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We demonstrate a powerful tool for high-resolution mid-IR spectroscopy and frequency metrology with quantum cascade lasers (QCLs). We have implemented frequency stabilization of a QCL to an ultra-low expansion (ULE) reference cavity, via…

We have built a frequency chain which enables to measure the absolute frequency of a laser emitting in the 28-31 THz frequency range and stabilized onto a molecular absorption line. The set-up uses an optical frequency comb and an…

A continuous-wave Fabry-Perot quantum cascade laser (QCL) emitting at 8.1 $\mu$m operating in the single mode regime has been coherently phase locked to a turn-key low-noise commercial mid-Infrared (mid-IR) optical frequency comb. The…

Quantum Cascade Lasers (QCL) are increasingly being used to probe the mid-infrared "molecular fingerprint" region. This prompted efforts towards improving their spectral performance, in order to reach ever-higher resolution and precision.…

The advancement of technologies for the precise interrogation of molecules offers exciting possibilities for new studies in the realms of precision spectroscopy and quantum technologies. Experiments in these domains often address molecular…

Optics · Physics 2022-09-15 Mudit Sinhal , Anatoly Johnson , Stefan Willitsch

Quantum cascade laser (QCL) frequency combs have revolutionized mid-infrared (MIR) spectroscopy by their high brightness and fast temporal resolution, and are a promising technology for fully-integrated and cost-effective sensors. As for…

We present a new method for accurate mid-infrared frequency measurements and stabilization to a near-infrared ultra-stable frequency reference, transmitted with a long-distance fibre link and continuously monitored against state-of-the-art…

The mid-infrared (mid-IR) regime (typically the wavelength regime of $\lambda \sim 2.5-20 \ \mathrm{\mu m}$) is an important spectral range for spectroscopy as many molecules have their fundamental rotational-vibrational absorption in this…

Frequency-stabilized mid-infrared lasers are valuable tools for precision molecular spectroscopy. However, their implementation remains limited by complicated stabilization schemes. Here we achieve optical self-locking of a quantum cascade…

Optics · Physics 2021-06-29 Gang Zhao , Jianfei Tian , Joseph T. Hodges , Adam J. Fleisher

A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…

Optics · Physics 2017-04-05 Markku Vainio , Juho Karhu

Optical frequency comb synthesizers (FCs) [1] are laser sources covering a broad spectral range with a number of discrete, equally spaced and highly coherent frequency components, fully controlled through only two parameters: the frequency…

We describe a coherent mid-infrared continuum source with 700 cm-1 usable bandwidth, readily tuned within 600 - 2500 cm-1 (4 - 17 \mum) and thus covering much of the infrared "fingerprint" molecular vibration region. It is based on…

Quantum Physics · Physics 2015-06-04 Fritz Keilmann , Sergiu Amarie

Frequency combs are powerful tools for many applications and high performances are achieved by stabilizing these lasers. For operation in the mid-infrared, quantum cascade lasers (QCL) are ideal candidates as they present numerous…

Interferometric wavelength meters have attained frequency resolutions down to the MHz range. In particular, Fizeau interferometers, which have no moving parts, are becoming a popular tool for laser characterization and stabilization. In…

Mid-infrared (MIR) spectrometers are invaluable tools for molecular fingerprinting and hyper-spectral imaging. Among the available spectroscopic approaches, GHz MIR dual-comb absorption spectrometers have the potential to simultaneously…

Mid infrared (MIR) photonics is a key region for molecular physics [1]. High-resolution spectroscopy in the 1--10 {\mu}m region, though, has never been fully tackled for the lack of widely-tunable and practical light sources. Indeed, all…

We present a system for molecular spectroscopy using a broadband mid-infrared laser with near infrared detection. Difference frequency generation of a Yb:fiber femtosecond laser produced a mid-infrared (MIR) source tunable from 2100-3700…

Optics · Physics 2015-05-30 Todd A. Johnson , Scott A. Diddams

We report on a calibration procedure that enhances the precision of an interferometer based frequency stabilization by several orders of magnitude. For this purpose the frequency deviations of the stabilization are measured precisely by…

Optics · Physics 2012-08-14 Johannes F. S. Brachmann , Thomas Kinder , Kai Dieckmann

We present a solid-state laser system that generates over 200 mW of continuous-wave, narrowband light, tunable from 316.3 nm - 317.7 nm and 318.0 nm - 319.3 nm. The laser is based on commercially available fiber amplifiers and optical…

In this paper, we present an experimental study of the metrological stabilization of a solid-state frequency comb for embedded metrology applications. The comb is a passively mode-locked laser diode based on InGaAs/InP Quantum-dash…

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