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Low-dimensional magnetic materials with spin-$\frac{1}{2}$ moments can host a range of exotic magnetic phenomena due to the intrinsic importance of quantum fluctuations to their behavior. Here, we report the structure, magnetic structure…

The magnetic properties of a new family of molecular-based quasi-two dimension $S=1/2$ Heisenberg antiferromagnets are reported. Three compounds, ($Cu(pz)_2(ClO_4)_2$, $Cu(pz)_2(BF_4)_2$, and $[Cu(pz)_2(NO_3)](PF_6)$) contain similar planes…

We report structural and magnetic properties of the spin-$\frac12$ quantum antiferromagnet Cu[C$_6$H$_2$(COO)$_4$][C$_2$H$_5$NH$_3$]$_2$ by means of single-crystal x-ray diffraction, magnetization, heat capacity, and electron spin resonance…

We present an investigation of the effect of randomizing exchange strengths in the $S=1/2$ square lattice quasi-two-dimensional quantum Heisenberg antiferromagnet (QuinH)$_2$Cu(Cl$_{x}$Br$_{1-x}$)$_{4}\cdot$2H$_2$O (QuinH$=$Quinolinium,…

We present an investigation of magnetic ordering in the two-dimensional S=1/2 quantum magnet Cu(Pz)_2(ClO_4)_2 using specific heat and zero field muon-spin relaxation (\mu^+SR). The magnetic contribution to the specific heat is consistent…

We investigate the structural and magnetic properties of the new quantum magnet BaCuTe$_2$O$_6$. This compound is synthesized for the first time in powder and single crystal form. Synchrotron X-ray and neutron diffraction reveal a cubic…

Strongly Correlated Electrons · Physics 2021-03-17 A. Samartzis , D. Khalyavin , A. T. M. N. Islam , S. Chillal , K. Siemensmeyer , K. Prokes , D. J. Voneshen , A. Senyshyn , B. Lake

Using the exact solution in terms of the generalized classical transfer matrix method we presented a detailed analysis of the magnetic properties and ground state structure of the simplified model of the single-chain magnet, trimetallic…

Statistical Mechanics · Physics 2014-03-12 Stefano Bellucci , Vadim Ohanyan , Onofre Rojas

Field-induced magnetic ordering in the structurally disordered quantum magnets Ni(Cl$_{1-x}$Br$_x$)$_2$$\cdot$4SC(NH$_2$)$_2$, $x=8$% and 13%, is studied by means of neutron diffraction. The order parameter critical exponent is found to be…

Strongly Correlated Electrons · Physics 2015-06-17 E. Wulf , D. Huvonen , J. -W. Kim , A. Paduan-Filho , E. Ressouche , S. Gvasaliya , V. Zapf , A. Zheludev

Manganese-rich Heusler compounds are attracting much interest in the context of spin transfer torque and rare-earth free hard magnets. Here we give a comprehensive overview of the magnetic properties of non-centrosymmetric cubic…

Materials Science · Physics 2014-12-10 Lukas Wollmann , Stanislav Chadov , Jürgen Kübler , Claudia Felser

Low-dimensional quantum magnets are a versatile materials platform for studying the emergent many-body physics and collective excitations that can arise even in systems with only short-range interactions. Understanding their low-temperature…

The magnetic ground state of two isostructural coordination polymers (i) the quasi two-dimensional S = 1/2 square-lattice antiferromagnet [Cu(HF$_{2}$)(pyrazine)$_{2}$]SbF$_{6}$; and (ii) a new compound…

Depending on the crystal growth conditions, an orthorhombic (O-type) or a tetragonal (T-type) structure can be found in the solid solution Cs2CuCl4-xBrx (0 < x < 4). Here we present measurements of the temperature-dependent magnetic…

We report on a comprehensive characterization of the newly synthesized Cu$^{2+}$-based molecular magnet [Cu(pz)$_2$(2-HOpy)$_2$](PF$_6$)$_2$ (CuPOF), where pz = C$_4$H$_4$N$_2$ and 2-HOpy = C$_5$H$_4$NHO. From a comparison of theoretical…

The magnetic structures of small clusters of Fe, Mn, and Cr supported on a Cu(111) surface have been studied with non-collinear first principles theory. Different geometries such as triangles, pyramids and wires are considered and the…

The synthesis of molecular magnets has undergone rapid progress in recent years. Each of the identical molecular units can contain as few as two and up to several dozens of paramagnetic ions (spins). Although these materials appear as…

Strongly Correlated Electrons · Physics 2009-11-11 J. Schnack

We present a numerical study of the spin-1/2 bilayer Heisenberg antiferromagnet with random interlayer dimer dilution. From the temperature dependence of the uniform susceptibility and a scaling analysis of the spin correlation length we…

Disordered Systems and Neural Networks · Physics 2009-11-07 O. P. Vajk , M. Greven

We investigated the crystal and magnetic structures of the spin-1/2 frustrated antiferromagnet Cu3Mo2O9 in which the spin system consists of antiferromagnetic chains and dimers. The space group at room temperature has been reported to be…

Our experimental (neutron diffraction, M\"ossbauer spectroscopy, magnetic susceptibility, specific heat) and numerical studies on the evolution of short- and long-range magnetic order in $\gamma_{\rm II}$-Li\(_2\)FeSiO\(_4\) suggest a…

Strongly Correlated Electrons · Physics 2025-01-20 W. Hergett , N. Bouldi , M. Jonak , C. Neef , C. Ritter , M. Abdel-Hafiez , F. Seewald , H. -H. Klauss , M. W. -Haverkort , R. Klingeler

The magnetic susceptibility and magnetization of two new layered S=1/2 Heisenberg antiferromagnets with moderate exchange are reported. The two isostructural compounds, (2-amino-5-chloropyridinium)2CuBr4 ((5CAP)2CuBr4) and…

Materials Science · Physics 2009-11-07 F. M. Woodward , A. S. Albrecht , C. M. Wynn , C. P. Landee , M. M. Turnbull

Long range magnetic ordering in the quasi-one-dimensional random-bond antiferromagnet BaCu$_2$(Si$_{1-x}$Ge$_{x}$)$_2$O$_7$ is studied in $\mu$SR experiments as a function of disorder strength. Compared to the disorder-free parent…

Strongly Correlated Electrons · Physics 2014-12-04 M. Thede , T. Haku , T. Masuda , C. Baines , E. Pomjakushina , G. Dhalenne , A. Revcolevschi , E. Morenzoni , A. Zheludev
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