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We simulate binary soft disk systems in two dimensions, and investigate how the dynamics slow as the area fraction is increased toward the glass transition. The "fragility" quantifies how sensitively the relaxation time scale depends on the…

Soft Condensed Matter · Physics 2010-10-12 Rei Kurita , Eric R. Weeks

We present a theory for the dynamics of a binary mixture with particle size swaps. The theory is based on a factorization approximation similar to that employed in the mode-coupling theory of glassy dynamics. The theory shows that, in…

Soft Condensed Matter · Physics 2018-11-14 Grzegorz Szamel

Polymer blends offer an exciting material for various potential applications due to their tunable properties by varying constituting components and their relative composition. Our simulation results unravel an intrinsic relationship between…

Soft Condensed Matter · Physics 2016-10-13 Ashok Kumar Dasmahapatra

Structural relaxation in binary hard spherical particles has been shown recently to exhibit a wealth of remarkable features when size disparity or mixture's composition is varied. In this paper, we test whether or not similar dynamical…

Soft Condensed Matter · Physics 2014-12-03 Wen-Sheng Xu , Zhao-Yan Sun , Li-Jia An

The binary hard-sphere mixture is one of the simplest representations of a many-body system with competing time and length scales. This model is relevant to fundamentally understand both the structural and dynamical properties of materials,…

This paper shows by computer simulations that some crystalline systems have curves in their thermodynamic phase diagrams, so-called isomorphs, along which structure and dynamics in reduced units are invariant to a good approximation. The…

Statistical Mechanics · Physics 2024-01-17 Dan E. Albrechtsen , Andreas E. Olsen , Ulf R. Pedersen , Thomas B. Schrøder , Jeppe C. Dyre

We present an event-driven molecular dynamics study of glass formation in two-dimensional binary mixtures composed of hard disks and hard ellipses, where both types of particles have the same area. We demonstrate that characteristic…

Soft Condensed Matter · Physics 2015-05-27 Wen-Sheng Xu , Xiaozheng Duan , Zhao-Yan Sun , Li-Jia An

Multiple distinct glass states occur in binary hard-sphere mixtures with constituents of very disparate sizes according to the mode-coupling theory of the glass transition (MCT), distinguished by considering whether small particles remain…

Soft Condensed Matter · Physics 2015-05-20 Th. Voigtmann

We perform molecular dynamics (MD) simulations of the crystallization process in binary Lennard-Jones systems during heating and cooling to investigate atomic-scale crystallization kinetics in glass-forming materials. For the cooling…

Soft Condensed Matter · Physics 2015-06-23 Minglei Wang , Kai Zhang , Zhusong Li , Yanhui Liu , Jan Schroers , Mark D. Shattuck , Corey S. O'Hern

Bulk metallic glass forms when liquid metal alloys solidify without crystalization. In the search for Iron-based bulk glass-forming alloys of the metal-metalloid type (Fe-B- and Fe-C-based), crystals based on the structural prototype C6Cr23…

Materials Science · Physics 2009-11-10 M. Widom , M. Mihalkovic

We investigate mixing effects on the glass state of binary colloidal hard-sphere-like mixtures with large size asymmetry, at a constant volume fraction phi = 0.61. The structure, dynamics and viscoelastic response as a function of mixing…

Soft Condensed Matter · Physics 2015-06-12 Tatjana Sentjabrskaja , Donald Guu , M Paul Lettinga , Stefan U Egelhaaf , Marco Laurati

The freezing mechanism, recently suggested for a monodisperse hard-disk fluid [Huerta et al., Phys. Rev. E, 2006, 74, 061106] is extended here to an equimolar binary hard-disk mixtures. We are showing that for diameter ratios, smaller than…

Soft Condensed Matter · Physics 2013-01-01 A. Huerta , V. Carrasco-Fadanelli , A. Trokhymchuk

We study structural transitions in a system of interacting particles arranged as a crystalline bilayer, as a function of the density $\rho$ and the distance $d$ between the layers. As $d$ is decreased a sequence of transitions involving…

Soft Condensed Matter · Physics 2015-05-13 Tamoghna Das , Surajit Sengupta , Subhasis Sinha

We systematically study the relationship between equilibrium and non-equilibrium phase diagrams of a system of short-ranged attractive colloids. Using Monte Carlo and Brownian dynamics simulations we find a window of enhanced…

Soft Condensed Matter · Physics 2009-11-13 Andrea Fortini , Eduardo Sanz , Marjolein Dijkstra

The glass transition in binary mixtures of star polymers is studied by mode coupling theory and extensive molecular dynamics computer simulations. In particular, we have explored vitrification in the parameter space of size asymmetry…

The behavior of identical particles interacting through the harmonic-repulsive pair potential has been studied in 3D using molecular dynamics simulations at a number of different densities. We found that at many densities, as the…

Soft Condensed Matter · Physics 2017-10-11 V. A. Levashov

We study glass transitions in mixtures of elliptic and circular particles in two dimensions using an orientation-dependent Lennard-Jones potential. Changing anisotropic parameters of the potential, the size ratio, and the concentration, we…

Soft Condensed Matter · Physics 2013-05-21 Kyohei Takae , Akira Onuki

Our earlier Monte Carlo simulations of metastable supercooled-liquid and glass phases of Lennard-Jones atoms found several distinct signatures for identifying the glass transition boundary; i.e., the density, enthalpy, and pair distribution…

Materials Science · Physics 2015-05-05 Farid F. Abraham

In this paper, we report dynamic Monte Carlo simulation results on the crystallization of crystalline/crystalline (A/B) symmetric binary polymer blend, wherein the melting temperature of A-polymer is higher than B-polymer. Crystallization…

Soft Condensed Matter · Physics 2015-06-18 Ashok Kumar Dasmahapatra

Colloidal crystals formed by size-asymmetric binary particles co-assemble into a wide variety of colloidal compounds with lattices akin to ionic crystals. Recently, a transition from a compound phase with a sublattice of small particles to…

Soft Condensed Matter · Physics 2023-09-12 Ali Ehlen , Hector Lopez-Rios , Monica Olvera de la Cruz