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Conventional absorption spectroscopy relies on coherent laser sources, and in turn suffers from the inherent limitation of shot noise, especially in estimating weak absorption. Here we propose a measurement strategy with correlated photons…

Quantum Physics · Physics 2025-04-17 Zhucheng Zhang , Xue Zhang , Jing Liu , Hui Dong

Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…

Chemical Physics · Physics 2026-04-21 Yuta Fujihashi , Ozora Iso , Ryosuke Shimizu , Akihito Ishizaki

Sympathetic cooling of trapped ions has been established as a powerful technique for manipulation of non-laser-coolable ions (Raizen1992,Waki1992,Bowe1999,Barrett2003). For molecular ions, it promises vastly enhanced spectroscopic…

Quantum Physics · Physics 2018-06-06 Soroosh Alighanbari , Michael Georg Hansen , Vladimir Korobov , Stephan Schiller

Precision spectroscopy of atomic hydrogen is an important way to test bound-state quantum electrodynamics (QED), one of the building blocks of the Standard Model. In its simplest form, such a test consists of the comparison of a measured…

Atomic Physics · Physics 2025-12-24 Lothar Maisenbacher

Laser spectroscopy of cold and trapped molecular ions is a powerful tool for fundamental physics, including the determination of fundamental constants, the laboratory test for their possible variation, and the search for a possible electric…

Atomic Physics · Physics 2016-02-26 Fabian Wolf , Yong Wan , Jan C. Heip , Florian Gebert , Chunyan Shi , Piet O. Schmidt

Macroscopic quantum phenomena, such as observed in superfluids and superconductors, have led to promising technological advancements and some of the most important tests of fundamental physics. At present, quantum detection of light is…

We describe a high-resolution spectroscopy method, in which the detection of single excitation events is enhanced by a complete loss of coherence of a superposition of two ground states. Thereby, transitions of a single isolated atom nearly…

Atomic Physics · Physics 2014-03-25 Govinda Clos , Martin Enderlein , Ulrich Warring , Dietrich Leibfried , Tobias Schaetz

The resolution limits of classical spectroscopy can be surpassed by quantum-inspired methods leveraging the information contained in the phase of the complex electromagnetic field. Their counterpart in spatial imaging has been widely…

Optics · Physics 2024-09-02 Michał Lipka , Michał Parniak

Photoabsorption of atomic oxygen in the energy region below the $\rm 1s^{-1}$ threshold in x-ray spectroscopy from {\it Chandra} and {\it XMM-Newton} is observed in a variety of x-ray binary spectra. Photoabsorption cross sections…

High Energy Astrophysical Phenomena · Physics 2015-06-16 B. M. McLaughlin , C. P. Ballance , K. P. Bowen , D. J. Gardenghi , W. C. Stolte

Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires…

Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…

Quantum Physics · Physics 2022-11-23 Yuanyuan Chen , Roberto de J. León-Montiel , Lixiang Chen

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

Realistic attosecond wave packets have complex profiles that, in dispersive conditions, rapidly broaden or split into multiple components. Such behaviors are encoded in sharp features of the wave packet spectral phase. Here, we exploit the…

Entangled photons have the remarkable ability to be more sensitive to signal and less sensitive to noise than classical light. Joint photons can sample an object collectively, resulting in faster phase accumulation and higher spatial…

Optics · Physics 2015-09-04 Chien-Hung Lu , Matthew Reichert , Xiaohang Sun , Jason W. Fleischer

Quasar spectra reveal a rich array of important astrophysical information about galaxies which intersect the quasar line of sight. They also enable tests of the variability of fundamental constants over cosmological time and…

Cosmology and Nongalactic Astrophysics · Physics 2015-06-17 Michael T. Murphy , Julian C. Berengut

We propose a scheme for quantum logic spectroscopy of an electron or positron in a Penning trap. An electron or positron in a spectroscopy trap is coupled to a remote logic electron or positron via a wire to achieve motional entanglement.…

Quantum Physics · Physics 2025-06-05 Xing Fan , Atsushi Noguchi , Kento Taniguchi

Direct frequency comb spectroscopy of trapped ions is demonstated for the first time. It is shown that the 4s^2S_(1/2)-4p^2P_(3/2) transition in calcium ions can be excited directly with a frequency comb laser that is upconverted to 393 nm.…

Atomic Physics · Physics 2009-06-08 A. L. Wolf , S. A. van den Berg , W. Ubachs , K. S. E. Eikema

Ultrasensitive detection of the frequency, phase, and amplitude of radio frequency (RF) electric fields is central to a variety of important applications, including radio communication, cosmology, dark matter searches, and high-fidelity…

Atomic Physics · Physics 2026-04-29 Hao Wu , Grant Mitts , Clayton Ho , Joshua Rabinowitz , Eric R. Hudson

Multiphoton absorption is of vital importance in many spectroscopic, microscopic or lithographic applications. However, given that it is an inherently weak process, the detection of multiphoton absorption signals typically requires large…

Quantum Physics · Physics 2023-05-31 Shahram Panahiyan , Carlos Sánchez Muñoz , Maria V. Chekhova , Frank Schlawin

Precise spectroscopy of oscillating fields plays significant roles in many fields. Here, we propose an experimentally feasible scheme to measure the frequency of a fast-oscillating field using a single-qubit sensor. By invoking a stable…

Quantum Physics · Physics 2021-01-21 Yaoming Chu , Pengcheng Yang , Musang Gong , Min Yu , Baiyi Yu , Martin B. Plenio , Alex Retzker , Jianming Cai