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The electronic wavefunctions of an atom or molecule are affected by its interactions with its environment. These interactions dictate electronic and optical processes at interfaces, and is especially relevant in the case of thin film…

Materials Science · Physics 2021-01-13 Sameer Vajjala Kesava , Moritz K. Riede

Holography relies on the interference between a known reference and a signal of interest to reconstruct both the amplitude and phase of that signal. Commonly performed with photons and electrons, it finds numerous applications in imaging,…

Interfaces remain one of the major issues in limiting the understanding and designing polymer nanocomposites due to their complexity and pivotal role in determining the ultimate composites properties. In this study, we take multi-walled…

Materials Science · Physics 2017-11-20 Yuhan Li , Faxiang Qin , Huan Wang , Hua-Xin Peng

Diffraction of light at lateral inhomogenities is a central process in the near-field studies of nanoscale phenomena, especially the propagation of surface waves. Theoretical description of this process is extremely challenging due to…

Mesoscale and Nanoscale Physics · Physics 2021-02-24 Egor Nikulin , Denis Bandurin , Dmitry Svintsov

The nanoscopic mass and charge distribution within the double layer at electrified interfaces plays a key role in electrochemical phenomena of huge technological relevance for energy production and conversion. However, in spite of its…

Chemical Physics · Physics 2019-05-29 Remi Khatib , Ashwinee Kumar , Stefano Sanvito , Marialore Sulpizi , Clotilde S. Cucinotta

We study emission of photoelectrons from plasmonic nanoparticles into surrounding matrix. We consider two mechanisms of the photoelectric effect from nanoparticles - surface and volume ones, and use models of these two effects which allow…

This work describes three diffuse-interface methods for the simulation of immiscible, compressible multiphase fluid flows and elastic-plastic deformation in solids. The first method is the localized-artificial-diffusivity approach of Cook…

Computational Physics · Physics 2021-09-21 Suhas S. Jain , Michael C. Adler , Jacob R. West , Ali Mani , Parviz Moin , Sanjiva K. Lele

Injection from metallic electrodes serves as a main channel of charge generation in organic semiconducting devices and the quantum effect is normally regarded to be essential. We develop a dynamic approach based upon the surface hopping…

Applied Physics · Physics 2021-01-20 Jiaqing Huang , Yijie Mo , Yao Yao

Light absorption and scattering of plasmonic metal nanoparticles can lead to non-equilibrium charge carriers, intense electromagnetic near-fields, and heat generation, with promising applications in a vast range of fields, from chemical and…

Optics · Physics 2020-08-27 Guillaume Baffou , Ivan Bordacchini , Andrea Baldi , Romain Quidant

Multilayer van der Waals (vdW) heterostructures have become an important platform in which to study novel fundamental effects emerging at the nanoscale. Standard nanopatterning techniques relying on electron-beam lithography and reactive…

We study the significance and characteristics of interfacial dynamical charge transfer at metal-organic interfaces for the organic semiconductor model system 1,4,5,8-naphthalene-tetracarboxylic dianhydride (NTCDA) on Ag(111) quantitatively.…

Chemical Physics · Physics 2016-05-26 Phil Rosenow , Peter Jakob , Ralf Tonner

We propose a method for ultra-sensitive displacement and phase metrology based on the interferometric evanescent wave excitation of nano-antennas. We show that with a proper choice of nano-antenna, tiny displacements or relative phase…

The structure and dynamics of isolated nanosamples in free flight can be directly visualized via single-shot coherent diffractive imaging using the intense and short pulses of X-ray free-electron lasers. Wide-angle scattering images even…

Near-field microscopy is widely used for characterizing electromagnetic fields at nanoscale, where nanoprobes afford the opportunity to extract subwavelength optical quantities, including the amplitude, phase, polarization and chirality.…

Optics · Physics 2018-08-01 Lin Sun , Benfeng Bai , Jia Wang

Direct observation of nanoscale transformations in three dimensions (3D) is essential for understanding materials evolution under operating conditions, yet dynamic electron tomography remains limited by slow tilt series acquisition and by…

Atomic diffusion at nanometer length scale may differ significantly from bulk diffusion, and may sometimes even exhibit counterintuitive behavior. In the present work, taking Cu/Ni as a model system, a general phenomenon is reported which…

Materials Science · Physics 2019-05-15 Atul Tiwari , M. K. Tiwari , Mukul Gupta , H. -C. Wille , Ajay Gupta

Spatial interferometry, based on the measurement of total absorbed power, can be used to determine the state of coherence of the electromagnetic field to which any energy-absorbing structure is sensitive. The measured coherence tensor can…

Quantum Physics · Physics 2015-06-11 Stafford Withington , Christopher N. Thomas

This paper reports theoretical and numerical investigations on free molecular gas flows through micro-channels. Both diffusely and specularly reflective channel surfaces are considered. Gaskinetic methods are adopted to develop the…

Fluid Dynamics · Physics 2020-08-26 Shiying Cai , Chunpei Cai , Jun Li

Nonlinear optics underpins a broad range of photonic technologies, from classical and quantum light sources to emerging nonlinear photonic neural networks. Yet, conventional nonlinear optical devices exhibit static functionality: their…

We investigate the mobility of nanometer-size solutes in water in a uniform external electric field. General arguments are presented to show that a closed surface cutting a volume from a polar liquid will carry an effective non-zero surface…

Soft Condensed Matter · Physics 2016-08-24 Mohammadhasan Dinpajooh , Dmitry V. Matyushov