Related papers: Probing the dynamic interference in molecular high…
Measurements of the thermal conductance of single-molecule junctions have recently been reported for the first time. It is presently unclear, how much the heat transport can be controlled through molecule-internal effects. The search for…
We experimentally observe a new type of quantum-path interference, in two-dimensions (2D-QPI), in high-harmonic generation (HHG) driven by an orthogonally-polarised highly-bichromatic field. This regime is marked by comparable intensities…
We present a theoretical model of high-harmonic generation from diatomic molecules. The theory includes effects of alignment as well as nuclear motion and is used to predict results for N$_2$, O$_2$, H$_2$ and D$_2$. The results show that…
We investigate high-harmonic generation in closed systems, using the two-level atom as a simplified model. By means of a windowed Fourier transform of the time-dependent dipole acceleration, we extract the main contributions to this process…
We investigate the effect of dynamic electron correlation on high-harmonic generation in helium atoms using intense visible light (\lambda=390nm). Two complementary approaches are used which account for correlation in an approximate manner:…
We show that the Floquet approach with a Sturmian basis means an efficient description of high-order harmonic generation with monochromatic excitation. This method, although involves numerical calculations, is close to analytic approaches…
From the famous classical "simple man" model to the recent multichannel model for polyatomic molecules, this tutorial will guide you through the several landmarks in our understanding of high harmonic generation and high harmonic…
We experimentally disentangle the contributions of different quantum paths in high-order harmonic generation (HHG) from the spectrally and spatially resolved harmonic spectra. By adjusting the laser intensity and focusing position, we…
A new High Harmonic Generation (HHG) scheme, which doesn't rely on Tunnel-Ionization as the ionization mechanism but rather on Single-Photon Ionization, is theoretically proposed and numerically demonstrated. The scheme uses two driver…
We present a new trajectory formulation of high harmonic generation that treats classically allowed and classically forbidden processes within a single dynamical framework. Complex trajectories orbit the nucleus, producing the stationary…
Molecular dynamics simulations yield large amounts of trajectory data. For their durable storage and accessibility an efficient compression algorithm is paramount. State of the art domain-specific algorithms combine quantization, Huffman…
High harmonic generation (HHG) provides a flexible framework for the development of coherent light sources in the extreme-ultraviolet and soft x-ray regimes. However it suffers from low conversion efficiencies as the control of the HHG…
We study the Bohmian dynamics of a large class of bipartite systems of non-ideal qubit systems, by modifying the basic physical parameters of an ideal two-qubit system, made of coherent states of the quantum harmonic oscillator. First we…
We investigate both ordered and chaotic Bohmian trajectories within the Born distribution of Bohmian particles of an anisotropic 2d quantum harmonic oscillator. We compute the average values of energy, momentum, angular momentum, and…
We predict the existence of high frequency modes in the interference pattern of two condensates made of fermionic-atom dimers. These modes, which result from fermion exchanges between condensates, constitute a striking signature of the…
We consider the interaction of gapped graphene in the two-band approximation using an explicit time-dependent approach. In addition to the full high-order harmonic generation (HHG) spectrum, we also obtain the perturbative harmonic response…
High order harmonic (HOH) generation by interacting extremely intense electromagnetic waves in the quantum vacuum is investigated within the framework of the Heisenberg-Euler formalism. We consider here the process in the lowest order of a…
The precise description of quantum nuclear fluctuations in atomistic modelling is possible by employing path integral techniques, which involve a considerable computational overhead due to the need of simulating multiple replicas of the…
Here the ionization and high harmonic generation in Hydrogen and Helium by using quantum (hydrodynamic) trajectories is analyzed theoretically. The quantum trajectories allow a self-contained treatment of the electron exchange and…
We investigate high-order harmonic spectra from aligned diatomic molecules in intense driving fields whose components have orthogonal polarizations. We focus on how the driving-field ellipticity influences structural interference patterns…