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Calcium monofluoride (CaF) molecules are loaded into an optical dipole trap (ODT) and subsequently laser cooled within the trap. Starting with magneto-optical trapping, we sub-Doppler cool CaF and then load $150(30)$ CaF molecules into an…

Laser slowing of CaF molecules down to the capture velocity of a magneto-optical trap (MOT) for molecules is achieved. Starting from a two-stage buffer gas beam source, we apply frequency-broadened "white-light" slowing and observe…

We report the experimental realization of a conveyor-belt magneto-optical trap for calcium monofluoride (CaF) molecules. The obtained highly-compressed cloud has a mean radius of 64(5) $\mu$m and a peak number density of $3.6(5) \times…

We report non-destructive imaging of optically trapped calcium monofluoride (CaF) molecules using in-situ $\Lambda$-enhanced gray molasses cooling. $200$ times more fluorescence is obtained compared to destructive on-resonance imaging, and…

We demonstrate with a RF-MOT the one dimensional, transverse magneto-optical compression of a cold beam of calcium monofluoride (CaF). By continually alternating the magnetic field direction and laser polarizations of the magneto-optical…

Magneto-optical trapping forces for molecules are far weaker than for alkali atoms because the photon scattering rate is reduced when there are multiple ground states, and because of optical pumping into dark states. The force is further…

Atomic Physics · Physics 2021-12-14 M. R. Tarbutt , T. C. Steimle

We present the properties of a magneto-optical trap (MOT) of CaF molecules. We study the process of loading the MOT from a decelerated buffer-gas-cooled beam, and how best to slow this molecular beam in order to capture the most molecules.…

Atomic Physics · Physics 2017-12-06 H. J. Williams , S. Truppe , M. Hambach , L. Caldwell , N. J. Fitch , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times…

Molecular magneto-optical traps (MOTs) typically capture orders of magnitude fewer particles than their atomic counterparts due in part to their significantly lower capture velocities. Here, we employ a Stochastic Schr\"odinger Equation…

Magneto-optical trapping of molecules has thus far been restricted to molecules with $^2\Sigma$ electronic ground states. These species are chemically reactive and only support a simple laser cooling scheme from their first excited…

We describe experiments demonstrating efficient transfer of molecules from a magneto-optical trap (MOT) into a conservative magnetic quadrupole trap. Our scheme begins with a blue-detuned optical molasses to cool SrF molecules to $\sim\!50$…

Atomic Physics · Physics 2018-07-11 D. J. McCarron , M. H. Steinecker , Y. Zhu , D. DeMille

As a heavy molecule, barium monofluoride (BaF) presents itself as a promising candidate for measuring permanent electric dipole moment. The precision of such measurements can be significantly enhanced by utilizing a cold molecular sample.…

Atomic Physics · Physics 2024-10-29 Zixuan Zeng , Shuhua Deng , Shoukang Yang , Bo Yan

Laser cooling and trapping are central to modern atomic physics. The workhorse technique in cold-atom physics is the magneto-optical trap (MOT), which combines laser cooling with a restoring force from radiation pressure. For a variety of…

Atomic Physics · Physics 2014-10-20 J. F. Barry , D. J. McCarron , E. B. Norrgard , M. H. Steinecker , D. DeMille

We report optical trapping of a polyatomic molecule, calcium monohydroxide (CaOH). CaOH molecules from a magneto-optical trap are sub-Doppler laser cooled to $20(3)~\mu\text{K}$ in free space and loaded into an optical dipole trap. We…

First laser cooling and trapping of the heavy alkaline earth element barium has been achieved based on the strong 6s$^2$ $^1$S$_0$ - 6s6p $^1$P$_1$ transition for the main cooling. Due to the large branching into metastable D-states several…

Atomic Physics · Physics 2015-05-13 S. De , U. Dammalapati , K. Jungmann , L. Willmann

Metastable calcium atoms, produced in a magneto-optic trap (MOT) operating within the singlet system, are continuously loaded into a magnetic trap formed by the magnetic quadrupole field of the MOT. At MOT temperatures of 3 mK and 240 ms…

Atomic Physics · Physics 2009-11-07 Dirk P. Hansen , Janis R. Mohr , Andreas Hemmerich

We demonstrate a scheme for magneto-optically trapping strontium monofluoride (SrF) molecules at temperatures one order of magnitude lower and phase space densities three orders of magnitude higher than obtained previously with laser-cooled…

Atomic Physics · Physics 2016-02-17 E. B. Norrgard , D. J. McCarron , M. H. Steinecker , M. R. Tarbutt , D. DeMille

Optically trapped laser-cooled polar molecules hold promise for new science and technology in quantum information and quantum simulation. Large numerical aperture optical access and long trap lifetimes are needed for many studies, but these…

We present experimental results from a new scheme for magneto-optically trapping strontium monofluoride (SrF) molecules, which provides increased confinement compared to our original work. The improved trap employs a new approach to…

Atomic Physics · Physics 2015-06-23 D. J. McCarron , E. B. Norrgard , M. H. Steinecker , D. DeMille

We have realized a scheme for continuous loading of a magnetic trap (MT). ^{52}Cr atoms are continuously captured and cooled in a magneto-optical trap (MOT). Optical pumping to a metastable state decouples atoms from the cooling light. Due…

Quantum Physics · Physics 2009-11-06 J. Stuhler , P. O. Schmidt , S. Hensler , J. Werner , J. Mlynek , T. Pfau
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