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Phase equilibria in the Al-Ti-Nb-Zr-Ta refractory complex concentrated alloy system were investigated using a high throughput experimental approach. A pseudo-ternary section of the quinary compositional space was prepared by a honeycomb…

While the high-entropy wind (HEW) of Type II supernovae remains one of the more promising sites for the rapid neutron-capture (r-) process, hydrodynamic simulations have yet to reproduce the astrophysical conditions under which the latter…

Solar and Stellar Astrophysics · Physics 2009-11-13 K. Farouqi , K. -L. Kratz , L. I. Mashonkina , B. Pfeiffer , J. J Cowan , F. -K. Thielemann , J. W. Truran

The prediction of new high entropy oxides (HEOs) remains a profound challenge due to their inherent chemical complexity. In this work, we combine experimental and computational methods to search for new HEOs in the tetravalent $A$O$_2$…

We use high-throughput first-principles sampling to investigate competitive factors that determine the crystal structure of high-entropy alloys (HEAs) and the energetics dependence of the stable phase on the atomic configuration of fully…

Materials Science · Physics 2022-01-03 Hiroshi Mizuseki , Ryoji Sahara , Kenta Hongo

Bare and surface-passivated Fe2N, Co2N, and Ni2N MXene were investigated by using density functional theory. Fe2N(OH)2, Fe2NO2, Co2NO2, Ni2NF2, Ni2N(OH)2, and Ni2NO2 are intrinsic half-metals, while other structures have antiferromagnetic…

Materials Science · Physics 2017-09-13 Guo Wang , Yi Liao

The alloying effect on the lattice parameters, isostructural mixing enthalpies and ductility of the ternary nitride systems Cr1-xTMxN (TM=Sc, Y; Ti, Zr, Hf; V, Nb, Ta; Mo, W) in the cubic B1 structure has been investigated using…

Materials Science · Physics 2014-07-10 Liangcai Zhou , David Holec , Paul. H. Mayrhofer

We perform density functional theory calculation to investigate the structural and electronic properties of various two-dimensional transition metal dichalcogenides, MX$_2$ (M$=$Ti, V, Cr, Zr, Nb, Mo, Hf, Ta, or W, and X$=$S or Se), and…

Materials Science · Physics 2019-05-21 Seoung-Hun Kang , Young-Kyun Kwon

We present a kinetic model for solid state phase transformation (alpha<-->beta) of common zirconium alloys used as fuel cladding material in light water reactors. The model computes the relative amounts of beta or alpha phase fraction as a…

Materials Science · Physics 2021-04-01 A. R. Massih , L. O. Jernkvist

The phase diagram of Al-Li-Cu system in the Al-rich region was determined by means of first-principles calculations and statistical mechanics. The mixing enthalpies of many configurations for different lattices in the whole Al-Li-Cu system…

Materials Science · Physics 2022-06-29 S. Liu , J. S. Wróbel , J. LLorca

We report on first-principles calculations of multilayers of zinc-blende half-metallic ferromagnets CrAs and CrSb with III-V and II-VI semiconductors, in the [001] orientation. We examine the ideal and tetragonalised structures, as well as…

Materials Science · Physics 2009-11-10 Ph. Mavropoulos , I. Galanakis , P. H. Dederichs

Contrary to prior calculations, the Ni-rich ordered structures of the Cr-Ni alloy system are found to be antiferromagnetic under semi-local density-functional theory. The optimization of local magnetic moments significantly increases the…

Materials Science · Physics 2023-08-23 Flynn Walsh , Robert O. Ritchie , Mark Asta

Motivated by the recent discovery of near-room temperature superconductivity in high-pressure superhydrides, we investigate from first-principles the high-pressure superconducting phase diagram of the ternary Ca-B-H system, using ab-initio…

Superconductivity · Physics 2020-08-26 Simone Di Cataldo , Wolfgang von der Linden , Lilia Boeri

In rare-earth permanent magnets (REPM's), trade-off's between intrinsic magnetic properties are often encountered. A recent example is SmFe$_{12}$ where excellent magnetic properties can be achieved at the sacrifice of bulk structure…

Materials Science · Physics 2020-06-22 Munehisa Matsumoto , Takafumi Hawai , Kanta Ono

Using the hybrid exchange-correlation functional within the density-functional theory, we have systematically investigated the structural and electronic properties of MO (M = Be, Mg, Ca, Sr, Ba, Zn, Cd) in binary rocksalt (B1), zincblende…

Materials Science · Physics 2019-03-19 Jinying Yu , Mingke Zhang , Zihan Zhang , Shangwei Wang , Yelong Wu

Hydrogen embrittlement in zirconium alloys is one of current challenges of nuclear reactor containment and can lead to a rapid decrease in mechanical properties of materials. Although many previous studies investigated the mechanism of…

Materials Science · Physics 2018-11-27 Heng-Yu Li , Hao-Jun Jia , Yan-Zhen Zhao , L. A. Svyatkin , I. P. Chernov

The multiple scattering-based theory of Gaspari and Gyorffy for the electron-ion matrix element in close packed metals is applied to Im-3m H3S, which has been predicted by Duan {\it et al.} and Bernstein {\it et al} to be the stable phase…

Superconductivity · Physics 2015-05-28 D. A. Papaconstantopoulos , B. M. Klein , M. J. Mehl , W. E. Pickett

We calculate the cohesive energies of Fe-based glass-forming alloys in the B-Fe-Y-Zr quaternary system. Our {\it ab-initio} calculations fully relax atomic positions and lattice parameters yielding enthalpies of mixing at T=0K. We examine…

Materials Science · Physics 2007-05-23 M. Mihalkovič , M. Widom

The effect of solute hydrogen on the stability of vacancy clusters in hexagonal closed packed zirconium is investigated with an ab initio approach, including contributions of H vibrations. Atomistic simulations within the density functional…

Materials Science · Physics 2015-09-29 Céline Varvenne , Olivier Mackain , Laurent Proville , Emmanuel Clouet

We perform an exhaustive theoretical study of the phase diagram of Cu-I binaries, focusing on Cu-poor compositions, relevant for p-type transparent conduction. We find that the interaction between neighboring Cu vacancies is the determining…

Using density-functional theory with ultrasoft pseudopotentials, we previously investigated the structural and electronic properties of the low-pressure (cubic, tetragonal, and monoclinic) phases of ZrO2 and HfO2, in order to elucidate…

Materials Science · Physics 2007-05-23 Xinyuan Zhao , David Vanderbilt