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High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…

Structured light carrying orbital angular momentum enables new regimes of nonlinear light-matter interaction. Here we develop a molecular quantum electrodynamics description of third-harmonic generation (THG) driven by focused…

Optics · Physics 2026-03-30 Szymon Kurkowski , Kayn A Forbes

We experimentally study the behavior of orbital angular momentum (OAM) of light in a noncollinear second harmonic generation (SHG) process. The experiment is performed by using a type I BBO crystal under phase matching conditions with…

In the rapidly evolving field of structured light, the self-torque has been recently defined as an intrinsic property of light beams carrying time-dependent orbital angular momentum. In particular, extreme-ultraviolet (EUV) beams with…

We investigate the use of light beams carrying orbital angular momentum (OAM) in the context of high harmonic generation (HHG) within semiconductor crystals. Our contribution deals with the transfer and conservation of OAM in the…

Optics · Physics 2024-10-01 C. Granados , B. Kumar Das , M. F. Ciappina

In previous studies of spin-to-orbital angular momentum (AM) conversion in laser high harmonic generation (HHG) using a plasma target, one unit of spin AM is always converted into precisely one unit of OAM [1, 2]. Here we show, through…

Plasma Physics · Physics 2023-05-22 R. M. G. M. Trines , H. Schmitz , M. King , P. McKenna , R. Bingham

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

Optics · Physics 2020-05-20 Jonas Wätzel , Jamal Berakdar

High-harmonic generation (HHG) is a nonlinear process in which a strong driving field interacts with a material, resulting in the frequency up-conversion of the driver into its high-order harmonics. This process is highly sensitive to the…

Quantum Physics · Physics 2025-07-04 J. Rivera-Dean , P. Stammer , M. F. Ciappina , M. Lewenstein

High-harmonic generation (HHG), an extreme nonlinear effect, introduces an unprecedented paradigm to detect emergent quantum phases and electron dynamics inconceivable in the framework of linear and low-order nonlinear processes. As an…

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…

We identify and explore a high orbital angular momentum (OAM) harmonics generation and amplification mechanism that manipulates the OAM independently of any other laser property, by preserving the initial laser wavelength, through…

Toroidal vortex is a kind of novel and exotic structured light with potential applications in photonic topology and quantum information. Here, we present the study on high harmonic generation (HHG) from the interaction of the intense…

Optics · Physics 2024-10-10 Zijian Lyu , Yiqi Fang , Yunquan Liu

Nonlinear photon upconversion processes driven by diverse forms of structured light are receiving increasing attention. In harmonic and high-order harmonic generation (HG and HHG) with Laguerre-Gauss (LG) beams, linear scaling the driver…

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

Materials Science · Physics 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

We study the high harmonic generation with vortex beams beyond the dipole approximation. To do so we employ the full minimal coupling approach to account for multipolar coupling without truncation and describe the full spatio-temporal…

Atomic Physics · Physics 2026-01-21 Esra Ilke Albar , Valeriia P. Kosheleva , Heiko Appel , Angel Rubio , Franco P. Bonafé

High-order harmonic generation (HHG) is investigated theoretically in the over-the-barrier ionization (OBI) regime revealing the strong signature of interference between two separately ionized and separately propagating free wave packets of…

Photons can undergo spin-orbit coupling, by which the polarization (spin) and spatial profile (orbit) of the electromagnetic field interact and mix. Strong photonic spin-orbit coupling may reportedly arise from light propagation confined in…

Optics · Physics 2023-08-08 Chang Kyun Ha , Eun Mi Kim , Kyoung Jun Moon , Myeong Soo Kang