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The formation of ice in mixed phase clouds greatly impacts Earths hydrologic cycle. The intensity, distribution and frequency of precipitation as well as radiative properties of clouds in the mid latitudes are strongly influenced by the…

Atmospheric and Oceanic Physics · Physics 2019-06-17 Prasanth Prabhakaran , Gregory Kinney , Will Cantrell , Raymond A. Shaw , Eberhard Bodenschatz

Context. Water together with O2 are important gas phase ingredients to cool dense gas in order to form stars. On dust grains, H2 O is an important constituent of the icy mantle in which a complex chemistry is taking place, as revealed by…

Solar and Stellar Astrophysics · Physics 2015-05-19 S. Cazaux , V. Cobut , M. Marseille , M. Spaans , P. Caselli

Methanol is formed via surface reactions on icy dust grains. Methanol is also detected in the gas-phase at temperatures below its thermal desorption temperature and at levels higher than can be explained by pure gas-phase chemistry. The…

Solar and Stellar Astrophysics · Physics 2018-05-02 N. F. W. Ligterink , C. Walsh , R. G. Bhuin , S. Vissapragada , J. Terwisscha van Scheltinga , H. Linnartz

During the evolution of diffuse clouds to molecular clouds, gas-phase molecules freeze out on surfaces of small dust particles to form ices. On dust surfaces, water is the main constituent of the icy mantle in which a complex chemistry is…

Solar and Stellar Astrophysics · Physics 2015-06-22 S. Hocuk , S. Cazaux

Ice nucleation from vapor presents a variety of challenges across a wide range of industries and applications including refrigeration, transportation, and energy generation. However, a rational comprehensive approach to fabricating…

Condensation and frost formation degrade the heat transfer performance of air-conditioners and refrigerators. Yet, the frost formation mechanism has not been fully understood. In the present study, we numerically investigated H2O droplets…

Mesoscale and Nanoscale Physics · Physics 2021-04-27 Yoshitaka Ueki , Yuta Tsutsumi , Masahiko Shibahara

We have performed experimental investigations of methanol formation via the reactions of low energy $CH_{3}^{+}$ ions with an amorphous solid water (ASW) surface around 10 K. A newly developed experimental apparatus enabled irradiation of…

Astrophysics of Galaxies · Physics 2023-04-27 Y. Nakai , W. M. C. Sameera , K. Furuya , H. Hidaka , A. Ishibashi , N. Watanabe

Solid particles in protoplanetary discs can grow by direct vapour deposition outside of ice lines. The presence of microscopic silicate particles may nevertheless hinder growth into large pebbles, since the available vapour is deposited…

Earth and Planetary Astrophysics · Physics 2019-09-11 Katrin Ros , Anders Johansen , Ilona Riipinen , Daniel Schlesinger

In this work, we perform a systematic computer simulation study of ice premelting, and explore the thickness and structure of quasi-liquid layers formed at the interface of ice with substrates of different hydrophilicity. Our study shows…

Soft Condensed Matter · Physics 2024-10-30 Łukasz Baran , Pablo Llombart , Luis G. MacDowell

In this work we perform computer simulations of the ice surface in order to elucidate the role of nitrogen in the crystal growth rates and crystal habits of snow in the atmosphere. In pure water vapor at temperatures typical of ice crystal…

Chemical Physics · Physics 2020-09-09 Pablo Llombart , Ramón M. Bergua , Eva G. Noya , Luis G. MacDowell

Methanol is a common component of interstellar and circumstellar ice mantles and is often used as an evolution indicator in star-forming regions. The observations of gas-phase methanol in the interiors of dense molecular clouds at…

Instrumentation and Methods for Astrophysics · Physics 2016-07-27 Gustavo A. Cruz-Diaz , Rafael Martín-Doménech , Guillermo M. Muñoz Caro , Y. -J. Chen

It is surprisingly difficult to freeze water. Almost all ice that forms under "mild" conditions (temperatures > -40 degrees Celsius) requires the presence of a nucleating agent - a solid particle that facilitates the freezing process - such…

Statistical Mechanics · Physics 2014-04-25 Stephen J. Cox , Zamaan Raza , Shawn M. Kathmann , Ben Slater , Angelos Michaelides

A uniform solidification front undergoes non-trivial deformations when encountering an insoluble dispersed particle in a melt. For solid particles, the overall deformation characteristics are primarily dictated by heat transfer between the…

Fluid Dynamics · Physics 2024-03-01 Duco van Buuren , Pallav Kant , Jochem G. Meijer , Christian Diddens , Detlef Lohse

Dendrites formation in the course of crystallization presents very general phenomenon, which is analyzed in details via the example of ice crystals growth in deionized water. Neutral molecules of water on the surface are combined into the…

Atmospheric and Oceanic Physics · Physics 2009-11-13 Mark E. Perel'man , Galina M. Rubinstein , Vitali A. Tatartchenko

We present experimental constraints on the insertion of oxygen atoms into methane to form methanol in astrophysical ice analogs. In gas-phase and theoretical studies this process has previously been demonstrated to have a very low or…

Earth and Planetary Astrophysics · Physics 2017-08-23 Jennifer B. Bergner , Karin I. Oberg , Mahesh Rajappan

The issue of ice accumulation at low-temperature circumstances causes multiple problems and serious damages in many civil infrastructures which substantially influence human daily life. However, despite the significant consideration in…

Chemical Physics · Physics 2020-11-24 Amir Afshar , Dong Meng

Freezing is a fundamental physical phenomenon that has been studied over many decades; yet the role played by surfaces in determining nucleation has remained elusive. Here we report direct computational evidence of surface induced…

Statistical Mechanics · Physics 2015-05-13 T. Li , D. Donadio , L. M. Ghiringhelli , G. Galli

Water-repellent properties of superhydrophobic surfaces make them promising for anti-icing and deicing applications. Through experimental visualization of frozen sessile droplets undergoing melting on superhydrophobic surfaces, we identify…

Fluid Dynamics · Physics 2026-02-10 Jiawang Cui , Yugang Zhao , Tianyou Wang , Zhizhao Che

Despite its importance in atmospheric science, much remains unknown about the microscopic mechanism of heterogeneous ice nucleation. In this work, we perform hybrid Monte Carlo simulations of the heterogeneous nucleation of ice on a range…

Statistical Mechanics · Physics 2014-08-25 Aleks Reinhardt , Jonathan P. K. Doye

Control of water ice formation on surfaces is of key technological and economic importance, but the fundamental understanding of ice nucleation and growth mechanisms and the design of surfaces for controlling water freezing behaviour remain…

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