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Electrical tuning of second-order nonlinearity in optical materials is attractive to strengthen and expand the functionalities of nonlinear optical technologies, though its implementation remains elusive. Here, we report the electrically…

The emergent behaviors in thin films of a multiaxial ferroelectric due to an electrochemical coupling between the rotating polarization and surface ions are explored within the framework of the 2-4 Landau-Ginzburg-Devonshire (LGD)…

A key property that drives research in ferroelectric perovskite oxides is their strong piezoelectric response in which an electric field is induced by an applied strain, and vice-versa for the converse piezoelectric effect. We have achieved…

Materials Science · Physics 2015-06-11 J. Sinsheimer , S. J. Callori , B. Bein , Y. Benkara , J. Daley , J. Coraor , D. Su , P. W. Stephens , M. Dawber

Two-dimensional mirror symmetry enriched topological (SET) orders can be studied using the folding approach: it can be folded along the mirror axis and turned into a bilayer system on which the mirror symmetry acts as a $\mathbb Z_2$…

Strongly Correlated Electrons · Physics 2024-11-08 Zhaoyang Ding , Yang Qi

At interfaces between conventional materials, band bending and alignment are classically controlled by differences in electrochemical potential. Applying this concept to oxides in which interfaces can be polar and cations may adopt a mixed…

We investigate two-dimensional trilayered quantum systems with multi-orbital conduction bands by focusing on the role played by the layer degree of freedom in setting the character of nodal line semimetals. The layer index can label the…

Mesoscale and Nanoscale Physics · Physics 2019-07-24 F. Forte , D. Guerra , C. Noce , W. Brzezicki , M. Cuoco

Understanding and controlling the atomic structure of polar oxide surfaces is essential for unraveling surface reactivilty and designing advanced catalytic materials. Among these, the polar CeO2(100) surface is a prototypical and…

Large electron-electron Coulomb-interactions in correlated systems can lead to a periodic arrangement of localized electrons, the so called "charge-order". The latter is here proposed as a driving force behind ferroelectricity in iron…

Materials Science · Physics 2015-05-14 Kunihiko Yamauchi , Silvia Picozzi

Nonlinear electrostatic interaction between the surface ions of electrochemical nature and ferroelectric dipoles gives rise to the coupled ferroionic states in nanoscale ferroelectrics. Here, we investigated the role of the surface ions…

We explore computationally the formation of tri-layer superlattices as an alternative approach for combining ferroelectricity with magnetism to form magnetoelectric multiferroics. We find that the contribution to the superlattice…

Materials Science · Physics 2011-11-09 Alison J. Hatt , Nicola A. Spaldin

In the light of new experimental evidence we study the insulating ground state of the $3d^2$-transition metal trihalides VX$_3$ (X=Cl, I). Based on Density Functional Theory with the Hubbard correction (DFT$+U$) we systematically show how…

Strongly Correlated Electrons · Physics 2025-03-13 Luigi Camerano , Gianni Profeta

We investigate the phase separated inhomogeneous charge and spin states in magnetic oxides. In particular, we study one dimensional harmonic waves and stripe structures. We show that harmonic spin charge waves are unstable and inevitably…

Strongly Correlated Electrons · Physics 2019-09-04 O. G. Udalov , I. S. Beloborodov

The electric field control of functional properties is a crucial goal in oxide-based electronics. Non-volatile switching between different resistivity or magnetic states in an oxide channel can be achieved through charge accumulation or…

Transition metal dichalcogenides (TMDs) combine interesting optical and spintronic properties in an atomically-thin material, where the light polarization can be used to control the spin and valley degrees-of-freedom for the development of…

Mesoscale and Nanoscale Physics · Physics 2021-03-10 Carmem M. Gilardoni , Freddie Hendriks , Caspar H. van der Wal , Marcos H. D. Guimarães

Cooperative optical effects are enabled and controlled by interactions between molecular dipoles, meaning that their mutual orientation is of paramount importance to, for example, superabsorbing light-harvesting antennas. Here we show how…

Optics · Physics 2025-02-27 Adam Burgess , Madeline C. Waller , Erik M. Gauger , Robert Bennett

The coexistence of different ferroelectric phases enables the tunability of the macroscopic properties and extensive applications from piezoelectric transducers to nonvolatile memories. Here we develop a thermodynamic model to predict the…

Materials Science · Physics 2022-01-26 Yang Zhang , Fei Xue , Bo Wang , Jia-Mian Hu , Shuai Dong , Jun-Ming Liu , Long-Qing Chen

The crystal structure of a material plays an important role in determining its electronic properties. Changing from one crystal structure to another involves a phase transition which is usually controlled by a state variable such as…

Strong-field methods in solids enable new strategies for ultrafast nonlinear spectroscopy and provide all-optical insights into the electronic properties of condensed matter in reciprocal and real space. Additionally, solid-state media…

The synergy of ferroicity with altermagnetism offers a novel platform for designing multifunctional altermagnetic-spintronic device technology. In this work, we propose a mechanism to achieve nonvolatile electrical manipulation of spin and…

Materials Science · Physics 2026-03-12 Rui Peng , Guangxu Su , Yangyang Fan , Jiaan Li , Fanxin Liu , Yee Sin Ang

We study the geometric and electronic structures of silicene monolayer using density functional theory based calculations. The electronic structures of silicene show that it is a semi-metal and the charge carriers in silicene behave like…

Mesoscale and Nanoscale Physics · Physics 2012-05-23 Kamal Chinnathambi