain elusive in real materials. Multiferroic hexagonal ferrites are an interesting realization of frustrated triangular lattice, where…

Strongly Correlated Electrons · Physics 2020-01-08 Francesco Foggetti , Sang-Wook Cheong , Sergey Artyukhin

We investigated the electronic structure of multiferroic hexagonal RMnO3 (R = Gd, Tb, Dy, and Ho) thin films using both optical spectroscopy and first-principles calculations. Using artificially stabilized hexagonal RMnO3, we extended the…

Strongly Correlated Electrons · Physics 2010-05-17 W. S. Choi , D. G. Kim , S. S. A. Seo , S. J. Moon , D. Lee , J. H. Lee , H. S. Lee , D. -Y. Cho , Y. S. Lee , P. Murugavel , Jaejun Yu , T. W. Noh

Hexagonal HoMnO$_{3}$ is a frustrated antiferromagnet (T$_{N}$=72 K) ferroelectric (T$_{C}$=875 K) in which these two order parameters are coupled. Our neutron measurements of the spin wave dispersion for the S=2 Mn$^{3+}$ on the layered…

Strongly Correlated Electrons · Physics 2009-11-11 O. P. Vajk , M. Kenzelmann , J. W. Lynn , S. B. Kim , S. -W. Cheong

We report a detailed high-resolution powder neutron diffraction investigation of the structural behaviour of the multiferroic hexagonal polymorph of YMnO3 between room temperature and 1403 K. The study was aimed at resolving previous…

Materials Science · Physics 2015-05-19 Alexandra S. Gibbs , Kevin S. Knight , Philip Lightfoot

Using first-principles calculations we examine the band structures of ferromagnetic hexagonal manganites $\mathrm{YXO_3}$ (X=V, Cr, Mn, Fe and Co) in the nonpolar nonsymmorphic $P6_3/mmc$ space group. For $\mathrm{YVO_3}$ and…

Materials Science · Physics 2019-07-03 Sophie F. Weber , Sinéad M. Griffin , Jeffrey B. Neaton

The structural and magnetic properties of the hexagonal four-layer form of SrMnO$_3$ have been investigated by combining magnetization measurements, electron diffraction and high-resolution synchrotron X-ray and neutron powder diffraction.…

Strongly Correlated Electrons · Physics 2007-05-23 A. Daoud-Aladine , C. Martin , L. C. Chapon , M. Hervieu , K. S. Knight , M. Brunelli , P. G. Radaelli

Emergent topological phenomena in multiferroic materials arise from the intricate coupling between structural, electric, and magnetic order parameters. Hexagonal manganites provide a paradigmatic platform for such studies. These compounds…

Materials Science · Physics 2025-10-16 Aaron Merlin Müller , Lukas Heckendorn , Manfred Fiebig , Thomas Lottermoser

The ferroelectric phase of the multiferroic hexagonal manganites (h-ReMnO3) has been reported to undergo a series of magnetic transitions involving long-range ordering/reorientation of 4fRe3+ and/or 3dMn3+ spins below room temperature.…

A series of manganites Tb1-xHoxMnO3 (0<=x<=0.6) with orthorhombic structure are synthesized and detailed investigations on their multiferroicity are performed. Successive magnetic transitions upon temperature variation are evidenced for all…

Strongly Correlated Electrons · Physics 2010-04-19 C. L. Lu , S. Dong , K. F. Wang , J. -M. Liu

The optical spectra in the family of multiferroic manganites RMnO3 is a great puzzle. Current models can not explain the fact that two strong electromagnons are present in the non-collinear spin cycloidal phase, with only one electromagnon…

Strongly Correlated Electrons · Physics 2013-03-05 Markku P. V. Stenberg , Rogério de Sousa
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