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For several atomistic models of glass formers, at conditions below their glassy dynamics onset temperatures, ${T_\mathrm{o}}$, we use importance sampling of trajectory space to study the structure, statistics and dynamics of excitations…

Statistical Mechanics · Physics 2014-05-08 Aaron S. Keys , Lester O. Hedges , Juan P. Garrahan , Sharon C. Glotzer , David Chandler

We investigate the stress relaxation behavior on the application of step strains to aging aqueous suspensions of the synthetic clay Laponite. The stress exhibits a two-step decay, from which the slow relaxation modes are extracted as…

Soft Condensed Matter · Physics 2015-03-13 Ranjini Bandyopadhyay , P. Harsha Mohan , Yogesh M. Joshi

We study a two-dimensional model for interacting colloidal particles which displays spontaneous clustering. Within this model we investigate the competition between the pinning to a periodic corrugation potential, and a sideways constant…

Soft Condensed Matter · Physics 2018-05-23 Mirko Rossini , Lorenzo Consonni , Andrea Stenco , Luciano Reatto , Nicola Manini

Diverse processes -- e.g., environmental pollution, groundwater remediation, oil recovery, filtration, and drug delivery -- involve the transport of colloidal particles in porous media. Using confocal microscopy, we directly visualize this…

Soft Condensed Matter · Physics 2021-03-23 Navid Bizmark , Joanna Schneider , Rodney D. Priestley , Sujit S. Datta

We study the conditions under which and how an imposed cluster of fixed colloidal particles at prescribed positions triggers crystal nucleation from a metastable colloidal fluid. Dynamical density functional theory of freezing and Brownian…

Soft Condensed Matter · Physics 2009-11-13 Sven van Teeffelen , Christos N. Likos , Hartmut Löwen

The properties of crystals consisting of several components can be widely tuned. Often solid solutions are produced, where substitutional or interstitional disorder determines the crystal thermodynamic and mechanical properties. The…

Soft Condensed Matter · Physics 2019-10-30 Tadeus Ras , Michael Szafarczyk , Matthias Fuchs

We investigate the spatial correlations of microscopic stresses in soft particulate gels, using 2D and 3D numerical simulations. We use a recently developed theoretical framework predicting the analytical form of stress-stress correlations…

Soft Condensed Matter · Physics 2023-03-29 H. A. Vinutha , Fabiola Diaz Ruiz , Xiaoming Mao , Bulbul Chakraborty , Emanuela Del Gado

Fatigue refers to the changes in material properties caused by repeatedly applied loads. It has been widely studied for, e.g., construction materials, but much less has been done on soft materials. Here, we characterize the fatigue dynamics…

Soft Condensed Matter · Physics 2016-08-30 Thomas Gibaud , Christophe Perge , Stefan B. Lindstrom , Nicolas Taberlet , Sebastien Manneville

We examine the structural relaxation of glassy materials at finite temperatures, considering the effect of activated rearrangements and long-range elastic interactions. Our three-dimensional mesoscopic relaxation model shows how the…

Soft Condensed Matter · Physics 2023-12-20 Gieberth Rodriguez-Lopez , Kirsten Martens , Ezequiel E. Ferrero

The consolidation of suspended particulate matter under external forces such as pressure or gravity is of widespread interest. In this work, we derive a constitutive relation to describe the deformation of a {\it two-dimensional} strongly…

Soft Condensed Matter · Physics 2014-02-26 Saikat Roy , Mahesh S Tirumkudulu

Dynamical heterogeneities in a colloidal fluid close to gelation are studied by means of computer simulations. A clear distinction between some fast particles and the rest, slow ones, is observed, yielding a picture of the gel composed by…

Soft Condensed Matter · Physics 2009-11-10 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

Upon cooling, glass-forming liquids experience a two-step relaxation associated to the cage rattling and the escape from the cage, and the following decoupling between the \b{eta}- and the {\alpha}-relaxations. The found decoupling…

Disordered Systems and Neural Networks · Physics 2017-06-07 P. Luo , P. Wen , H. Y. Bai , B. Ruta , W. H. Wang

The process of structural relaxation in disordered solids subjected to repeated tension-compression loading is studied using molecular dynamics simulations. The binary glass is prepared by rapid cooling well below the glass transition…

Soft Condensed Matter · Physics 2020-05-04 Pritam Kumar Jana , Nikolai V. Priezjev

Soft colloids allow to explore high density states well beyond random close packing. An important open question is whether softness controls the dynamics under these dense conditions. While experimental works reported conflicting results,…

Soft Condensed Matter · Physics 2021-06-08 Nicoletta Gnan , Emanuela Zaccarelli

We propose a new method to characterize the spatial distribution of particles' vibrations in solids with much lower computational costs compared to the usual normal mode analysis. We excite the specific vibrational mode in a two dimensional…

Soft Condensed Matter · Physics 2016-05-24 Elsen Tjhung , Takeshi Kawasaki

Elucidating collective dynamics in crystalline systems is a common scientific question in multiple fields. In this work, by combination of high-precision numerical approach and analytical normal mode analysis, we systematically investigate…

Soft Condensed Matter · Physics 2023-01-24 Zhenwei Yao

The origin of the microscopic motions that lead to stress relaxation in deeply supercooled liquid remains unclear. We show that in such a liquid the stress relaxation is locally anisotropic which can serve as the driving force for the…

Chemical Physics · Physics 2007-05-23 Sarika Bhattacharyya , Biman Bagchi

The dynamics of soft colloids in solutions is characterized by internal collective motion as well as center-of-mass diffusion. Using neutron scattering we demonstrate that the competition between the relaxation processes associated with…

Packing of particles in confined environments is a common problem in multiple fields. Here, based on the two-dimensional Hertzian particle model, we study the packing of deformable spherical particles under compression, and reveal the…

Soft Condensed Matter · Physics 2020-07-01 Zhenwei Yao

In the wake of previous studies on the rattling-and-jumping diffusion in smectic liquid crystal phases of colloidal rods, we analyze here for the first time the heterogeneous dynamics in columnar phases. More specifically, we perform…

Soft Condensed Matter · Physics 2015-05-19 Simone Belli , Alessandro Patti , René van Roij , Marjolein Dijkstra