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Multi-dimensional coherent spectroscopy (MDCS)1,2 is a powerful method for optical spectroscopy that has become an important tool for studying ultrafast dynamics in a wide range of systems. It is an optical analog of multidimensional…

Optics · Physics 2018-10-24 Bachana Lomsadze , Brad. C. Smith , Steven T. Cundiff

A full-field chromatic confocal microscopy using a multispectral sensor was developed for quasi-one-shot microscopic 3D surface measurement. An innovative optical configuration employs a digital micromirror device (DMD) and a multispectral…

Photocurrent spectroscopy is a versatile technique to identify and understand the optoelectronic dynamics occurring in semiconductor nanowires. Conventional photocurrent spectroscopy allows to explore the morphology and material properties…

Mesoscale and Nanoscale Physics · Physics 2014-09-02 Nadine Erhard , Alexander Holleitner

Multiphoton femtosecond coherent control of is used for implementing innovative photo-induced analog coherent computation that generally might be a basis for future "smart hardware". The specific implemented computational task the…

Atomic Physics · Physics 2009-10-21 Lev Chuntonov , Leonid Rybak , Andrey Gandman , Zohar Amitay

Multidimensional coherent spectroscopy (MDCS) has been established in quantum chemistry as a powerful tool for studying the nonlinear response and nonequilibrium dynamics of molecular systems. More recently, the technique has also been…

Strongly Correlated Electrons · Physics 2025-05-12 Jiyu Chen , Philipp Werner

On-chip spectroscopy that could realize real-time fingerprinting with label-free and high-throughput detection of trace molecules is one of the 'holy grails" of sensing. Such miniaturized spectrometers would greatly enable applications in…

We report, for the first time, a multi-confocal Fluorescence Correlation Spectroscopy (mFCS) technique which allows parallel measurements at different locations, by combining a Spatial Light Modulator (SLM), with an Electron Multiplying-CCD…

We have previously demonstrated that in the context of two-dimensional (2D) coherent electronic spectroscopy measured by phase modulation and phase-sensitive detection, an \emph{incoherent} nonlinear response, due to pairs of…

Wide bandgap semiconductors are widely used in photonic technologies due to their advantageous features, such as large optical bandgap, low losses, and fast operational speeds. Silicon carbide is a prototypical wide bandgap semiconductor…

Optics · Physics 2023-10-26 Ahsan Ali , Chuanliang Wang , Jinyang Cai , Khadga Jung Karki

We employ polarization-shaped ultrafast optical pulses to generate photocurrents which only arise if the optically induced coherent polarization is frequency modulated. This frequency modulation is obtained via detuned excitation of…

Optics · Physics 2013-06-14 Shekhar Priyadarshi , Klaus Pierz , Mark Bieler

We employ two-dimensional (2D) coherent, nonlinear spectroscopy to investigate couplings within individual InAs quantum dots (QD) and QD molecules. Swapping pulse ordering in a two-beam sequence permits to distinguish between rephasing and…

We report a theoretical description and experimental implementation of a novel two-dimensional coherent excitation spectroscopy based on quasi-steady-state photoinduced absorption measurement of a long-lived nonlinear population. We have…

Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…

Double-quantum two-dimensional coherent spectroscopy (MDCS) is a powerful optical method that is used to study optical properties of atomic and complex molecular systems and semiconductor materials. Double-quantum 2D spectra and…

Optics · Physics 2020-10-21 Bachana Lomsadze , Steven T. Cundiff

The investigation of optoelectronic devices based on two-dimensional materials and their heterostructures is a very active area of investigation with both fundamental and applied aspects involved. We present a description of a home-built…

Mesoscale and Nanoscale Physics · Physics 2017-05-05 Christoph Reuter , Riccardo Frisenda , Der-Yuh Lin , Tsung-Shine Ko , David Perez de Lara , Andres Castellanos-Gomez

Dual-comb interferometry utilizes two optical frequency combs to map the optical field's spectrum to a radio-frequency signal without using moving parts, allowing improved speed and accuracy. However, the method is compounded by the…

We present a novel three-dimensional (3D) imaging approach that combines two-dimensional spatial Fourier-domain imaging techniques with traditional radar pulse compression to recover both cross-range and down-range scene information. The…

Signal Processing · Electrical Eng. & Systems 2025-07-11 Jorge R. Colon-Berrios , Jason M. Merlo , Jeffrey A. Nanzer

In high-performance solar cells based on polymeric semiconductors, the mechanism of photocarrier generation on $<100$-fs timescales is yet to be unravelled. In particular the dynamics of early-time electronic coupling between excitons on…

Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent…

Coplanar waveguide resonators are central to the thriving field of circuit quantum electrodynamics. Recently, we have demonstrated the generation of a broadband microwave-frequency comb spectrum using a superconducting quantum interference…

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