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Related papers: Mixed valency and site-preference chemistry for Ce…

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We have measured the magnetic properties of a mixed valency iron phosphate. It presents an original structure with crossed chains containing Fe II and orthogonal to the longest direction of the crystallites. Microstructural investigations…

Materials Science · Physics 2015-05-19 Laure Adam , Alain Pautrat , Olivier Perez , Philippe Boullay

By performing density functional calculations, we find a giant magnetocrystalline anisotropy (MCA) constant in abundant element cerium (Ce) substituted M-type hexaferrite, in the energetically favorable strontium site, assisted by a quantum…

Materials Science · Physics 2023-08-21 Churna Bhandari , Durga Paudyal

The electronic structures of element cerium under high pressure remain unclear all the time. We tried to calculate the electronic structures of $\alpha'$, $\alpha"$, and $\epsilon$-Ce which only exist in the presence of pressure, by using…

Strongly Correlated Electrons · Physics 2018-11-02 Haiyan Lu , Li Huang

In the pressure range 5-12 GPa the fractional valence of cerium is independent of pressure because of the coexistence of two or more structural phases. The observation of a single crystallographic structure in this pressure range arises…

Materials Science · Physics 2008-02-03 J. Röhler

A systematic analysis of thermodynamic properties performed on Ce-base exemplary compounds allows to identify different types of behaviors as the system approaches the quantum critical region. They are recognized in the respective magnetic…

Strongly Correlated Electrons · Physics 2011-08-02 Julian G. Sereni

At ambient temperatures, CeRuSn exhibits an extraordinary structure with a coexistence of two types of Ce ions in a metallic environment, namely trivalent Ce3+ and intermediate valent Ce(4-x)+. Charge ordering produces a doubling of the…

Strongly Correlated Electrons · Physics 2012-02-24 R. Feyerherm , E. Dudzik , S. Valencia , J. A. Mydosh , Y. -K. Huang , W. Hermes , R. Pöttgen

The nature of the elemental cerium phases, undergoing an isostructural volume collapse transition, cannot be understood using conventional solid state concepts. Using the combination of density functional theory and dynamical mean-field…

Strongly Correlated Electrons · Physics 2014-03-18 B. Chakrabarti , M. E. Pezzoli , G. Sordi , K. Haule , G. Kotliar

On the basis of the Ward-Pitaevskii identity, the residual resistivity $\rho_{0}$ is shown to exhibit huge enhancement around the quantum critical point of valence transition in Ce-based heavy electron systems. This explains a sharp peak of…

Strongly Correlated Electrons · Physics 2009-11-07 Kazumasa Miyake , Hideaki Maebashi

We present a density-functional theory (DFT) study of the structural, electronic, and chemical bonding behaviour in germanium (Ge)-doped vanadium dioxide (VO$_2$). Our motivation is to explain the reported increase of the metal-insulator…

Materials Science · Physics 2023-02-03 Peter Mlkvik , Claude Ederer , Nicola A. Spaldin

Tricationic protactinium monofluoride ($^{229}$PaF$^{3+}$) has been proposed as a candidate for probing physics beyond the Standard Model of particle physics. Since studies with $^{229}$PaF$^{3+}$ require significant experimental advances,…

Cerium hydride has a variety of interesting properties, including a known lattice contraction and densification with increasing hydrogen content. However, precise stoichiometric control is not experimentally straightforward and {\it ab…

Materials Science · Physics 2026-02-19 Brenden W. Hamilton , Travis E. Jones , Timothy C. Germann , Benjamin T. Nebgen

Recently, the hydrogen adsorption and diffusion on the CeO2 (111) surface have been a vividly discussed topic because of its outstanding catalytic activity and selectivity in hydrogenation reactions. However, for the strongly reduced CeO2…

Materials Science · Physics 2019-05-01 Xiaoke Li , Joachim Paier , Joachim Sauer

The roles of critical valence fluctuations of Ce and Yb are discussed as a key origin of several anomalies observed in Ce- and Yb-based heavy fermion systems. Recent development of the theory has revealed that a magnetic field is an…

Strongly Correlated Electrons · Physics 2012-02-10 Shinji Watanabe , Kazumasa Miyake

Rare-earth doped form, ceria (CeO2) is of interest as a potential candidate for solid oxide fuel cells (SOFCs) because of its relatively high oxygen ion conductivity at temperatures below 600 {\deg}C. At the present time, computational…

Materials Science · Physics 2016-05-25 Musa Alaydrus , Mamoru Sakaue , Hideaki Kasai

CeRuSn exhibits an extraordinary room temperature structure at 300~K with coexistence of two types of Ce ions, namely trivalent Ce$^{3+}$ and intermediate valent Ce$^{(4-\delta)+}$, in a metallic environment. The ordered arrangement of…

Strongly Correlated Electrons · Physics 2014-07-23 R. Feyerherm , E. Dudzik , K. Prokes , J. A. Mydosh , Y. -K. Huang , R. Pöttgen

Influence of quantum critical point (QCP) of first-order valence transition (FOVT) on Ce- and Yb-based heavy fermions is discussed as a key origin of anomalies such as non-Fermi liquid, metamagnetism, and unconventional superconductivity.…

Strongly Correlated Electrons · Physics 2015-03-17 Shinji Watanabe , Kazumasa Miyake

Enhanced visible light photocatalytic activity of transition metal-doped ceria (CeO2) nanomaterials have experimentally been demonstrated, whereas there are very few reports mentioning the mechanism of this behavior. Here we use…

Materials Science · Physics 2017-02-01 Ke Yang , Dong-Feng Li , Wei-Qing Huang , Liang Xu , Gui-Fang Huang , Shuangchun Wen

Lanthanum and yttrium compounds with composition RE2M2O7 (RE=Y, La; M = Ti, Zr, Hf) have high density and high Z and can be doped with Ce onto the La and Y sites. This makes these compounds good candidates for Ce activated scintillator…

Materials Science · Physics 2012-03-05 A. Chaudhry , A. Canning , R. Boutchko , M. J. Weber , N. Grønbech-Jensen , S. E. Derenzo

Luminescence in Ce doped materials corresponds to a transition from an excited state where the lowest Ce 5d level is filled to the ground state where a single 4f level is filled. We have performed theoretical calculations based on Density…

Materials Science · Physics 2012-03-05 A. Canning , A. Chaudhry , R. Boutchko , N. Grønbech-Jensen

In ceria-based catalysis, the shape of the catalyst particle, which determines the exposed crystal facets, profoundly affects its reactivity. The vibrational frequency of adsorbed carbon monoxide (CO) can be used as a sensitive probe to…