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In this technical review we give an introduction to optical spectroscopy for layered materials as a powerful, non-invasive tool to access details of the electronic band structure and crystal quality. Potential applications in photonics and…

Materials Science · Physics 2020-12-18 Shivangi Shree , Ioannis Paradisanos , Xavier Marie , Cedric Robert , Bernhard Urbaszek

Advances in micro-technology of the last years have made it possible to carry optics textbooks experiments over to atomic and molecular beams, such as diffraction by a double slit or transmission grating. The usual wave-optical approach…

Quantum Physics · Physics 2017-08-23 Gerhard C. Hegerfeldt , Thorsten Koehler

The evolution of both information and energy technology is intimately connected to complex condensed matter systems, the properties of which are determined by electronic and chemical interactions and processes on a broad range of length and…

Materials Science · Physics 2015-03-19 Martina Müller , Slavomir Nemsak , Lukasz Plucinski , Claus M. Schneider

The interpretation of the electronic kinetic processes in the quantum zero dimensional nanostructures is considered. The main mechanism of the processes is supposed to be the interaction of electrons with the optical phonons. An emphasis is…

Mesoscale and Nanoscale Physics · Physics 2012-01-05 K. Kral , M. Mensik

Quantum beats in nonlinear spectroscopy of molecular aggregates are often attributed to electronic phenomena of excitonic systems, while nuclear degrees of freedom are commonly included into models as overdamped oscillations of bath…

Chemical Physics · Physics 2012-11-27 Vytautas Butkus , Leonas Valkunas , Darius Abramavicius

To advance hierarchial equations of motion as a standard theory for quantum dissipative dynamics, we put forward a mixed Heisenberg--Schrodinger scheme with block-matrix implementation on efficient evaluation of nonlinear optical response…

Chemical Physics · Physics 2015-05-30 Jian Xu , Rui-Xue Xu , Darius Abramavicius , Houdao Zhang , YiJing Yan

The dynamics of excitonic energy transfer in molecular complexes triggered by interaction with laser pulses offers a unique window into the underlying physical processes. The absorbed energy moves through the network of interlinked pigments…

Quantum Physics · Physics 2025-12-30 Tobias Kramer

Conventional nonlinear spectroscopy uses classical light to detect matter properties through the variation of its response with frequencies or time delays. Quantum light opens up new avenues for spectroscopy by utilizing parameters of the…

Quantum Physics · Physics 2017-02-01 Konstantin E. Dorfman , Frank Schlawin , Shaul Mukamel

Two-dimensional (2D) spectroscopy combines high temporal and spectral resolution, allowing the observation of ultrafast energy transfer and the separation of homogeneous and inhomogeneous broadening. Typically, 2D spectroscopy is dominated…

Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…

Chemical Physics · Physics 2026-04-21 Yuta Fujihashi , Ozora Iso , Ryosuke Shimizu , Akihito Ishizaki

Quantum opto- and electromechanical systems interface mechanical motion with the electromagnetic modes of optical resonators and microwave circuits. The capabilities and promise of these hybrid devices have been showcased through a variety…

Quantum Physics · Physics 2025-08-20 Yiwen Chu , Simon Gröblacher

Two- and multi-dimensional spectroscopy is used in physics and chemistry to obtain structural and dynamical information that would otherwise be invisible by the projection into a one-dimensional data set such as a single emission or…

Entangled two-photon spectroscopy is expected to provide advantages compared with classical protocols. It is achieved by coherently controlling the spectral properties of energy-entangled photons. We present here an experimental setup that…

Quantum Physics · Physics 2021-08-25 Stefan Lerch , André Stefanov

Here we review some of the recent developments in Quantum Optics. After a brief introduction to the historical development of the subject, we discuss some of the modern aspects of quantum optics including atom field interactions, quantum…

Quantum Physics · Physics 2019-02-25 Subhashish Banerjee , Arun Jayannavar

Strong light-matter interactions enabled by surface plasmons have given rise to a wide range of photonic, optoelectronic and chemical functionalities. In recent years, the interest in this research area has focused on the quantum regime,…

Until very recently, two-photon interaction processes have been considered only as arising from second- or higher-order effects in driven systems, and so limited to extremely small coupling strengths. However, a variety of novel physical…

Quantum Physics · Physics 2019-07-25 Simone Felicetti , Alexandre Le Boité

The modes of the electromagnetic field are solutions of Maxwell's equations taking into account the material boundary conditions. The field modes of classical optics - properly normalized - are also the mode functions of quantum optics.…

Quantum Physics · Physics 2014-11-27 Birgit Stiller , Ulrich Seyfarth , Gerd Leuchs

The photophysics of $\pi$-conjugated polymers has been of considerable interest over the last three decades because of their organic semiconductor properties. Primary photoexcitations, Frenkel excitons, can be probed optically by means of…

Techniques in time- and angle-resolved photoemission spectroscopy have facilitated a number of recent advances in the study of quantum materials. We review developments in this field related to the study of incoherent nonequilibrium…

Strongly Correlated Electrons · Physics 2016-10-04 Christopher L. Smallwood , Robert A. Kaindl , Alessandra Lanzara

The goal of this research is to determine and study a physical system that will enable a fast and intrinsically two-photon detector, which would be of interest for quantum information and metrology applications. We consider two types of…

Quantum Physics · Physics 2009-11-07 Dmitry V. Strekalov , Matt Stowe , Maria V. Chekhova , Jonathan P. Dowling