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The onset of structural arrest and glass formation in a concentrated suspension of silica nanoparticles in a water-lutidine binary mixture near its consolute point is studied by exploiting the near-critical fluid degrees of freedom to…

Soft Condensed Matter · Physics 2009-11-13 Xinhui Lu , S. G. J. Mochrie , S. Narayanan , A. R. Sandy , M. Sprung

We report observation of crystallization of the glass-forming binary Lennard-Jones liquid first used by Wahnstr\"om [G. Wahnstr\"om, Phys. Rev. A 44, 3752 (1991)]. Molecular dynamics simulations of the metastable liquid on a timescale of…

Materials Science · Physics 2007-06-12 Ulf R. Pedersen , Nicholas P. Bailey , Jeppe C. Dyre , Thomas B. Schrøder

We investigate a binary Lennard-Jones mixture with molecular dynamics simulations. We consider first a system cooled linearly in time with the cooling rate gamma. By varying gamma over almost four decades we study the influence of the…

Statistical Mechanics · Physics 2015-06-25 K. Vollmayr-Lee , W. Kob , K. Binder , A. Zippelius

Understanding the phase behaviour of mixtures continues to pose challenges, even for systems that might be considered "simple". Here we consider a very simple mixture of two colloidal and one non-adsorbing polymer species which can be…

It has been well established that particulate systems show the jamming transition and critical scaling behaviors associated with it. However, our knowledge is limited to (nearly) monodisperse systems. Recently, a binary mixture of jammed…

Soft Condensed Matter · Physics 2021-05-12 Yusuke Hara , Hideyuki Mizuno , Atsushi Ikeda

Polymers with both soluble and insoluble blocks typically self-assemble into micelles, aggregates of a finite number of polymers where the soluble blocks shield the insoluble ones from contact with the solvent. Upon increasing…

Soft Condensed Matter · Physics 2009-11-13 J. A. Anderson , C. D. Lorenz , A. Travesset

We use molecular dynamics simulation to study the relationship between structure and dynamics in supercooled binary Lennard--Jones nanoparticles over a range of particle sizes. The glass transition temperature of the nanoparticles is found…

Soft Condensed Matter · Physics 2025-05-15 Weikai Qi , Shreya Tiwary , Richard K. Bowles

Extending mode-coupling theory, we elaborate a microscopic theory for the glass transition of liquids confined between two parallel flat hard walls. The theory contains the standard MCT equations in bulk and in two dimensions as limiting…

Soft Condensed Matter · Physics 2010-09-15 Simon Lang , Vitalie Botan , Martin Oettel , David Hajnal , Thomas Franosch , Rolf Schilling

When strained beyond the linear regime, soft colloidal glasses yield to steady-state plastic flow in a way that is similar to the deformation of conventional amorphous solids. Due to the much larger size of the colloidal particles with…

Soft Condensed Matter · Physics 2017-04-12 Antina Ghosh , Zoe Budrikis , Vijayakumar Chikkadi , Alessandro Sellerio , Stefano Zapperi , Peter Schall

Binary Cu-Zr system is a representative bulk glassformer demonstrating high glass forming ability due to pronounced icosahedral local ordering. From the first glance, Ni-Zr system is the most natural object to expect the same behavior…

Disordered Systems and Neural Networks · Physics 2018-10-09 B. A. Klumov , R. E. Ryltsev , N. M. Chtchelkatchev

We simulate a strongly size-disperse hard-sphere fluid confined between two parallel, hard walls. We find that confinement induces crystallization into n-layered hexagonal lattices and a novel honeycomb-shaped structure, facilitated by…

Soft Condensed Matter · Physics 2020-08-12 Gerhard Jung , Charlotte F. Petersen

We report a molecular dynamics study of crystallization in highly asymmetric binary hard-sphere mixtures, in which the large spheres can form a crystal phase while the small ones remain disordered during the crystallization process of the…

Soft Condensed Matter · Physics 2015-05-28 Wen-Sheng Xu , Zhao-Yan Sun , Li-Jia An

Extensive molecular dynamics simulations show that a short-range central potential, suited to model C60, undergoes a high temperature transition to a glassy phase characterized by the positional disorder of the constituent particles.…

Soft Condensed Matter · Physics 2007-05-23 Maria C. Abramo , Carlo Caccamo , Dino Costa , Romina Ruberto

A binary system of particles that move in opposite directions under an applied field can exhibit disordered states as well as laned states where the particles organize into oppositely moving high-mobility lanes to reduce collisions.…

Soft Condensed Matter · Physics 2025-10-21 C. Reichhardt , C. J. O. Reichhardt

Multicomponent crystals are often assumed to form nearly random solid solutions when thermodynamically stable. However, crystal growth proceeds from structurally heterogeneous liquids, raising the possibility that the liquid state may…

Soft Condensed Matter · Physics 2026-03-30 Rikuya Ishikawa , Kyohei Takae , Daisuke Takegami , Yoshikazu Mizuguchi , Rei Kurita

Special role in computer simulations of supercooled liquid and glasses is played by few general models representing certain classes of real glass-forming systems. Recently, it was shown that one of the most widely used model glassformers --…

Materials Science · Physics 2018-11-14 R. E. Ryltsev , B. A. Klumov , N. M. Chtchelkatchev , K. Yu. Shunyaev

The binary Kob-Andersen (KA) Lennard-Jones mixture is the standard model for computational studies of viscous liquids and the glass transition. For very long simulations the viscous KA system crystallizes, however, by phase separating into…

Soft Condensed Matter · Physics 2018-04-24 Ulf R. Pedersen , Thomas B. Schrøder , Jeppe C. Dyre

The stability of a quasicrystalline structure, recently obtained in a molecular-dynamics simulation of rapid cooling of a binary melt, is analyzed for binary hard-sphere mixtures within a density-functional approach. It is found that this…

Materials Science · Physics 2017-02-08 H. M. Cataldo

We study the interplay between the fluid-crystal transition and the glass transition of elastic sphere system with polydispersity using nonequilibrium molecular dynamics simulations. It is found that the end point of the crystal-fluid…

Statistical Mechanics · Physics 2010-09-29 Tomoaki Nogawa , Nobuyasu Ito , Hiroshi Watanabe

The dynamics of glass formation in monatomic and binary liquids are studied numerically using a microscopic field theory for the evolution of the time-averaged atomic number density. A stochastic framework combining phase field crystal free…

Materials Science · Physics 2015-05-27 Joel Berry , Martin Grant
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