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Using a minimal model based on the continuum theory of a 2D hard-core/square-shoulder ensemble, we reinterpret the main features of cluster mesophases formed by colloids with soft concave repulsive interactions. We rederive the lattice…

Soft Condensed Matter · Physics 2011-06-06 P. Ziherl , Randall D. Kamien

Nowadays, there is pressing demand for sustainable energy sources, or clean and 'green' fuel and hydrogen is a perfect candidate. It can be made by dissociating methane with the energy input compensated by metal-hydrogen bond formation.…

Chemical Physics · Physics 2022-06-22 Philip E. Hoggan

We revisit here the lowest vertical excitations of cyanine dyes using quantum Monte Carlo and leverage on recent developments to systematically improve on previous results. In particular, we employ a protocol for the construction of compact…

Chemical Physics · Physics 2021-11-22 Alice Cuzzocrea , Saverio Moroni , Anthony Scemama , Claudia Filippi

Analytical expressions for the binding energy of electrons and positrons in dielectric clusters, analysed in this work, neglect the elastic effects. Therefore, we present the density-functional theory for neutral liquid clusters that…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Valentin V. Pogosov , Walter V. Pogosov , Denis P. Kotlyarov

We introduce a novel many body method which combines two powerful many body techniques, viz., quantum Monte Carlo and coupled cluster theory. Coupled cluster wave functions are introduced as importance functions in a Monte Carlo method…

Nuclear Theory · Physics 2013-12-04 Alessandro Roggero , Abhishek Mukherjee , Francesco Pederiva

Atomic properties such as field shift constants, magnetic dipole and electric quadrupole hyperfine structure constants, Land\'e $g_J$ factors, and electric quadrupole moments that are described by electronic operators with different ranks…

Atomic Physics · Physics 2018-03-14 Pradeep Kumar , Cheng-Bin Li , B. K. Sahoo

Weak H2 physisorption energies present a significant challenge to even the best correlated theoretical many-body methods. We use the phaseless auxiliary-field quantum Monte Carlo (AFQMC) method to accurately predict the binding energy of…

Computational Physics · Physics 2011-11-02 Wirawan Purwanto , Henry Krakauer , Yudistira Virgus , Shiwei Zhang

A relativistic version of the coupled-cluster single-double (CCSD) method is developed for atoms with a single valence electron. In earlier work, a linearized version of the CCSD method (with extensions to include a dominant class of triple…

Atomic Physics · Physics 2009-11-13 Rupsi Pal , M. S. Safronova , W. R. Johnson , Andrei Derevianko , Sergey G. Porsev

We extend the variational cluster approach to deal with strongly correlated lattice bosons in the superfluid phase. To this end, we reformulate the approach within a pseudoparticle formalism, whereby cluster excitations are described by…

Quantum Gases · Physics 2011-04-11 Michael Knap , Enrico Arrigoni , Wolfgang von der Linden

Modern quantum Monte Carlo (QMC) methods often capture electron correlation through both explicitly correlating Jastrow factors and small to mid-sized configuration interaction (CI) expansions. Here, we study the additional optimization…

Chemical Physics · Physics 2023-02-08 Scott M. Garner , Eric Neuscamman

Properties of nuclear systems at subsaturation densities can be obtained from different approaches. We demonstrate the use of the density autocorrelation function which is related to the isothermal compressibility and, after integration, to…

Nuclear Theory · Physics 2017-12-07 Gerd Roepke , Dmitri Voskresensky , Ivan Kryukov , David Blaschke

In this work, we present an analytical theory of strongly correlated Wigner crystals (WCs) in the lowest Landau level (LLL) by constructing an approximate, but accurate effective two-body interaction for composite fermions (CFs)…

Strongly Correlated Electrons · Physics 2015-09-09 Jun-Won Rhim , Jainendra K. Jain , Kwon Park

We investigate possible effects of correlations between stopped nucleons on higher order proton cumulants at low energy heavy-ion collisions. We find that fluctuations of the number of wounded nucleons $N_{\mathrm{part}}$ lead to rather…

Nuclear Theory · Physics 2017-05-24 Adam Bzdak , Volker Koch , Vladimir Skokov

We have studied electron correlations in the doped two-dimensional (2D) Hubbard model by using the coupled-cluster method (CCM) to investigate whether or not the method can be applied to correct the independent particle approximations…

Strongly Correlated Electrons · Physics 2009-10-31 Yoshihiro Asai , Hideki Katagiri

We present an ab initio study of electronic correlation effects in a molecular cluster derived from the hexanuclear ferric wheel [LiFe6(OCH3)12-(dbm)6]PF6. The electronic and magnetic properties of this cluster have been studied with…

Materials Science · Physics 2007-05-23 H. Nieber , K. Doll , G. Zwicknagl

A theory is developed for the paired even-denominator fractional quantum Hall states in the lowest Landau level. We show that electrons bind to quantized vortices to form composite fermions, interacting through an exact instantaneous…

Strongly Correlated Electrons · Physics 2015-05-14 Yuan-Ming Lu , Yue Yu , Ziqiang Wang

In this paper, we have studied electron correlation and Gaunt interaction effects in ionization potentials (IPs) and hyperfine constants A of 2p$^2P_{1/2}$ and 2p$^2P_{3/2}$ states along with the fine structure splitting (FSS) between them…

Atomic Physics · Physics 2011-11-23 Narendra Nath Dutta , Sonjoy Majumder

Herein, we report accurate atomization energy calculations for 55 molecules in the Gaussian-2 (G2) set using lattice regularized diffusion Monte Carlo (LRDMC). We compare the Jastrow-Slater determinant ansatz with a more flexible JsAGPs…

Chemical Physics · Physics 2023-04-19 Abhishek Raghav , Ryo Maezono , Kenta Hongo , Sandro Sorella , Kousuke Nakano

Hyperfine-structure constants of odd Ra$^{+}$ due to the interactions of nuclear magnetic dipole, electric quadrupole, and magnetic octupole moments with the electrons are investigated in the framework of relativistic coupled-cluster method…

Atomic Physics · Physics 2021-03-16 Fei-Chen Li , Yong-Bo Tang , Hao-Xue Qiao , Ting-Yun Shi

We present an investigation into the use of an explicitly correlated plane wave basis for periodic wavefunction expansions at the level of second-order M{\o}ller-Plesset perturbation theory (MP2). The convergence of the electronic…

Computational Physics · Physics 2014-10-10 Andreas Grüneis , James J. Shepherd , Ali Alavi , David P. Tew , George H. Booth