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We investigate electrostatic stability of charged droplets, modeled as permeable, charged spheres, and their encapsidation in thin, arbitrarily charged nano-shells, immersed in a neutralizing asymmetric electrolyte background. The latter…

Soft Condensed Matter · Physics 2013-11-15 Leili Javidpour , Anže Lošdorfer Božič , Ali Naji , Rudolf Podgornik

We formulate an extension of the Debye-Hueckel-Bjerrum theory [M. E. Fisher and Y. Levin, Phys. Rev. Lett. 71, 3826 (1993)] to the fluid state of a highly asymmetric charged colloid. Allowing for the formation of clusters consisting of one…

Soft Condensed Matter · Physics 2015-06-25 M. N. Tamashiro , Yan Levin , Marcia C. Barbosa

This article presents a systematic theoretical enquiry concerning the conceptual foundations and the nature of phonon-mediated electron-electron interactions. Starting from the fundamental many-body Hamiltonian, we propose a simple scheme…

Materials Science · Physics 2020-09-08 R. Starke , G. A. H. Schober

We present theoretical and numerical studies on stiff, linear polyelectrolytes within the framework of the cell model. We first review analytical results obtained on a mean-field Poisson-Boltzmann level, and then use molecular dynamics…

Soft Condensed Matter · Physics 2009-11-07 Markus Deserno , Christian Holm

Understanding the response of the surface of metallic solids to external electric field sources is crucial to characterize electrode-electrolyte interfaces. Continuum electrostatics offer a simple description of the induced charge density…

Chemical Physics · Physics 2021-12-14 Giovanni Pireddu , Laura Scalfi , Benjamin Rotenberg

We present a theory which allows us to calculate the interaction potential between charge-regulated metal nanoparticles inside an acid-electrolyte solution. The approach is based on the recently introduced model of charge regulation which…

Soft Condensed Matter · Physics 2020-12-11 Amin Bakhshandeh , Alexandre P. dos Santos , Yan Levin

The general form of the electrostatic potential around an arbitrarily charged colloid at an interface between a dielectric and a screening phase (such as air and water, respectively) is analyzed in terms of a multipole expansion. The…

Soft Condensed Matter · Physics 2008-07-11 A. Dominguez , D. Frydel , M. Oettel

A proper treatment of electrostatic interactions is crucial for the accurate calculation of forces in computer simulations. Electrostatic interactions are typically modeled using Ewald based methods, which have become one of the…

Soft Condensed Matter · Physics 2016-09-21 K. A. Terrón-Mejía , R. López-Rendón , A. Gama Goicochea

We study thermal equilibrium of classical pointlike counterions confined between symmetrically charged walls at distance $d$. At very large couplings when the counterion system is in its crystal phase, a harmonic expansion of particle…

Soft Condensed Matter · Physics 2019-01-21 L. Samaj , M. Trulsson , E. Trizac

The article presents a comprehensive study of counterion dynamics around a generic linear polyelectrolyte (PE) chain with the help of coarse-grained computer simulations. The ion-chain coupling is discussed in the form of binding time,…

Soft Condensed Matter · Physics 2022-04-13 Keerthi Radhakrishnan , Sunil P. Singh

We set up a mesoscopic theory for interacting Brownian particles embedded in a nonequilibrium environment, starting from the microscopic interacting many-body theory. Using nonequilibrium linear response theory, we characterize the…

Statistical Mechanics · Physics 2017-01-04 Stefano Steffenoni , Klaus Kroy , Gianmaria Falasco

Electrolytes play an important role in a plethora of applications ranging from energy storage to biomaterials. Notwithstanding this, the structure of concentrated electrolytes remains enigmatic. Many theoretical approaches attempt to model…

Soft Condensed Matter · Physics 2021-04-14 Penelope Jones , Fabian Coupette , Andreas Härtel , Alpha A. Lee

We compare the recent experimentally measured forces between charged colloidal particles, as well as their effective surface potentials (surface charge) in the presence of multivalent counterions in a bathing monovalent salt solution, with…

Soft Condensed Matter · Physics 2017-05-24 Matej Kanduč , Mohsen Moazzami Gudarzi , Valentina Valmacco , Rudolf Podgornik , Gregor Trefalt

Machine learning models for the potential energy of multi-atomic systems, such as the deep potential (DP) model, make possible molecular simulations with the accuracy of quantum mechanical density functional theory, at a cost only…

We numerically simulate collisions of charged shockwaves in Einstein-Maxwell theory in anti-de Sitter space as a toy model of heavy ion collisions with non-zero baryon charge. The stress tensor and the baryon current become well described…

High Energy Physics - Theory · Physics 2017-07-05 Jorge Casalderrey-Solana , David Mateos , Wilke van der Schee , Miquel Triana

Forces between charged silica particles in solutions of multivalent coions are measured with colloidal probe technique based on atomic force microscopy. The concentration of 1:z electrolytes is systematically varied to understand the…

Soft Condensed Matter · Physics 2019-08-08 Biljana Uzelac , Valentina Valmacco , Gregor Trefalt

Recently, underscreening in concentrated electrolytes was discovered in experiments and confirmed in simulations and theory. It was found that the correlation length of the charge-charge correlations, $\lambda_s$, satisfies the scaling…

Statistical Mechanics · Physics 2022-11-07 A. Ciach , O. Patsahan

Bulk properties and free interfaces of mixtures of charged platelike colloids and salt are studied within density-functional theory. The particles are modeled by hard cuboids with their edges constrained to be parallel to the artesian axes…

Other Condensed Matter · Physics 2011-09-14 Markus Bier , Ludger Harnau , S. Dietrich

In this brief contribution to the Proceedings of the NATO-ASI on ``Electrostatic Effects in Soft Matter and Biophysics'', which took place in Les Houches from Oct. 1-13, 2000, we summarize in short aspects of the simulations methods to…

Soft Condensed Matter · Physics 2007-05-23 C. Holm , K. Kremer

Using computer simulations, the electrophoretic motion of a positively charged colloid (macroion) in an electrolyte solution is studied in the framework of the primitive model. Hydrodynamic interactions are fully taken into account by…

Soft Condensed Matter · Physics 2015-06-25 Apratim Chatterji , Jürgen Horbach
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