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We analyze, through resonant photoluminescence, the spin dynamics of an individual magnetic atom (Mn) coupled to a hole in a semiconductor quantum dot. The hybrid Mn-hole spin and the positively charged exciton in a CdTe/ZnTe quantum dot…

Mesoscale and Nanoscale Physics · Physics 2017-06-21 A. Lafuente-Sampietro , H. Boukari , L. Besombes

We have investigated the spin preparation efficiency by optical pumping of individual Mn atoms embedded in CdTe/ZnTe quantum dots. Monitoring the time dependence of the intensity of the fluorescence during the resonant optical pumping…

Mesoscale and Nanoscale Physics · Physics 2012-06-18 C. Le Gall , R. S. Kolodka , C. Cao , H. Boukari , H. Mariette , J. Fernández-Rossier , L. Besombes

Using the emission of the positively charged exciton as a probe, we analyze the dynamics of the optical pumping and the dynamics of the relaxation of a Mn spin exchange-coupled with a confined hole spin in a II-VI semiconductor quantum dot.…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 B. Varghese , H. Boukari , L. Besombes

We analyze the spin dynamics of an individual magnetic atom (Mn) inserted in a II-VI semiconductor quantum dot under resonant optical excitation. In addition to standard optical pumping expected for a resonant excitation, we show that for…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 S. Jamet , H. Boukari , L. Besombes

We report on the coherent dynamics of the spin of an individual magnetic atom coupled to carriers in a semiconductor quantum dot which has been investigated by resonant photoluminescence of the positively charged exciton (X+). We…

Mesoscale and Nanoscale Physics · Physics 2015-09-02 A. Lafuente-Sampietro , H. Boukari , L. Besombes

We investigate the optical properties of neutral excitons in CdTe/ZnTe quantum dots containing a single Ni2+ ion. We show that the photoluminescence spectra provide a direct spectroscopic signature of strain induced mixing of the Ni2+ spin…

Mesoscale and Nanoscale Physics · Physics 2026-03-19 K. E. Polczynska , S. Karouaz , W. Pacuski , L. Besombes

The spin dynamics of a single Mn atom in a laser driven CdTe quantum dot is addressed theoretically. Recent experimental results\cite{Le-Gall_PRL_2009,Goryca_PRL_2009,Le-Gall_PRB_2010}show that it is possible to induce Mn spin polarization…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 C. L. Cao , L. Besombes , J. Fernández-Rossier

We report on the resonant optical pumping of the |\pm1> spin states of a single Mn dopant in an InAs/GaAs quantum dot embedded itself in a charge tuneable device. The experiment relies on a "W" scheme of transitions reached when a suitable…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Emmanuel Baudin , Emile Benjamin , Aristide Lemaître , Olivier Krebs

We present the photoluminescence excitation study of the self-assembled CdTe/ZnTe quantum dots doped with manganese ions. We demonstrate the identification method of spontaneously coupled quantum dots pairs containing single Mn2+ ions. As…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 M. Koperski , M. Goryca , T. Kazimierczuk , T. Smoleński , A. Golnik , P. Wojnar , P. Kossacki

We show that through the resonant optical excitation of spin-polarized excitons into CdMnTe magnetic quantum dots, we can induce a macroscopic magnetization of the Mn impurities. We observe very broad (4 meV linewidth) emission lines of…

Soft Condensed Matter · Physics 2009-11-10 T. Gurung , S. Mackowski , H. E. Jackson , L. M. Smith , W. Heiss , J. Kossut , G. Karczewski

We review spin properties of semiconductor quantum dots and their effect on optical spectra. Photoluminescence and other types of spectroscopy are used to probe neutral and charged excitons in individual quantum dots with high spectral and…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Allan S. Bracker , Daniel Gammon , Vladimir L. Korenev

For future quantum technologies the combination of a long quantum state lifetime and an efficient interface with external optical excitation are required. In solids, the former is for example achieved by individual spins, while the latter…

We study the dynamics of the spin system that consist of a positively charged II-VI semiconductor quantum dot doped with a single Cr$^+$ ion. The resonant photoluminescence (PL) of the positively charged exciton coupled with the Cr$^+$ spin…

Mesoscale and Nanoscale Physics · Physics 2022-08-17 V. Tiwari , M. Morita T. Inoue , S. Ando S. Kuroda , H. Boukari , L. Besombes

A hight degree of spin polarization is achieved for a Mn atom localized in a semiconductor quantum dot using quasi-resonant optical excitation at zero magnetic field. Optically created spin polarized carriers generate an energy splitting of…

Other Condensed Matter · Physics 2012-06-18 C. Le Gall , L. Besombes , H. Boukari , R. Kolodka , H. Mariette , J. Cibert

We present a magneto-optical study of individual self-assembled CdSe/ZnSe quantum dots doped with single Mn$^{2+}$ ions. Properties of the studied dots are analyzed analogously to more explored system of Mn-doped CdTe/ZnTe dots.…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Tomasz Smoleński

We present the results of a comprehensive magneto-optical characterization of single CdTe quantum dots containing a few Mn2+ ions. We find that some quantum dots exhibit an unexpected evolution of excitonic photoluminescence spectrum with…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Maciej Koperski , Tomasz Smoleński , Mateusz Goryca , Piotr Wojnar , Marek Potemski , Piotr Kossacki

We report on the dynamics of optically induced nuclear spin polarization in individual CdTe/ZnTe quantum dots loaded with one electron by modulation doping. The fine structure of the hot trion (charged exciton $X^-$ with an electron in the…

Mesoscale and Nanoscale Physics · Physics 2012-06-18 C. Le Gall , A. Brunetti , H. Boukari , L. Besombes

We present a comprehensive experimental and theoretical studies of photoluminescence of single CdMnTe quantum dots with Mn content x ranging from 0.01 to 0.2. We distinguish three stages of the equilibration of the exciton-Mn ion spin…

Mesoscale and Nanoscale Physics · Physics 2013-07-23 Ł. Kłopotowski , Ł. Cywiński , M. Szymura , V. Voliotis , R. Grousson , P. Wojnar , K. Fronc , T. Kazimierczuk , A. Golnik , G. Karczewski , T. Wojtowicz

A system of two coupled CdTe quantum dots, one of them containing a single Mn ion, was studied in continuous wave and modulated photoluminescence, photoluminescence excitation, and photon correlation experiments. Optical writing of…

Other Condensed Matter · Physics 2011-01-13 M. Goryca , T. Kazimierczuk , M. Nawrocki , A. Golnik , J. A. Gaj , P. Kossacki , P. Wojnar , G. Karczewski

We demonstrate that the spin of a Cr atom in a quantum dot (QD) can be controlled optically and we discuss the main properties of this single spin system. The photoluminescence of individual Cr-doped QDs and their evolution in magnetic…

Mesoscale and Nanoscale Physics · Physics 2019-11-27 L. Besombes , H. Boukari , V. Tiwari , A. Lafuente-Sampietro , S. Kuroda , K. Makita
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