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A method for decelerating a continuous beam of neutral polar molecules is theoretically demonstrated. This method utilizes non-uniform, static electric fields and regions of adiabatic population transfer to generate a mechanical force that…

Atomic Physics · Physics 2015-05-13 Eric R. Hudson

A new type of decelerator is presented where polar neutral molecules are guided and decelerated using the principle of traveling electric potential wells, such that molecules are confined in stable three-dimensional traps throughout. This…

Atomic Physics · Physics 2010-05-24 Andreas Osterwalder , Samuel A. Meek , Georg Hammer , Henrik Haak , Gerard Meijer

We describe the combination of buffer-gas cooling with electrostatic velocity filtering to produce a high-flux continuous guided beam of internally cold and slow polar molecules. In a previous paper (L.D. van Buuren et al.,…

Ultracold molecules represent a fascinating research frontier in physics and chemistry, but it has proven challenging to prepare dense samples at low velocities. Here we present a solution to this goal by a non-conventional approach dubbed…

Atomic Physics · Physics 2018-12-04 Xing Wu , Thomas Gantner , Manuel Koller , Martin Zeppenfeld , Sotir Chervenkov , Gerhard Rempe

Polar heavy-atom molecules have been well recognized as promising candidates for precision measurements and tests of fundamental physics. A much slower molecular beam to increase the interaction time should lead to a more sensitive…

Atomic Physics · Physics 2018-04-11 Yanning Yin , Supeng Xu , Meng Xia , Yong Xia , Jianping Yin

We here report on the experimental realization of a microwave decelerator for neutral polar molecules, suitable for decelerating and focusing molecules in high-field-seeking states. The multi-stage decelerator consists of a cylindrical…

Chemical Physics · Physics 2015-06-04 Simon Merz , Nicolas Vanhaecke , Wolfgang Jäger , Melanie Schnell , Gerard Meijer

Employing a two-stage cryogenic buffer gas cell, we produce a cold, hydrodynamically extracted beam of calcium monohydride molecules with a near effusive velocity distribution. Beam dynamics, thermalization and slowing are studied using…

Atomic Physics · Physics 2017-09-13 Hsin-I Lu , Julia Rasmussen , Matthew J. Wright , Dave Patterson , John M. Doyle

Cryogenic buffer-gas beams are a promising method for producing bright sources of cold molecular radicals for cold collision and chemical reaction experiments. In order to use these beams in studies of reactions with controlled collision…

Chemical Physics · Physics 2015-06-18 M. I. Fabrikant , Tian Li , N. J. Fitch , N. Farrow , Jonathan D. Weinstein , H. J. Lewandowski

Using frequency-chirped radiation pressure slowing, we precisely control the velocity of a pulsed CaF molecular beam down to a few m/s, compressing its velocity spread by a factor of 10 while retaining high intensity: at a velocity of…

Atomic Physics · Physics 2017-04-05 S. Truppe , H. J. Williams , N. J. Fitch , M. Hambach , T. E. Wall , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

Recently, a decelerator for neutral polar molecules has been presented that operates on the basis of macroscopic, three-dimensional, traveling electrostatic traps (Osterwalder et al., Phys. Rev. A 81, 051401 (2010)). In the present paper, a…

There is substantial interest in producing samples of ultracold molecules for possible applications in quantum computation, quantum simulation of condensed matter systems, precision measurements, controlled chemistry, and high precision…

Atomic Physics · Physics 2013-05-30 J. F. Barry , E. S. Shuman , E. B. Norrgard , D. DeMille

Stark deceleration enables the production of cold and dense molecular beams with applications in trapping, collisional studies, and precision measurement. Improving the efficiency of Stark deceleration, and hence the achievable molecular…

Chemical Physics · Physics 2020-07-22 David Reens , Hao Wu , Alexander Aeppli , Anna McAuliffe , Piotr Wcisło , Tim Langen , Jun Ye

We demonstrate experimentally the guiding of cold and slow ND3 molecules along a thin charged wire over a distance of ~0.34 m through an entire molecular beam apparatus. Trajectory simulations confirm that both linear and quadratic…

Atomic and Molecular Clusters · Physics 2011-12-19 M. Strebel , S. Spieler , F. Stienkemeier , M. Mudrich

We present a robust, continuous molecular decelerator that employs high magnetic fields and few optical pumping steps. CaOH molecules are slowed, accumulating at low velocities in a range sufficient for loading both magnetic and…

Ultracold molecular gases are promising as an avenue to rich many-body physics, quantum chemistry, quantum information, and precision measurements. This richness, which flows from the complex internal structure of molecules, makes the…

Atomic Physics · Physics 2015-06-18 A. M. Jayich , A. C. Vutha , M. T. Hummon , J. V. Porto , W. C. Campbell

We present an analysis of the deceleration and trapping of heavy diatomic molecules in low-field seeking states by a moving electric potential. This moving potential is created by a 'ring-decelerator', which consists of a series of…

We present a method which delivers a continuous, high-density beam of slow and internally cold polar molecules. In our source, warm molecules are first cooled by collisions with a cryogenic helium buffer gas. Cold molecules are then…

Chemical Physics · Physics 2009-01-23 L. D. van Buuren , C. Sommer , M. Motsch , S. Pohle , M. Schenk , J. Bayerl , P. W. H. Pinkse , G. Rempe

A Stark decelerator is an effective tool for controlling motional degrees of freedom of polar molecules. Due to technical limitations, many of the current Stark decelerators focus on molecules in low-field-seeking quantum states and are…

Atomic Physics · Physics 2017-05-25 Demitri Y. Balabanov , Liam M. Duffy

A microstructured array of 1254 electrodes on a substrate has been configured to generate an array of local minima of electric field strength with a periodicity of 120 $\mu$m about 25 $\mu$m above the substrate. By applying sinusoidally…

Atomic Physics · Physics 2009-05-20 Samuel A Meek , Horst Conrad , Gerard Meijer

We explore a technique for decelerating molecules using a static magnetic field and optical pumping. Molecules travel through a spatially varying magnetic field and are repeatedly pumped into a weak-field seeking state as they move towards…

Atomic Physics · Physics 2016-09-20 N. J. Fitch , M. R. Tarbutt
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