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This work constructs an advanced force field, the Completely Multipolar Model (CMM), to quantitatively reproduce each term of an energy decomposition analysis (EDA) for aqueous solvated alkali metal cations and halide anions and their ion…

Chemical Physics · Physics 2024-10-14 J. P. Heindel , L. Kim , M. Head-Gordon , T. Head-Gordon

We give examples showing that two well-known versions of the S-matrix theory, which describes a nonresonant multiphoton ionization of atoms and ions in intense laser fields, lead to qualitatively different results. The latter refer not only…

Atomic Physics · Physics 2015-05-28 J. H. Bauer

Particle-in-cell codes are now standard tools for studying ultra-intense laser-plasma interactions. Motivated by direct laser acceleration of electrons in sub-critical plasmas, we examine temporal resolution requirements that must be…

Photoelectron interferometry with femto- and atto-second light pulses is a powerful probe of the fast electron wavepacket dynamics, albeit it has practical limitations on the energy resolution. We show that one can simultaneously obtain…

Atomic Physics · Physics 2022-02-24 A. Plunkett , M. A. Alarcon , J. K. Wood , C. H. Greene , A. Sandhu

Two-color laser fields offer significantly enhanced control over electron excitation dynamics under ultrashort intense laser pulses compared to monochromatic fields. However, their strong nonlinearity necessitates computationally expensive…

Optics · Physics 2025-07-03 Mizuki Tani , Kenichi L. Ishikawa , Tomohito Otobe

We reanalyze the problem of radiative polarization of electrons brought into collision with a circularly polarized strong plane wave. We present an independent analytical verification of formulae for the cross section given by D.\,Yu.…

Accelerator Physics · Physics 2011-12-23 Dmitry Karlovets

Strong-field light-matter interactions initiate a wide range of phenomena in which the quantumpaths of electronic wavepackets can be manipulated by tailoring the laser field. Among the electronsreleased by a strong laser pulse from atomic…

Chemical Physics · Physics 2022-11-30 S Rozen , S Larroque , N Dudovich , Y Mairesse , B Pons

In this work we report ab initio calculations for the $H_2^+$ molecule interacting with ultrashort intense laser pulses. We analyse several observables that can, in principle, be available experimentally, in order to get a deeper…

Atomic Physics · Physics 2017-05-25 R. E. F. Silva

Multiple electron processes occur widely in atoms, molecules, clusters, and condensed matters when they are interacting with energetic particles or intense laser fields. In this work, a unified and accurate theoretical formalism is proposed…

Atomic Physics · Physics 2018-04-18 Pengfei Liu , Jiaolong Zeng , Jianmin Yuan

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the…

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

Atomic Physics · Physics 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

We investigate the possibility to deduce momentum space properties from time-dependent density functional calculations. Electron and ion momentum distributions after double ionization of a model Helium atom in a strong few-cycle laser pulse…

Atomic Physics · Physics 2009-11-13 F. Wilken , D. Bauer

This article presents a systematic theoretical enquiry concerning the conceptual foundations and the nature of phonon-mediated electron-electron interactions. Starting from the fundamental many-body Hamiltonian, we propose a simple scheme…

Materials Science · Physics 2020-09-08 R. Starke , G. A. H. Schober

Electron heating and ionization dynamics in capacitively coupled radio frequency (RF) atmospheric pressure microplasmas operated in helium are investigated by Particle in Cell simulations and semi-analytical modeling. A strong heating of…

Plasma Physics · Physics 2013-06-03 T. Hemke , D. Eremin , T. Mussenbrock , A. Derzsi , Z. Donkó , K. Dittmann , J. Meichsner , J. Schulze

A scheme which allows to compute the dynamics of strongly correlated classical ions embedded into a partiallzy ionized quantum plasma by first principles molecular dynamics is presented. The dynamically screened dust approach of Joyce and…

Plasma Physics · Physics 2008-10-10 M. Bonitz , P. Ludwig , J. W. Dufty

We investigate the ionization dynamics of atoms irradiated by an intense laser field using a semiclassical model that includes magnetic Lorentz force in the rescattering process. We find that, the electrons tunneled with different initial…

Atomic Physics · Physics 2017-01-25 J. F. Tao , Q. Z. Xia , J. Cai , L. B. Fu , J. Liu

An analytical model of a single-atom electron source is presented, where electrons are created by near-threshold photoionization of an isolated atom. The model considers the classical dynamics of the electron just after the photon…

Atomic Physics · Physics 2014-07-29 W. J. Engelen , E. J. D. Vredenbregt , O. J. Luiten

The interaction of energetic ions with the electronic and ionic system of target materials is an interesting but challenging multi-scale problem and understanding of the early stages after impact of heavy, initially charged ions is…

Materials Science · Physics 2020-07-29 Cheng-Wei Lee , James A. Stewart , Stephen M. Foiles , Rémi Dingreville , André Schleife

We consider trasfer-ionization in collisions of fast (3.6 -- 11 MeV/u) protons, alpha-particles and lithium nuclei with helium atoms. There are just a few basic mechanisms contributing to this process which can be grouped into correlated…

Atomic Physics · Physics 2015-06-05 A. B. Voitkiv , X. Ma

More than 100 years after its discovery and its explanation in the energy domain, the duration of the photoelectric effect is still heavily studied. The emission time of a photoelectron can be quantified by the Wigner time delay.…