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We report the generation of the 5th harmonic of Ti:sapphire, at 160 nm, with more than 4~$\mu$J of pulse energy, and a pulse length of 37 fs with a 1 kHz repetition rate. The VUV pulses are produced using Four-Wave Difference Frequency…

Optics · Physics 2024-04-01 Ruaridh Forbes , Paul Hockett , Quentin Leterrier , Rune Lausten

The combination of electronic sources operating at high frequencies and modern microwave instrumentation has enabled the recent development of chirped-pulse spectrometers for the millimetre and THz bands. This type of instrument can operate…

Instrumentation and Detectors · Physics 2018-10-12 Francis Hindle , Cédric Bray , Daniele Fontanari , Meriem Mouelhi , Arnaud Cuisset , Gael Mouret , Robin Bocquet

A feasible method is proposed to generate isolated attosecond terawatt x-ray radiation pulses in high-gain free-electron lasers. In the proposed scheme, a frequency chirped laser pulse is employed to generate a gradually-varied spacing…

Accelerator Physics · Physics 2017-04-26 Zhen Wang , Chao Feng , Zhentang Zhao

We describe a system for generating frequency-chirped and amplitude-shaped pulses on time scales from sub-nanosecond to ten nanoseconds. The system starts with cw diode-laser light at 780 nm and utilizes fiber-based electro-optical phase…

Atomic Physics · Physics 2016-04-20 Charles E. Rogers , Phillip L. Gould

High energy terahertz pulses are produced by optical rectification (OR) in organic crystals DAST and DSTMS by a Ti:sapphire amplifier system centered at 0.8 microns. The simple scheme provides broadband spectra between 1 and 5 THz, when…

Optics · Physics 2015-06-17 B. Monoszlai , C. Vicario , M. Jazbinsek , C. P. Hauri

We demonstrate a new regime for mid-infrared optical parametric chirped pulse amplification (OPCPA) based on achromatic quasi-phase-matching. Our mid-infrared OPCPA system is based on collinear aperiodically poled lithium niobate (APPLN)…

The mid-infrared spectral region holds growing importance for applications such as gas sensing and spectroscopy. Although compact ultrashort pulse laser sources are essential to enable these applications, their realization in this spectral…

Ultrafast optical excitation with intense mid-infrared and terahertz pulses has emerged as a new tool to control materials dynamically. As most experiments are performed with femtosecond pulse excitation, typical lifetimes of most…

Optics · Physics 2021-02-24 Matthias Budden , Thomas Gebert , Andrea Cavalleri

The growing requirements of pump-probe techniques and nonlinear optics experiments greatly promote the studies of two-color free-electron lasers (FELs). We propose a new method to generate coherent two-color pulses in a high-gain harmonic…

Accelerator Physics · Physics 2018-02-14 Zhouyu Zhao , Heting Li , Qika Jia

A method is proposed for arbitrarily engineering the high-order harmonic generation phase achieved by shaping a laser pulse and employing xuv light or x rays for ionization. This renders the production of bandwidth-limited attosecond pulses…

Atomic Physics · Physics 2011-02-25 Markus C. Kohler , Christoph H. Keitel , Karen Z. Hatsagortsyan

Typically, in Self-Amplified Spontaneous Emission Free Electron Laser (SASE FEL) based short-pulse schemes, pulse duration is limited by FEL coherence time. For hard X-ray FELs, coherence time is in a few hundred attosecond range while for…

Accelerator Physics · Physics 2022-02-09 E. A. Schneidmiller

We demonstrate an efficient procedure for terahertz-wave radiation generation by applying a nonlinear wavelength conversion approach using a mid-infrared pump source. We used a 3.3 {\mu}m dual-chirped optical parametric amplification source…

Active frequency-chirp compensation for a narrowband pulsed Titanium-Sapphire laser system is demonstrated using an intra-cavity electro-optic modulator resulting in improved spectral resolution and stability. With referencing to an optical…

Optics · Physics 2021-12-24 J. Hussels , C. Cheng , E. J. Salumbides , W. Ubachs

High-energy terahertz pulses are challenging to produce due to the low conversion efficiency and limited optical damage threshold of nonlinear crystals. Here, we describe the high-efficiency generation of terahertz radiation pulses with…

Plasma Physics · Physics 2026-04-22 Sida Cao , Matthew R. Edwards

Four-wave mixing processes are ubiquitous in ultrafast optics and the determination of the coefficients of the $\chi^{(3)}$ tensor is thus essential. We introduce a novel time-resolved ultrafast spectroscopic method to characterize the…

We theoretically study chirped four-wave mixing for VUV pulse generation in hollow-core photonic crystal fibers. We predict the generation of sub-10-fs VUV pulses with energy of up to hundreds of microjoule by broad-band chirped idler…

Optics · Physics 2015-07-29 Song-Jin Im

We present a novel technique for producing pulses of laser light whose frequency is arbitrarily chirped. The output from a diode laser is sent through a fiber-optical delay line containing a fiber-based electro-optical phase modulator. Upon…

Atomic Physics · Physics 2009-11-13 C. E. Rogers , M. J. Wright , J. L. Carini , J. A. Pechkis , P. L. Gould

We present a method of producing single attosecond pulses by high-order harmonic generation with multi-cycle nonlinear chirped driver laser pulses. The symmetry of the laser feld in several optical cycles near the pulse center is…

Optics · Physics 2009-06-12 Yang Xiang , Yueping Niu , Yihong Qi , Shangqing Gong

A recirculating frequency-shifting loop (FSL) provides a highly flexible platform for generating coherent optically chirped light with tunable bandwidth, duration, chirp rate and repetition rate. The properties of the chirped light are…

We report a 1 kHz repetition-rate mid-IR (MIR) optical parametric amplifier (OPA) system operating at a central wavelength of 5.2 $\mu$m with the tail-to-tail spectrum extending over 1.5 $\mu$m and delivering 40 $\mu$J pulses that are…