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High quality factor optical nanostructures provide great opportunity to enhance nonlinear optical processes such as third harmonic generation. However, the field enhancement in these high quality factor structures is typically accompanied…

Optics · Physics 2023-11-22 Claudio U. Hail , Lior Michaeli , Harry A. Atwater

Plasmons in atomically thin materials offer a compelling route to trigger nonlinear light-matter interactions through extreme optical confinement in the two-dimensional (2D) limit. However, optical nonlocality in plasmons is typically…

Mesoscale and Nanoscale Physics · Physics 2025-12-23 Line Jelver , Joel D. Cox

Notwithstanding its long history, the study of nonlinear optics from metal surfaces is still an active field of research. For instance, in view of the presence of absorption questions remain concerning the possibility of significantly…

Nonlinear nanophotonics leverages engineered nanostructures to funnel light into small volumes and intensify nonlinear optical processes with spectral and spatial control. Due to its intrinsically large and electrically tunable nonlinear…

Plasmonic nanoantennas have been recently proposed to boost nonlinear optical processes. In a metal dipole nanoantenna with a dielectric nanoparticle placed in the gap, the linear field enhancement can be exploited to enhance third harmonic…

Optics · Physics 2017-04-13 Antonino Calà Lesina , Pierre Berini , Lora Ramunno

The emergence of strong-field nanoplasmonics brings extreme laser field-matter interaction into the realm of nanoscale science, unveiling exciting new physics. Highly nonlinear interaction is enabled by tightly confined electric fields in…

Optics · Physics 2013-09-02 Shawn Sederberg , Abdulhakem Y. Elezzabi

Frequency conversion processes, such as second- and third-harmonic generation, are one of the most common effects in nonlinear optics which offer many opportunities for photonics, chemistry, material science, characterization, and…

Optics · Physics 2017-06-26 Alexander Krasnok , Mykhailo Tymchenko , Andrea Alu

Nonlinear nanostructured surfaces provide a paradigm shift in nonlinear optics with new ways to control and manipulate frequency conversion processes at the nanoscale, also offering novel opportunities for applications in photonics,…

Applied Physics · Physics 2019-11-07 Kirill Koshelev , Yutao Tang , Kingfai Li , Duk-Yong Choi , Guixin Li , Yuri Kivshar

We study nonlinear effects in two-dimensional photonic metasurfaces supporting topologically-protected helical edge states at the nanoscale. We observe strong third-harmonic generation mediated by optical nonlinearities boosted by…

Optical response of free-electron gas leads to inherent nonlinear optical behaviour of nanostructured plasmonic materials enabled via both strong local field enhancements and inherent complex electron dynamics. We present a comprehensive…

Collective responses of localized surface plasmon resonances, known as surface lattice resonances (SLRs) in metal nanoparticle arrays, can lead to high quality factors (~100), large local-field enhancements and strong light-matter…

Optics · Physics 2018-05-23 Mikko J. Huttunen , Payman Rasekh , Robert W. Boyd , Ksenia Dolgaleva

The search for miniaturized components for nonlinear optical processes needs a way to overcome the efficiency loss due to the effective size reduction of the active medium. We investigate here a combination of a nanosized nonlinear…

We study the effect of nonlocal optical response on the optical properties of metallic nanowires, by numerically implementing the hydrodynamical Drude model for arbitrary nanowire geometries. We first demonstrate the accuracy of our…

Mesoscale and Nanoscale Physics · Physics 2012-02-07 Giuseppe Toscano , Søren Raza , Antti-Pekka Jauho , N. Asger Mortensen , Martijn Wubs

Optical properties of periodic arrays of nanoholes of a triangular shape with experimentally realizable parameters are examined in both linear and nonlinear regimes. Utilizing fully vectorial three-dimensional approach based on the…

Mesoscale and Nanoscale Physics · Physics 2020-03-18 Elena Drobnyh , Maxim Sukharev

We perform a study of the achievable field enhancement of plasmonic cascade nanolenses in the quantum and classical regimes, and explore the limits enforced at larger sizes by retardation and at smaller sizes by nonlocality and other…

Optics · Physics 2017-12-25 Jamie M. Fitzgerald , Vincenzo Giannini

Plasmon resonances are known to amplify the electromagnetic fields near metallic nanostructures. Therefore, they are considered to provide a promising scheme to generate extreme-ultraviolet harmonics, using low power drivings. During…

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

We present a new theoretical approach to the study of second and third harmonic generation from metallic nanostructures and nanocavities filled with a nonlinear material, in the ultrashort pulse regime. We model the metal as a two-component…

The plasmon response of metallic nanostructures is anticipated to exhibit nonlocal dynamics of the electron gas when exploring the true nanoscale. We extend the local-response approximation (based on Ohm's law) to account for a general…

Mesoscale and Nanoscale Physics · Physics 2014-03-04 N. Asger Mortensen

We present theoretical investigations of high-order harmonic generation (HHG) resulting from the interaction of noble gases with localized surface plasmons. These plasmonic fields are produced when a metal nanoparticle is subject to a…

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