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Related papers: Modelling excitonic-energy transfer in light-harve…

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Two distinct approaches, the Frenkel-Dirac time-dependent variation and the Haken-Strobl model, are adopted to study energy transfer dynamics in single-ring and double-ring light-harvesting systems in purple bacteria. It is found that…

Chemical Physics · Physics 2015-06-05 Jun Ye , Kewei Sun , Yang Zhao , Yunjin Yu , Chee Kong Lee , Jianshu Cao

We investigate the role of quantum coherence in modulating the energy transfer rate between two independent energy donors and a single acceptor participating in an excitonic energy transfer process. The energy transfer rate depends…

Chemical Physics · Physics 2015-07-13 Sreenath K. Manikandan , Anil Shaji

Strong light--matter interactions forming hybrid quasiparticles termed polaritons can specifically tailor molecular photophysics. In this spirit, enhancing energy transport has recently been of special interest. Exciton--exciton…

Chemical Physics · Physics 2026-01-14 Luca Nils Philipp , Julian Lüttig , Roland Mitric

Heat transfer and dissipation exists in almost any physical, chemical or biological systems. Cells, as the basic unit of life, undergo continuous heat transfer and dissipation during their metabolism. The heat transfer and dissipation…

Biological Physics · Physics 2019-01-03 Pei Song , He Gao , Miao Zhang , Fan Yang , Shan-Shan Li , Bin Kang , Jing-Juan Xu , Hong-Yuan Chen

Photosynthetic antenna complexes achieve high quantum efficiency through exciton transport in coupled pigment networks. Conventional Frenkel-exciton models treat each chromophore as a structureless site and neglect internal electronic…

Optics · Physics 2026-04-01 Jingyu Liu , Tao-Yuan Du

We recently proposed effective normal modes for excitonically coupled aggregates which exactly transform the energy transfer Hamiltonian into a sum of one-dimensional Hamiltonians along the effective normal modes. Identifying physically…

Chemical Physics · Physics 2022-05-25 Sanjoy Patra , Vivek Tiwari

We consider generation of an electrical pulse by an optical pulse in the ``virtual excitation'' regime. The electronic system, which is any electro-optic material including a quantum well structure biased by a dc electric field, is assumed…

Quantum Physics · Physics 2009-10-31 Akira Shimizu , Masamichi Yamanishi

Assessing the role of interference in natural and artificial quantum dyanamical processes is a crucial task in quantum information theory. To this aim, an appopriate formalism is provided by the decoherent histories framework. While this…

Quantum Physics · Physics 2016-04-13 Michele Allegra , Paolo Giorda , Seth Lloyd

Creation of electron or exciton by external fields in a system with initially statistically independent unrelaxed vibrational modes leads to an initial condition term. The contribution of this term in the time convolution generalized master…

Biological Physics · Physics 2011-12-07 M. Pudlak , K. N. Pichugin , R. G. Nazmitdinov , R. Pincak

We model and study the processes of excitation, absorption, and transfer in various networks. The model consists of a harmonic oscillator representing a single-mode radiation field, a qubit acting as an antenna, a network through which the…

Quantum Physics · Physics 2024-11-28 E. Ballarin , D. A. Chisholm , A. Smirne , M. Paternostro , F. Anselmi , S. Donadi

Recent observations of beating signals in the excitation energy transfer dynamics of photosynthetic complexes have been interpreted as evidence for sustained coherences that are sufficiently long-lived for energy transport and coherence to…

Quantum Physics · Physics 2013-03-05 A. W. Chin , J. Prior , R. Rosenbach , F. Caycedo-Soler , S. F. Huelga , M. B. Plenio

We provide an intuitive platform for engineering exciton transfer dynamics. We show that careful consideration of the spectral density, which describes the system-bath interaction, leads to opportunities to engineer the transfer of an…

Quantum Physics · Physics 2015-05-18 Alejandro Perdomo , Leslie Vogt , Ali Najmaie , Alán Aspuru-Guzik

A photonic circuit is generally described as a structure in which light propagates by unitary exchange and transfers reversibly between channels. In contrast, the term `diffusive' is more akin to a chaotic propagation in scattering media,…

We investigate the quantum dynamics of energy and charge transfer in a wheel-shaped artificial photosynthetic antenna-reaction center complex.This complex consists of six light-harvesting chromophores and an electron-acceptor fullerene. To…

Biological Physics · Physics 2015-05-28 Pulak Kumar Ghosh , Anatoly Yu. Smirnov , Franco Nori

Excited-state charge-transfer complexes (exciplexes) have been actively exploited in organic optoelectronic devices to improve performance; however, diffusion of exciplexes has not been actively studied despite its influence on performance…

Materials Science · Physics 2019-06-25 Hwang-Beom Kim , Jang-Joo Kim

Non-Markovian and non-equilibrium phonon effects are believed to be key ingredients in the energy transfer in photosynthetic complexes, especially in complexes which exhibit a regime of intermediate exciton-phonon coupling. In this work, we…

Quantum Physics · Physics 2011-07-08 Patrick Rebentrost , Alán Aspuru-Guzik

The interplay of migration, recombination, and dissociation of excitons in disordered media is studied theoretically in the low temperature regime. An exact expression for the photoluminescence spectrum is obtained. The theory is applied to…

Condensed Matter · Physics 2009-10-28 M. C. J. M. Vissenberg , M. J. M. de Jong

We investigate the role of quantum coherence in the efficiency of excitation transfer in a ring-hub arrangement of interacting two-level systems, mimicking a light-harvesting antenna connected to a reaction center as it is found in natural…

Quantum Physics · Physics 2009-11-13 Alexandra Olaya-Castro , Chiu Fan Lee , Francesca Fassioli Olsen , Neil F. Johnson

Underlying physical principles for the high efficiency of excitation energy transfer in light-harvesting complexes are not fully understood. Notably, the degree of robustness of these systems for transporting energy is not known considering…

Quantum Physics · Physics 2015-03-19 Masoud Mohseni , Alireza Shabani , Seth Lloyd , Herschel Rabitz

We analyze efficiency of excitation energy transfer in photosynthetic complexes in transient and stationary setting. In the transient setting the absorption process is modeled as an individual event resulting in a subsequent relaxation…

Chemical Physics · Physics 2013-06-10 Simon Jesenko , Marko Znidaric