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Dielectric properties are intimately related to the content and composition of the liquid phase present in micro- and mesoporous materials. The presence of ions is recognized to affect the dielectric response of electrolytes in a complex…

Soft Condensed Matter · Physics 2019-10-25 Tulio Honorio , Thierry Bore , Farid Benboudjema , Eric Vourc'h , Mehdi Ferhat

Transport coefficients and dielectric relaxation in liquids are often treated as distinct manifestations of molecular dynamics. We show that, in polar liquids, orientational dipolar fluctuations generate a substantial contribution to the…

Statistical Mechanics · Physics 2026-05-12 David S. Dean , Haim Diamant

We present a nonlocal electrostatic formulation of nonuniform ions and water molecules with interstitial voids that uses a Fermi-like distribution to account for steric and correlation effects in electrolyte solutions. The formulation is…

Soft Condensed Matter · Physics 2017-03-27 Jinn-Liang Liu , Dexuan Xie , Bob Eisenberg

In situations involving large potentials or surface charges, the Poisson Boltzman(PB) equation has shortcomings because it neglects ion-ion interactions and steric effects. This has been widely recognized by the electrochemistry community,…

Chemical Physics · Physics 2007-05-23 Mustafa Sabri Kilic , Martin Z. Bazant , Armand Ajdari

In this paper, we study electrostatic properties between two similar or oppositely charged surfaces immersed in an electrolyte solution by using mean-field approach accounting for solvent polarization and non-uniform size effect. Applying a…

Soft Condensed Matter · Physics 2022-02-11 Jun-Sik Sin

For binary solvent mixtures composed of ions and two kinds of polar solvents, electric double layer near a charged object is strongly affected by not only the binary solvent composition but also nature of solvents such as volume and dipole…

Soft Condensed Matter · Physics 2022-02-11 Jun-Sik Sin , Chung-Sik Sin

In this paper, a nonuniform size modified Poisson-Boltzmann ion channel (nuSMPBIC) model is presented as a nonlinear system of an electrostatic potential and multiple ionic concentrations. It mixes nonlinear algebraic equations with a…

Numerical Analysis · Mathematics 2022-09-14 Dexuan Xie

The calculation of the solvation properties of a single water molecule in liquid water is carried out in two ways. In the first, the water molecule is placed in a cavity and the solvent is treated as a dielectric continuum. This model is…

chem-ph · Physics 2008-02-03 Steven W. Rick , B. J. Berne

We theoretically investigate electrostatic properties between two charged surfaces with a grafted polyelectrolyte layer in an aqueous electrolyte solution by using the Poisson-Boltzmann approach accounting for ion partitioning. In order to…

Soft Condensed Matter · Physics 2022-02-07 Jun-Sik Sin

The many-body $GW$ formalism, for the calculation of ionization potentials or electronic affinities, relies on the frequency-dependent dielectric function built from the electronic degrees of freedom. Considering the case of water as a…

Materials Science · Physics 2024-09-04 Ivan Duchemin , David Amblard , Xavier Blase

One important development in interaction potential models, or atomistic force fields, for molecular simulation is the inclusion of explicit polarisation, which represents the induction effects of charged or polar molecules on polarisable…

Soft Condensed Matter · Physics 2017-05-25 Agílio A. H. Pádua

We propose the construction of a set of quantum hydrodynamics equations for the Bose-Einstein condensate (BEC) where atoms have electric dipole moment (EDM). The contribution of the dipole-dipole interactions (DDI) to the Euler equation is…

Quantum Gases · Physics 2011-09-28 P. A. Andreev , L. S. Kuzmenkov

The Poisson-Boltzmann (PB) theory is extensively used to gain insight on charged colloids and biological systems as well as to elucidate fundamental properties of intermolecular forces. Many works were devoted in the past to study PB…

Soft Condensed Matter · Physics 2014-04-22 Dan Ben-Yaakov , David Andelman

We investigate the ground state properties of a polarized dipolar Bose-Einstein condensate trapped in a triple-well potential. By solving the dipolar Gross-Pitaevskii equation numerically for different geometries we identify states which…

Quantum Gases · Physics 2012-10-12 David Peter , Krzysztof Pawlowski , Tilman Pfau , Kazimierz Rzazewski

A new empirical potential for efficient, large scale molecular dynamics simulation of water is presented. The HIPPO (Hydrogen-like Intermolecular Polarizable POtential) force field is based upon the model electron density of a hydrogen-like…

Chemical Physics · Physics 2021-09-30 Joshua A. Rackers , Roseane R. Silva , Zhi Wang , Jay W. Ponder

We have investigated a single charged microgel in aqueous solution with a combined simulational model and Poisson-Boltzmann theory. In the simulations we use a coarse-grained charged bead-spring model in a dielectric continuum, with…

Soft Condensed Matter · Physics 2009-03-12 Gil C. Claudio , Christian Holm , Kurt Kremer

Lipid domains are found in systems such as multi-component bilayer membranes and single component monolayers at the air-water interface. It was shown by Andelman et al. (Comptes Rendus 301, 675 (1985)) and McConnell et al. (Phys. Chem. {\bf…

Soft Condensed Matter · Physics 2007-05-23 Alex Travesset

Electrostatic correlations between ions dissolved in water are known to impact their transport properties in numerous ways, from conductivity to ion selectivity. The effects of these correlations on the solvent itself remain, however, much…

Soft Condensed Matter · Physics 2024-01-31 Paul Robin

Perovskite structure materials based on the Ba1-xGdxTiO3 system, where x = 0.001, 0.002, 0.003, 0.004 and 0.005, were prepared via the Pechini chemical synthesis route. The dielectric properties have been analyzed over a wide temperature…

Materials Science · Physics 2024-09-25 T. H. T. Rosa , M. A. Oliveira , Y. Mendez-Gonzalez , F. Guerrero , R. Guo , A. S. Bhalla , J. D. S. Guerra

Osmotic coefficients, individual and mean activity coefficients of primitive model electrolyte solutions are computed at different molar concentrations using the symmetric Poisson-Boltzmann and modified Poisson-Boltzmann theories. The…

Statistical Mechanics · Physics 2018-06-27 A. O. Quiñones , L. B. Bhuiyan , C. W. Outhwaite