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We present an electron energy loss study using energy filtered TEM of spatially resolved surface plasmon excitations on a silver nanorod of aspect ratio 14.2 resting on a 30 nm thick silicon nitride membrane. Our results show that the…

The real and imaginary parts of the complex refractive index of SixNyHz have been calculated using density functional perturbation theory. Optical spectra for reflectivity, adsorption coefficient, energy-loss function (ELF), and refractive…

In this work we compare Monte Carlo (MC) simulations of electron transport properties with reflection electron energy loss measurements in diamond and graphite films. We assess the impact of different approximations of the dielectric…

A many-body Green's function approach to the microscopic theory of plasmon-enhanced spectroscopy is presented within the context of localized surface-plasmon resonance spectroscopy and applied to investigate the coupling between…

Chemical Physics · Physics 2015-05-14 David J. Masiello , George C. Schatz

An electron beam traversing a structured plasmonic field is shown to undergo diffraction with characteristic angular patterns of both elastic and inelastic outgoing electron components. In particular, a plasmonic {\it grating} (e.g., a…

Mesoscale and Nanoscale Physics · Physics 2016-07-20 F. Javier Garcia de Abajo , Brett Barwick , Fabrizio Carbone

A procedure is developed to rigorously decompose experimental loss spectra of medium-energy electrons reflected from solid surfaces into contributions due to surface and volume electronic excitations. This can be achieved by analysis of two…

Materials Science · Physics 2009-11-11 Wolfgang S. M. Werner

The rich information of electron energy-loss spectroscopy (EELS) comes from the complex inelastic scattering process whereby fast electrons transfer energy and momentum to atoms, exciting bound electrons from their ground states to higher…

The electromagnetic interaction between Ag nanoparticles on the top of the Si substrate and the incident light has been studied by numerical simulations. It is found that the presence of a dielectric layer with different thickness leads to…

Materials Science · Physics 2011-09-22 Xu Rui , Wang Xiao-Dong , Liu Wen , Xu Xiao-Na , Li Yue-Qiang , Ji An , Yang Fu-Hua , Li Jin-Min

The spatial distributions of anti-bonding $\pi^\ast$ and $\sigma^\ast$ states in epitaxial graphene multilayers are mapped using electron energy-loss spectroscopy in a scanning transmission electron microscope. Inelastic channeling…

Materials Science · Physics 2023-06-02 M. Bugnet , M. Ederer , V. K. Lazarov , L. Li , Q. M. Ramasse , S. Löffler , D. M. Kepaptsoglou

Launching of surface plasmons by swift electrons has long been utilized in electron-energy-loss spectroscopy (EELS) to investigate plasmonic properties of ultrathin, or two-dimensional (2D), electron systems. However, its spatio-temporal…

We introduce a method for calculating the dielectric function of nanostructures with an arbitrary band dispersion and Bloch wave functions. The linear response of a dissipative electronic system to an external electromagnetic field is…

Mesoscale and Nanoscale Physics · Physics 2016-06-07 F. Karimi , A. H. Davoody , I. Knezevic

Within the MNPBEM toolbox, we show how to simulate electron energy loss spectroscopy (EELS) of plasmonic nanoparticles using a boundary element method approach. The methodology underlying our approach closely follows the concepts developed…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Ulrich Hohenester

The electronic structures of ABO3 ferroelectrics are calculated within the density functional theory, and their evolution is analyzed as the crystal-field symmetry changes from cubic to rhombohedral via tetragonal phases. Electronic…

Materials Science · Physics 2012-04-19 Sevket Simsek , Amirullah M. Mamedov , Ekmel Ozbay

We present first-principles calculations of silicene/graphene and germanene/graphene bilayers. Various supercell models are constructed in the calculations in order to reduce the strain of the lattice-mismatched bilayer systems. Our…

Mesoscale and Nanoscale Physics · Physics 2013-12-10 Yongmao Cai , Chih-Piao Chuu , C. M. Wei , M. Y. Chou

The electronic excitation spectrum of a material characterises the response to external electromagnetic perturbations through its energy loss function (ELF), which is obtained from several experimental sources that usually do not completely…

Materials Science · Physics 2024-12-20 Fan Cheng , Pablo de Vera , Rafael Garcia-Molina

We study the surface plasmon (SP) resonance energy of isolated spherical Ag nanoparticles dispersed on a silicon nitride substrate in the diameter range 3.5-26 nm with monochromated electron energy-loss spectroscopy. A significant blueshift…

The electronic structure of the heavy fermion compound CeB6 is probed by resonant inelastic soft X-ray scattering using photon energies across the Ce 3d and 4d absorption edges. The hybridization between the localized 4f orbitals and the…

Materials Science · Physics 2012-01-04 M. Magnuson , S. M. Butorin , J. -H. Guo , A. Agui , J. Nordgren , H. Ogasawara , A. Kotani , T. Takahashi , S. Kunii

A new approach is developed to evaluate contribution of the electron-electron correlations into bremsstrahlung from few-electron ions and atoms. Our approach is based on the explicit formula for the electron density distribution in such…

Atomic Physics · Physics 2016-02-16 Alexei M. Frolov , David M. Wardlaw

The optical properties of metallic nanoparticles are dominated by localized surface plasmons (LSPs). Their properties only depend on the constituting material, the size and shape of the nano-object as well as its surrounding medium. In…

The reflectivity of low energy electrons from graphene on copper substrates is studied both experimentally and theoretically. Well-known oscillations in the reflectivity of electrons with energies 0 - 8 eV above the vacuum level are…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 N. Srivastava , Qin Gao , M. Widom , R. M. Feenstra , Shu Nie , K. F. McCarty , I. V. Vlassiouk