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The rapid and efficient exchange of ions between porous electrodes and aqueous solutions is important in many applications, such as electrical energy storage by super-capacitors, water desalination and purification by capacitive…

Chemical Physics · Physics 2015-05-14 P. M. Biesheuvel , M. Z. Bazant

In this paper we report the theory describing the electro-osmotic flow in charged nanopores with constant radius and charge density driven by alternating current. We solve the ion and solution transport in unsteady conditions as described…

Chemical Physics · Physics 2018-10-17 J. Catalano , P. M. Biesheuvel

Ionic Current Rectification (ICR) can appear in nanopores, causing a diode-like behavior that originates from different efficiency of ion transport through the pore channel with respect to the applied voltage bias polarity. This effect is…

Electrostatic charging of insulating fine particles can be responsible for numerous phenomena ranging from lightning in volcanic plumes to dust explosions. However, even basic aspects of how fine particles become charged are still unclear.…

Materials Science · Physics 2018-04-04 Victor Lee , Nicole M. James , Scott Waitukaitis , Heinrich M. Jaeger

Slow ionic transport and high voltage drop (IR drop) of homogeneous porous electrodes are the critical causes of severe performance degradation of lithium-ion (Li-ion) batteries under high charging rates. Herein, we demonstrate that a…

Materials Science · Physics 2021-07-30 Chenxi Sui , Yao-Yu Li , Xiuqiang Li , Genesis Higueros , Keyu Wang , Wanrong Xie , Po-Chun Hsu

Understanding how electrolyte-filled porous electrodes respond to an applied potential is important to many electrochemical technologies. Here, we consider a model supercapacitor of two blocking cylindrical pores on either side of a…

Soft Condensed Matter · Physics 2022-04-05 Jie Yang , Mathijs Janssen , Cheng Lian , René van Roij

Adding porosity to battery electrodes is believed to be universally useful for adding space to accommodate volumetric expansion, electrolyte access to all active materials, helping to mitigate poor C-rate performance for thicker electrodes…

Applied Physics · Physics 2020-08-26 Sally O'Hanlon , David McNulty , Ruiyuan Tian , Jonathan Coleman , Colm O'Dwyer

The forced intrusion of water in hydrophobic nanoporous pulverulent material is of interest for quick storage of energy. With nanometric pores the energy storage capacity is controlled by interfacial phenomena. With subnanometric pores, we…

Soft Condensed Matter · Physics 2015-07-03 Millán Michelin-Jamois , Cyril Picard , Gérard Vigier , Elisabeth Charlaix

Nanopores spanning synthetic membranes have been used as key components in proof-of-principle nanofluidic applications, particularly those involving manipulation of biomolecules or sequencing of DNA. The only practical way of manipulating…

Mesoscale and Nanoscale Physics · Physics 2016-09-21 Tom Chou

With controlled ionic current rectification (ICR) achieved through a strategically designed non-uniform surface charge distribution, short unipolar nanopores exhibit promising applications in nanofluidic sensors, ionic circuits, and ion…

Chemical Physics · Physics 2025-12-08 Hongwen Zhang , Long Ma , Di Liu , Tianyi Sui , Zuzanna S. Siwy , Yinghua Qiu

Next-generation high-energy-density batteries require ideally stable metal anodes, for which smooth metal deposits during battery recharging are considered a sign of interfacial stability that can ensure high efficiency and long cycle life.…

Materials Science · Physics 2022-01-11 Bingyuan Ma , Peng Bai

Ionic transport in nanopores or nanochannels is key to many cellular processes and is now being explored as a method for DNA/polymer sequencing and detection. Although apparently simple in its scope, the study of ionic dynamics in confined…

Mesoscale and Nanoscale Physics · Physics 2013-06-13 Andrew Meyertholen , Massimiliano Di Ventra

We present coarse-grained simulation results for enhanced ion diffusion in a charged nanopore grafted with ionomer sidechains. The pore surface is hydrophobic and its diameter is varied from 2.0 nm to 3.7 nm. The sidechains have from 2 to…

Soft Condensed Matter · Physics 2017-05-02 Elshad Allahyarov , Hartmut Löwen , Philip L. Taylor

The number of precise conductance measurements in nanopores is quickly growing. In order to clarify the dominant mechanisms at play and facilitate the characterization of such systems for which there is still no clear consensus, we propose…

Soft Condensed Matter · Physics 2018-07-25 Manoel Manghi , John Palmeri , Khadija Yazda , Francois Henn , Vincent Jourdain

We revisit the classical problem of flow of electrolyte solutions through charged capillary nanopores or nanotubes as described by the capillary pore model (also called "space charge" theory). This theory assumes very long and thin pores…

Chemical Physics · Physics 2019-08-16 P. B. Peters , R. van Roij , M. Z. Bazant , P. M. Biesheuvel

In the realm of battery charging, several complex aspects demand meticulous attention, including thermal management, capacity degradation, and the need for rapid charging while maintaining safety and battery lifespan. By employing the…

Systems and Control · Electrical Eng. & Systems 2024-09-19 Jorge Espin , Dong Zhang , Daniele Toti , Andrea Pozzi

Ionic current rectification (ICR) of charged conical nanopores has various applications in fields including nanofluidics, bio-sensing, and energy conversion, whose function is closely related to the dynamic response of nanopores. The…

Chemical Physics · Physics 2024-10-29 Zhe Liu , Long Ma , Hongwen Zhang , Jiakun Zhuang , Jia Man , Zuzanna S. Siwy , Yinghua Qiu

We report on the experimental studies of laser driven ion acceleration from double-layer target where a near-critical density target with a few-micron thickness is coated in front of a nanometer thin diamond-like carbon foil. A significant…

There is a growing interest in the development of functional metal oxides with mixed ionic electronic conduction for their application in different strategic fields. In particular, ionic transport-related phenomena are of primary importance…

Materials Science · Physics 2018-12-03 Francesco Chiabrera , Inigo Garbayo , Albert Tarancon

In the present work we propose "nanofluid filled enclosures" as potential photo-thermal energy conversion and sensible heat storage devices. Herein, the optical charging of the nanofluid has been modeled as "solar radiant energy -…

Applied Physics · Physics 2022-03-15 Inderpreet Singh , Satbir Singh Sehgal , Vikrant Khullar