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We report on accurate variational calculations of the Born-Oppenheimer potential for excited states of the hydrogen molecule with $\Pi$, $\Delta$, and $\Phi$ symmetries. The obtained potential energy curves reach the relative precision of…

Atomic Physics · Physics 2023-01-11 Michał Siłkowski , Krzysztof Pachucki

We report on highly accurate calculations of Born-Oppenheimer potentials for excited $n\,\Sigma^{+}$ states of the hydrogen molecule for all possible combinations of singlet/triplet and gerade/ungerade symmetries up to $n=7$. A relative…

Atomic Physics · Physics 2023-02-28 Michał Siłkowski , Magdalena Zientkiewicz , Krzysztof Pachucki

Adopting explicitly correlated Kolos-Wolniewicz-type basis functions, the Born-Oppenheimer potential curves of a number of excited $\Sigma$ states of the hydrogen-antihydrogen system ($\bar{\rm H}$) were calculated for both, even and odd, Q…

Atomic Physics · Physics 2025-11-12 L. Brumm , J. Schürmann , A. Saenz

Various properties of the general two-center two-electron integral over the explicitly correlated exponential function are analyzed for the potential use in high precision calculations for diatomic molecules. A compact one dimensional…

Chemical Physics · Physics 2015-06-11 Krzysztof Pachucki

The Born-Oppenheimer potential for the $^1\Sigma_g^+$ state of H$_2$ is obtained in the range of 0.1 -- 20 au, using analytic formulas and recursion relations for two-center two-electron integrals with exponential functions. For small…

Chemical Physics · Physics 2015-05-19 Krzysztof Pachucki

We present an efficient approach to evaluate two-center two-electron integrals with exponential functions and with an arbitrary polynomial in electron-nucleus and electron-electron distances. We show that the master integral with the single…

Chemical Physics · Physics 2009-09-29 Krzysztof Pachucki

For rovibronic states corresponding to the $B$ and $B'\ ^1\Sigma_\text{u}^+$ electronic states of the hydrogen molecule, the pre-Born--Oppenheimer (four-particle) non-relativistic energy is converged to a 1-3 parts-per-billion relative…

Chemical Physics · Physics 2023-01-10 Eszter Saly , Dávid Ferenc , Edit Mátyus

The difference of the values of observables for the time-independent Schroedinger equation, with matrix valued potentials, and the values of observables for ab initio Born-Oppenheimer molecular dynamics, of the ground state, depends on the…

Numerical Analysis · Mathematics 2015-05-13 Christian Bayer , Hakon Hoel , Ashraful Kadir , Petr Plechac , Mattias Sandberg , Anders Szepessy

Baryons containing two heavy quarks are treated in the Born-Oppenheimer approximation. Schr\"odinger equation for two center Coulomb plus harmonic oscillator potential is solved by the method of ethalon equation at large intercenter…

High Energy Physics - Phenomenology · Physics 2009-10-31 D. U. Matrasulov , M. M. Musakhanov , T. Morii

We perform a calculation of quantum electrodynamics effects in excited states with $l>1$ of arbitrary two-body systems up to $\alpha^6\,\mu$ order. The obtained results are valid for hadronic atoms, as long as the strong interaction effects…

Atomic Physics · Physics 2022-10-19 Jacek Zatorski , Vojtěch Patkóš , Krzysztof Pachucki

We present a new first-principles formalism for calculating forces for optically excited electronic states using the interacting Green's function approach with the GW-Bethe Salpeter Equation method. This advance allows for efficient…

Materials Science · Physics 2013-05-29 Sohrab Ismail-Beigi Steven G. Louie

Total cross sections for single ionization and excitation of molecular hydrogen by antiproton impact are presented over a wide range of impact energy from 1 keV to 6.5 MeV. A nonpertubative time-dependent close-coupling method is applied to…

Atomic Physics · Physics 2015-05-14 Armin Lühr , Alejandro Saenz

The processes of electron excitation, capture, and ionization were investigated in proton collisions with atomic hydrogen in the initial $n=1$ and $n=2$ states at impact energies from 1 to 300 keV. The theoretical analysis is based on the…

Atomic Physics · Physics 2019-12-10 Anthony C. K. Leung , Tom Kirchner

The calculation of molecular excited states is critically important to decipher a plethora of molecular properties. In this manuscript, we develop an equation of motion formalism on top of a bi-exponentially parametrized ground state…

Chemical Physics · Physics 2024-01-09 Anish Chakraborty , Pradipta Kumar Samanta , Rahul Maitra

In this paper we report calculations of potential energy curves in the $1.2 a.u.\le R\le100 a.u.$ range at Multireference Configuration Interaction (MRCI) level for doubly excited states of the H$_2$ molecule. We have focused on the $Q_2$…

The essence of atomic structure theory, quantum chemistry, and computational materials science is solving the multi-electron stationary Schr\"odinger equation. The Quantum Monte Carlo-based neural network wave function method has surpassed…

Atomic Physics · Physics 2023-12-27 JinDe Liu , Chenglong Qin , Xi He , Gang Jiang

Three-centre nuclear attraction integrals, which arise in density functional and \textit{ab initio} calculations, are one of the most time-consuming computations involved in molecular electronic structure calculations. Even for relatively…

Numerical Analysis · Mathematics 2024-12-20 Jordan Lovrod , Hassan Safouhi

Three simple $7-, (7+3)-, 10-$parametric trial functions for the ${\rm H}_3^+$ molecular ion are presented. Each of them provides subsequently the most accurate approximation for the Born-Oppenheimer ground state energy among…

Quantum Physics · Physics 2015-05-28 J. C. Lopez Vieyra , A. V. Turbiner , H. Medel Cobaxin

The two-center two-electron Coulomb and hybrid integrals arising in relativistic and nonrelativistic ab-initio calculations of molecules are evaluated over the non-integer Slater-type orbitals via ellipsoidal coordinates. These integrals…

Quantum Physics · Physics 2014-05-22 Ali Bağcı , Philip E. Hoggan

We calculate the energies of ground and three low lying excited states of confined helium atom centered in an impenetrable spherical box. We perform the calculation by employing variational method with two-parameter variational forms for…

Atomic Physics · Physics 2009-11-11 Arup Banerjee , C. Kamal , Avijit Chowdhury
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