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For the vast majority of naturally occurring, small, single domain proteins folding is often described as a two-state process that lacks detectable intermediates. This observation has often been rationalized on the basis of a nucleation…

Biomolecules · Quantitative Biology 2007-07-09 R. D. M. Travasso , P. F. N. Faisca , M. M. Telo da Gama

When a droplet is brought in contact with an undercooled surface, it wets the substrate and solidifies at the same time. The interplay between the phase transition effects and the contact-line motion, leading to its arrest, remains poorly…

Classical nucleation theory is used to estimate the free-energy barrier to nucleation of the solid phase of particles interacting via a potential which has a short-ranged attraction. Due to the high interfacial tension between the fluid and…

Soft Condensed Matter · Physics 2009-10-31 Richard P. Sear

Grain growth competition during solidification determines microstructural features, such as dendritic arm spacings, segregation pattern, and grain texture, which have a key impact on the final mechanical properties. During metal additive…

Materials Science · Physics 2023-06-23 Rouhollah Tavakoli , Damien Tourret

We investigate the atomistic mechanism of homogeneous nucleation during solidification in molybdenum employing transition path sampling. The mechanism is characterized by the formation of a pre-structured region of high bond-orientational…

Materials Science · Physics 2020-10-16 Sarath Menon , Grisell Díaz Leines , Ralf Drautz , Jutta Rogal

We study the nucleation and growth of flame fronts in slow combustion. This is modeled by a set of reaction-diffusion equations for the temperature field, coupled to a background of reactants and augmented by a term describing random…

Statistical Mechanics · Physics 2015-06-25 Mikko Karttunen , Nikolas Provatas , Tapio Ala-Nissila , Martin Grant

Bubble nucleation in water induced by boiling, gas supersaturation or cavitation usually originates from pre-existing gas cavities trapped into solid defects. Even though the destabilization of such gas pockets, called nuclei, has been…

Fluid Dynamics · Physics 2020-02-19 Adrien Bussonnière , Qingxia Liu , Peichun Amy Tsai

A simple method to get all main characteristics of nucleation process is proposed. The advantage of this method is an applicability to situations with non-linear behavior in time of effective external source of vapor. It is important…

Statistical Mechanics · Physics 2007-05-23 Victor Kurasov

We revisit the classical problem of nucleated polymerisation and derive a range of exact results describing polymerisation in systems intermediate between the well-known limiting cases of a reaction starting from purely soluble material and…

Biological Physics · Physics 2011-07-08 Samuel I. A. Cohen , Michele Vendruscolo , Christopher M. Dobson , Tuomas P. J. Knowles

The properties of the interface between solid and melt are key to solidification and melting, as the interfacial free energy introduces a kinetic barrier to phase transitions. This makes solidification happen below the melting temperature,…

Statistical Mechanics · Physics 2015-12-02 Bingqing Cheng , Gareth A. Tribello , Michele Ceriotti

The emergent dynamics in phase-separated mixtures of isometric active and passive Brownian particles is studied numerically in two dimensions. A novel steady-state of well-defined traveling fronts is observed, where the interface between…

Soft Condensed Matter · Physics 2024-06-03 Adam Wysocki , Roland G. Winkler , Gerhard Gompper

We predict the structural interaction of crystalline solid-melt interfaces using amplitude equations which are derived from classical density functional theory or phase-field-crystal modeling. The solid ordering decays exponentially on the…

Materials Science · Physics 2015-06-12 Robert Spatschek , Ari Adland , Alain Karma

The dynamics of quasicrystal growth remains an unsolved problem in condensed matter. By means of synchrotron live imaging, facetted growth proceeding by the tangential motion of ledges at the solid-melt interface is clearly evidenced all…

Nonequilibrium thermodynamics formalism is proposed to derive the flux of grainy (bubbles-containing) matter, emerging in a nucleation growth process. Some power and non-power limits, due to the applied potential as well as owing to basic…

Soft Condensed Matter · Physics 2009-11-10 J. M. Rubi , A. Gadomski

Ice nucleation plays a significant role in a large number of natural and technological processes, but it is challenging to investigate experimentally because of the small time (ns) and short length scales (nm) involved. On the other hand,…

Materials Science · Physics 2018-08-01 Philipp Pedevilla , Martin Fitzner , Gabriele C. Sosso , Angelos Michaelides

Dynamical interactions between colliding spiral galaxies strongly affect the state and distribution of their interstellar gas. Observations indicate that interactions funnel gas toward the nuclei, fueling bursts of star formation and…

Astrophysics of Galaxies · Physics 2018-07-04 Kelly Blumenthal , Joshua Barnes

We investigate a system of interacting clusters evolving through mass exchange and supplemented by input of small clusters. Three possibilities depending on the rate of exchange generically occur when input is homogeneous: continuous…

Statistical Mechanics · Physics 2015-06-09 P. L. Krapivsky

Despite its fundamental and technological importance, a microscopic understanding of the crystallization process is still elusive. By computer simulations of the hard-sphere model we reveal the mechanism by which thermal fluctuations drive…

Soft Condensed Matter · Physics 2012-06-29 John Russo , Hajime Tanaka

Motivated by unexpected morphologies of the emerging liquid phase (channels, bulges, droplets) at the edge of thin, melting alkane terraces, we propose a new heterogeneous nucleation pathway. The competition between bulk and interfacial…

Chemical Physics · Physics 2015-06-04 Halim Kusumaatmaja , Reinhard Lipowsky , Chenyu Jin , Radu-Cristian Mutihac , Hans Riegler

Despite its importance in atmospheric science, much remains unknown about the microscopic mechanism of heterogeneous ice nucleation. In this work, we perform hybrid Monte Carlo simulations of the heterogeneous nucleation of ice on a range…

Statistical Mechanics · Physics 2014-08-25 Aleks Reinhardt , Jonathan P. K. Doye
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