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We study the surface plasmon (SP) resonance energy of isolated spherical Ag nanoparticles dispersed on a silicon nitride substrate in the diameter range 3.5-26 nm with monochromated electron energy-loss spectroscopy. A significant blueshift…

Raza et al. recently observed the extraordinarily large energy blueshifts of localized surface plasmon resonances and additional surface plasmon resonances in silver nanoparticles encapsulated in silicon nitride, which are not fully…

Mesoscale and Nanoscale Physics · Physics 2021-05-19 Guozhong Wang

According to the hydrodynamic Drude model, surface-plasmon resonances of metallic nanostructures blueshift owing to the nonlocal response of the metal's electron gas. The screening length characterising the nonlocal effect is often small…

In electron energy-loss spectroscopy (EELS) of individual silver nanoparticles encapsulated in silicon nitride, we observe besides the usual dipole resonance an additional surface plasmon (SP) resonance corresponding to higher angular…

Localized surface plasmons (LSP) in semiconductor particles are expected to exhibit spatial nonlocal response effects as the geometry enters the nanometer scale. To investigate these nonlocal effects, we apply the hydrodynamic model to…

Mesoscale and Nanoscale Physics · Physics 2017-09-13 J. R. Maack , N. A. Mortensen , M. Wubs

Damping rates of multipolar, localized surface plasmons (SP) of gold and silver nanospheres of radii up to $1000nm$ were found with the tools of classical electrodynamics. The significant increase in damping rates followed by noteworthy…

Optics · Physics 2012-11-21 Krystyna Kolwas , Anastasiya Derkachova

Clear influence of particle size, surfactants and dispersion medium on surface plasmon resonance (SPR) features of Ag nanoparticles (NPs), synthesized in thermal decomposition method, in the broad range of ultraviolet (UV) radiation,…

Applied Physics · Physics 2020-01-29 Vikash Sharma , Divya Verma , Gunadhor Singh Okram

We have investigated the effects of tuning the localized surface plasmon resonances (LSPRs) of silver nanoparticles on the fluorescence intensity, lifetime, and Raman signal from nearby fluorophores. The presence of a metallic structure can…

Other Condensed Matter · Physics 2009-11-13 N. I. Cade , T. Ritman-Meer , D. Richards

Non-local effects in the optical response of noble metals are shown to produce significant blueshift and near-field quenching of plasmons in nanoparticle dimers, nanoshells, and thin metal waveguides. Compared with a local description…

Other Condensed Matter · Physics 2012-11-13 F. Javier Garcia de Abajo

Particle plasmons in metal nanoparticles have primarily been investigated through the use of local optical response approximations. However, as nanoparticle size approaches the average distance of electrons to the metal surface, mesoscopic…

Optics · Physics 2023-06-28 Weixiang Ye

The electronic environment causes decoherence and dissipation of the collective surface plasmon excitation in metallic nanoparticles. We show that the coupling to the electronic environment influences the width and the position of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Guillaume Weick , Gert-Ludwig Ingold , Rodolfo A. Jalabert , Dietmar Weinmann

We have observed the compensation of loss in metal by gain in interfacing dielectric in the mixture of aggregated silver nanoparticles and rhodamine 6G dye. The demonstrated six-fold enhancement of the Rayleigh scattering is the evidence of…

Inspired by recent measurements on individual metallic nanospheres that can not be explained with traditional classical electrodynamics, we theoretically investigate the effects of nonlocal response by metallic nanospheres in three distinct…

Mesoscale and Nanoscale Physics · Physics 2014-03-07 Thomas Christensen , Wei Yan , Søren Raza , Antti-Pekka Jauho , N. Asger Mortensen , Martijn Wubs

We develop a theoretical model of the surface plasmon resonance of metallic nanospheres in the size range down to the single nanometer size. Within this model we explicitly show how different microscopic mechanisms, namely quantization due…

Optics · Physics 2013-08-26 R. Carmina Monreal , Tomasz J. Antosiewicz , S. Peter Apell

We consider scattering of surface plasmon polaritons (SPPs) and light by individual high-refractive-index dielectric nanoparticles (NPs) located on a metal (gold) substrate and supporting electric and magnetic dipole resonances in the…

Mesoscale and Nanoscale Physics · Physics 2016-09-21 Andrey B. Evlyukhin , Sergey I. Bozhevolnyi

Nanometer-sized metal particles exhibit broadening of the localized surface plasmon resonance (LSPR) in comparison to its value predicted by the classical Mie theory. Using our model for the LSPR dependence on non-local surface screening…

Optics · Physics 2015-06-22 R. Carmina Monreal , S. Peter Apell , Tomasz J. Antosiewicz

Two possible mechanisms of surface plasmon (SP) oscillations damping in metallic nanoparticles (MNPs), not connected with electron-phonon interaction are investigated theoretically: a) the radiation damping of SP, b) resonant coupling of SP…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Armen Melikyan , Hayk Minassian

We present an electron energy loss study using energy filtered TEM of spatially resolved surface plasmon excitations on a silver nanorod of aspect ratio 14.2 resting on a 30 nm thick silicon nitride membrane. Our results show that the…

Absorption efficiency profiles and localized surface plasmon resonance (LSPR) wavelengths are reported for metallic core-shell nanoparticles (NPs) placed over a BK7 glass substrate. A numerical study is performed with the vectorized version…

Optics · Physics 2020-01-08 Dilan Avsar , Hakan Erturk , M. Pinar Menguc

We report a novel behavior of the surface plasmon linewidth in sodium nanospheres Na$_{1760}$ changing with the electron temperature, which monotonically decreases and bears a discontinuous sudden drop at high electron temperatures. Our…

Mesoscale and Nanoscale Physics · Physics 2014-08-15 Guozhong Wang , Yizhuang Zheng , Jian Zi
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