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When a laser pulse excites a ferromagnet, its spin undergoes a dramatic change. The initial demagnetization process is very fast. Experimentally, it is found that the demagnetization time is related to the spin moment in the sample. In this…

Materials Science · Physics 2016-11-11 G. P. Zhang , M. S. Si , Thomas F. George

Laser induced modulation of the magnetization dynamics occurring over various time-scales have been unified here for a Ni80Fe20 thin film excited by amplified femtosecond laser pulses. The weak correlation between demagnetization time and…

Mesoscale and Nanoscale Physics · Physics 2018-12-21 Sucheta Mondal , Anjan Barman

Excitation of a metallic ferromagnet such as Ni with an intensive femtosecond laser pulse causes an ultrafast demagnetization within approximately 300 fs. It was proposed that the ultrafast demagnetization measured in femtosecond…

Materials Science · Physics 2016-09-27 Ritwik Mondal , Marco Berritta , Karel Carva , Peter M. Oppeneer

We compare femtosecond pump-probe experiments in Ni and micromagnetic modelling based on the Landau-Lifshitz-Bloch equation coupled to a two-temperature model, revealing a predominant thermal ultrafast demagnetization mechanism. We show…

Materials Science · Physics 2009-04-29 U. Atxitia , O. Chubykalo-Fesenko , J. Walowski , A. Mann , M. Munzenberg

Femtosecond laser excitation of materials that exhibit magnetic spin textures promises advanced magnetic control via the generation of ultrafast and non-equilibrium spin dynamics. We explore such possibilities in ferrimagnetic [Fe(0.35…

Irradiating solids with ultrashort laser pulses is known to initiate femtosecond timescale magnetization dynamics. However, sub-femtosecond spin dynamics have not yet been observed or predicted. Here, we explore ultrafast light-driven spin…

Mesoscale and Nanoscale Physics · Physics 2023-03-28 Ofer Neufeld , Nicolas Tancogne-Dejean , Umberto De Giovannini , Hannes Hübener , Angel Rubio

Slow magnetic relaxation and two level fluctuations measurements under high current injection is performed in single-contacted ferromagnetic nanostructures. The magnetic configurations of the samples are described by two metastable states…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 J. -E. Wegrowe

Laser-induced femtosecond demagnetization, femtomagnetism, offers a potential route to develop faster magnetic storage devices. It is generally believed that the traditional spin-wave theory, which is developed for thermally driven slow…

Materials Science · Physics 2019-12-05 G. P. Zhang , M. Murakami , Y. H. Bai , Thomas F. George , X. S. Wu

Most laser-induced femtosecond magnetism investigations are done in magnetic thin films. Nanostructured magnetic dots, with their reduced dimensionality, present new opportunities for spin manipulation. Here we predict that if a magnetic…

Materials Science · Physics 2015-05-27 G. P. Zhang , M. S. Si , T. F. George

We demonstrate the coherent optical control of magnetization precession in a thin Ni film by a second excitation pulse which amplifies or attenuates the precession induced by a first pulse depending on the fluences of the pump-pulses and…

Materials Science · Physics 2023-11-09 M. Mattern , F. -C. Weber , D. Engel , C. Korff-Schmising , M. Bargheer

Femtosecond laser light can transfer spin angular momentum between magnetic subspecies that exhibit hybridized valence bands within an alloy or compound, and represents the fastest route for manipulating the magnetization of a material. To…

Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…

Materials Science · Physics 2010-07-06 Adrian Glaubitz

A quantitative understanding of the processes that trigger light-induced demagnetization on ultrashort timescales is crucial for achieving an ultrafast, radiation-controlled magnetic response in materials. This milestone is essential for…

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

Materials Science · Physics 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

We report on {\it ab-initio} simulations of the quantum dynamics of electronic charge and spin when subjected to intense laser pulses. By performing separate calculations for a Ni thin film and bulk Ni, we conclude that surface effects have…

Materials Science · Physics 2017-05-24 K. Krieger , P. Elliott , T. Müller , N. Singh , J. K. Dewhurst , E. K. U. Gross , S. Sharma

The ability to control the magnetic state provides a powerful means to tune the underlying band topology, enabling transitions between distinct electronic phases and the emergence of novel quantum phenomena. In this work, we address the…

We report on the manipulation of magnetization by femtosecond laser pulses in a periodic array of cylindrical nickel nanoparticles. By performing experiments at different wavelength, we show that the excitation of collective surface plasmon…

Laser-induced ultrafast demagnetization has puzzled researchers around the world for over two decades. Intrinsic complexity in electronic, magnetic, and phononic subsystems is difficult to understand microscopically. So far it is not…

Materials Science · Physics 2021-05-19 G. P. Zhang , Y. H. Bai , Thomas F. George

Laser-induced femtosecond magnetism or femtomagnetism simultaneously relies on two distinctive contributions: (a) the optical dipole interaction (ODI) between a laser field and a magnetic system and (b) the spin expectation value change…

Materials Science · Physics 2012-02-21 M. S. Si , G. P. Zhang

Using density matrix equations of motion, we predict a femtosecond collective spin tilt triggered by nonlinear, near--ultraviolet ($\sim$3eV), coherent photoexcitation of (Ga,Mn)As ferromagnetic semiconductors with linearly polarized light.…

Strongly Correlated Electrons · Physics 2009-08-06 M. D. Kapetanakis , I. E. Perakis , K. J. Wickey , C. Piermarocchi , J. Wang
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