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The optical spectra of CdSe nanocrystals up to 55 A in diameter are analyzed in a wide range of energies from the fine structure of the low-energy excitations to the so-called high-energy transitions. We apply a symmetry-based method in two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Perez-Conde , A. K. Bhattacharjee

Spatiotemporal dynamics of excitons in isolated semiconducting single-walled carbon nanotubes are studied using transient absorption microscopy. Differential reflection and transmission of an 810-nm probe pulse after excitation by a 750-nm…

Mesoscale and Nanoscale Physics · Physics 2013-01-08 Brian A. Ruzicka , Rui Wang , Jessica Lohrman , Shenqiang Ren , Hui Zhao

We show how to calculate the linear and nonlinear optical functions of CdSe nanoplatelets, taking into account the effect of a dielectric confinement on excitonic states. We consider both stationary and non-stationary excitation regime. We…

Mesoscale and Nanoscale Physics · Physics 2025-11-06 Gerard Czajkowski

Spin relaxation in undoped quasi-spherical CdS quantum dots at zero magnetic fields is investigated using time- and polarization-resolved transient absorption measurements. Unlike in previous studies of these systems, the measured signals…

Mesoscale and Nanoscale Physics · Physics 2007-09-27 P. Nahálková , D. Sprinzl , P. Malý , P. Němec , V. N. Gladilin , J. T. Devreese

We experimentally investigated for the first time the lowest four band structure of Cd Se nanoplatelets at the r point of Brillouin zone [heavy-hole (hh), light-hole (lh) and two spin-orbital bands] and its modification due to the changing…

Luminescent colloidal CdSe nanorings are a new type of semiconductor structure that have attracted interest due to the potential for unique physics arising from their non-trivial toroidal shape. However, the exciton properties and dynamics…

Two-dimensional electron-hole gases in colloidal semiconductors have a wide variety of applications. Therefore, a proper physical understanding of these materials is of great importance. In this paper we present a detailed theoretical…

Mesoscale and Nanoscale Physics · Physics 2019-12-18 F. García Flórez , Aditya Kulkarni , Laurens D. A. Siebbeles , H. T. C. Stoof

Using an approximate time-dependent density functional theory method, we calculate the absorption and luminescence spectra for hydrogen passivated silicon nanoscale structures with large aspect ratio. The effect of electron confinement in…

Materials Science · Physics 2009-09-27 Y. Wang , R. Q. Zhang , Th. Frauenheim , T. A. Niehaus

The bright exciton emission of semiconducting carbon nanotubes is appealing for optoelectronic and quantum photonic devices as well as fundamental studies of light-matter interaction in one-dimensional nanostructures. The photophysics of…

Mesoscale and Nanoscale Physics · Physics 2017-05-09 Ibrahim Sarpkaya , Zhengyi Zhang , William Walden-Newman , Xuesi Wang , James Hone , Chee Wei Wong , Stefan Strauf

Fully-inorganic cesium lead halide perovskite nanocrystals (NCs) have shown to exhibit outstanding optical properties such as wide spectral tunability, high quantum yield, high oscillator strength as well as blinking-free single photon…

We study spin dynamics of excitons confined in self-assembled CdSe quantum dots by means of optical orientation in magnetic field. At zero field the exciton emission from QDs populated via LO phonon-assisted absorption shows a circular…

Materials Science · Physics 2015-06-24 S. Mackowski , T. Gurung , H. E. Jackson , L. M. Smith , J. K. Furdyna , M. Dobrowolska

We investigate strongly asymmetric self-assembled nanostructures with one of dimensions reaching hundreds of nanometers. Close to the nanowire-like type of confinement, such objects are sometimes assigned as one-dimensional in nature. Here,…

Mesoscale and Nanoscale Physics · Physics 2021-06-29 M. Gawełczyk , P. Wyborski , P. Podemski , J. P. Reithmaier , S. Höfling , G. Sęk

We investigated the nonlinear optical properties of CdSe/CdS nanoplatelets in the vicinity of heavy hole and light hole exciton resonances. The two color pump-probe technique was applied. The first intense pulse created non-equilibrium…

We measured the intrinsic ground-state exciton dephasing and population dynamics in colloidal quasi two-dimensional (2D) CdSe nanoplatelets at low temperature (5-50K) using transient resonant four-wave mixing in heterodyne detection. Our…

Mesoscale and Nanoscale Physics · Physics 2015-05-05 Ali Naeem , Francesco Masia , Sotirios Christodoulou , Iwan Moreels , Paola Borri , Wolfgang Langbein

We have theoretically shown that optical properties of semiconductor nanorods are controlled by 1D excitons. The theory, which takes into account anisotropy of spacial and dielectric confinement, describes size dependence of interband…

Materials Science · Physics 2007-05-23 A. Shabaev , Al. L. Efros

Femtosecond (fs)-resolved photoemission electron micrographs of single and few-layer MoSe$_2$ track exciton dynamics in this model 2D quantum material system with joint nanometer (nm)-fs resolution. We illustrate the latter using two-photon…

Chemical Physics · Physics 2021-09-27 Paul M. Sass , Patrick Z. El-Khoury

Coupling to phonon modes is a primary mechanism of excitonic dephasing and energy loss in semiconductors. However, low-energy phonons in colloidal quantum dots and their coupling to excitons are poorly understood, since their experimental…

Mesoscale and Nanoscale Physics · Physics 2019-10-22 Albert Liu , Diogo B. Almeida , Wan-Ki Bae , Lazaro A. Padilha , Steven T. Cundiff

Heterostructures of layered transition metal dichalcogenides (TMDs) host long-lived, tunable excitons, making them intriguing candidates for material-based quantum information applications. Light absorption in these systems induces a…

Materials Science · Physics 2023-08-25 Tomer Amit , Sivan Refaely-Abramson

We study the band-edge exciton fine structure and in particular its bright-dark splitting in colloidal semiconductor nanocrystals by four different optical methods based on fluorescence line narrowing and time-resolved measurements at…

Colloidal semiconductor nanoplatelets exhibit quantum size effects due to their thickness of only few monolayers, together with strong optical band-edge transitions facilitated by large lateral extensions. In this article we demonstrate…

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