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A theoretical optimization method of high-harmonic-generation (HHG) is developed in the framework of optimal-control-theory (OCT). The target of optimization is the emission radiation of a particular frequency. The OCT formulation includes…

Quantum Physics · Physics 2020-02-19 Ido Schaefer , Ronnie Kosloff

Optical modulation of high-harmonics generation in solids enables the detection of material properties such as the band structure and promising new applications such as super-resolution imaging in semiconductors. Various recent studies have…

We show that the divergence of extreme ultraviolet pulses from high harmonic generation, which is directly linked to the shape and size of the refocused beam, can be controlled by the relative delay between the fundamental and its intense…

We study high-order harmonic generation (HHG) from aligned molecules in strong elliptically polarized laser fields numerically and analytically. Our simulations show that the spectra and polarization of HHG depend strongly on the molecular…

Atomic Physics · Physics 2021-05-19 F. J. Sun , C. Chen , W. Y. Li , X. Liu , W. Li , Y. J. Chen

Recent years have witnessed significant developments in the study of nonlinear properties of various optical materials at the nanoscale. However, in most cases experimental results on harmonic generation from nanostructured materials are…

In the realm of open quantum systems, steady states and high-harmonic generation (HHG) existing far from equilibrium have become core pillars of ultrafast science. Most solid-state research explores charge HHG with limited investigations…

Strongly Correlated Electrons · Physics 2024-08-20 Negin Moharrami Allafi , Michael H. Kolodrubetz , Marin Bukov , Vadim Oganesyan , Mohsen Yarmohammadi

A theory of ultra-fast pump-probe experiments proposed by us earlier [F.H.M. Faisal et al., Phys. Rev. Lett. 98, 143001 (2007) and F.H.M. Faisal and A. Abdurrouf, Phys. Rev. Lett. 100, 123005 (2008)] is developed here fully and applied to…

Atomic and Molecular Clusters · Physics 2009-11-13 A. Abdurrouf , F. H. M. Faisal

We study inhibition of absorption, transparency, energy and momentum transport of the inhomogeneous component of harmonic pulses in dielectrics and semiconductors, at visible and UV wavelengths, focusing on materials like GaP. In these…

State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…

Circularly polarized extreme ultraviolet (XUV) radiation is highly interesting for investigation of chirality-sensitive light-matter interactions. Recent breakthroughs have enabled generation of such light sources via high harmonic…

Optics · Physics 2019-02-19 Zi-Yu Chen , Rui Qin

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

High harmonic generation (HHG) in crystals has revealed a wealth of perspectives such as all-optical mapping of the electronic band structure, ultrafast quantum information and the creation of novel all-solid-state attosecond sources.…

The landscape of ultrafast structured light pulses has recently evolved driven by the capability of high-order harmonic generation (HHG) to up-convert orbital angular momentum (OAM) from the infrared to the extreme-ultraviolet (EUV)…

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

Thermotropic liquid crystals are versatile optical materials that exhibit a state of matter intermediate between liquids and solids. Their properties can change significantly with temperature, pressure, or other external factors, leading to…

Solids in an intense laser field show high-harmonic generation (HHG), which can provide information on carrier dynamics and band structures in weakly correlated systems. In strongly correlated systems, a laser field can induce a transition…

Strongly Correlated Electrons · Physics 2025-08-04 Ryohei Ikeda , Yuta Murakami , Daiki Sakai , Tatsuya Miyamoto , Toshimitsu Ito , Hiroshi Okamoto

Vector beam, with a spatial nonuniform polarization distribution, is important for many applications due to its unique field characteristics and novel effects when interacting with matter. Here through three-dimensional particle-in-cell…

Optics · Physics 2021-03-22 Zi-Yu Chen , Ronghao Hu

High-harmonic generation (HHG) in two-dimensional materials offers a compelling route toward compact extreme ultraviolet sources and probing electron dynamics on the attosecond scale. However, achieving precise control over the emission and…

Computational Physics · Physics 2026-05-19 Zhenjiang Zhao , Zhihua Zheng , Zhiyi Xu , Xing Ran , Xiaolong Yao , Fangping Ouyang

In this work, we demonstrate experimentally the efficient generation and tunability of energetic highly-elliptical high-harmonics in Ar gas, driven by intense two-color counter rotating laser electric fields. A bi-chromatic beam tailored by…

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated…

Atomic Physics · Physics 2008-11-14 Y. J. Chen , J. Liu , Bambi Hu