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Phase equilibria between regions of different thickness in thin liquid films stabilized by colloidal particles are investigated using a quasi-two-dimensional thermodynamic formalism. Appropriate equilibrium conditions for the film tension,…

Soft Condensed Matter · Physics 2009-11-11 J. Blawzdziewicz , E. Wajnryb

Patterns are quotidian in nature. Distinct multiscale patterns are generally a consequence of nonequilibrium dynamical processes associated with mechanical or hydrodynamic instabilities. In this thesis, I report experimental investigations…

Soft Condensed Matter · Physics 2019-05-30 Xiaolei Ma

The order-disorder transition of a sphere-forming block copolymer thin film was numerically studied through a Cahn-Hilliard model. Simulations show that the fundamental mechanisms of pattern formation are spinodal decomposition and…

Soft Condensed Matter · Physics 2017-08-28 Leopoldo R. Gómez , Nicolás A. García , Richard A. Register , Daniel A. Vega

The melting of ultrathin lubricant film by friction between atomically flat surfaces is studied. The additive noises of the elastic shear stress and strain, and the temperature are introduced for building a phase diagram with the domains of…

Statistical Mechanics · Physics 2009-11-10 Alexei V. Khomenko

Short time existence for a surface diffusion evolution equation with curvature regularization is proved in the context of epitaxially strained three-dimensional films. This is achieved by implementing a minimizing movement scheme, which is…

Analysis of PDEs · Mathematics 2016-01-20 Irene Fonseca , Nicola Fusco , Giovanni Leoni , Massimiliano Morini

A number of recent experiments have showed that surfactants can modify the growth mode of an epitaxial film, suppressing islanding and promoting layer-by-layer growth. Here a set of coupled equations are introduced to describe the coupling…

Condensed Matter · Physics 2016-11-03 Albert-Laszlo Barabasi

Recent experiments have shown that various structures may be formed during the evaporative dewetting of thin films of colloidal suspensions. Nano-particle deposits of strongly branched `flower-like', labyrinthine and network structures are…

Soft Condensed Matter · Physics 2011-10-03 M. J. Robbins , A. J. Archer , U. Thiele

This study reveals the influence of the surface energy and solid/liquid boundary condition on the breakup mechanism of dewetting ultra-thin polymer films. Using silane self-assembled monolayers, SiO$_2$ substrates are rendered hydrophobic…

Soft Condensed Matter · Physics 2017-05-03 Matthias Lessel , Joshua D. McGraw , Oliver Bäumchen , Karin Jacobs

Growth-induced instabilities are ubiquitous in biological systems and lead to diverse morphologies in the form of wrinkling, folding, and creasing. The current work focusses on the mechanics behind growth-induced wrinkling instabilities in…

Pattern Formation and Solitons · Physics 2022-06-28 Sumit Mehta , Gangadharan Raju , Prashant Saxena

Organisms in nature can alter the short-range order of an amorphous precursor phase, thereby controlling the resulting crystalline structure. This phenomenon inspired an investigation of the effect of modifying the short-range order within…

Materials Science · Physics 2020-01-13 Yael Etinger-Geller , Alex Katsman , Boaz Pokroy

Using three-dimensional numerical simulations, we demonstrate the growth saturation of an unstable thin liquid film on micropatterned hydrophilic-hydrophobic substrates. We consider different transverse-striped micropatterns, characterized…

Soft Condensed Matter · Physics 2011-10-26 Rodrigo Ledesma-Aguilar , Aurora Hernandez-Machado , Ignacio Pagonabarraga

-- A scientific hurdle in manufacturing solid films by drying colloidal layers is preventing them from fracturing. This paper examines how the drying rate of colloidal liquids influences the particle packing at the nanoscale in correlation…

Soft Condensed Matter · Physics 2016-02-29 Keyvan Piroird , Véronique Lazarus , Georges Gauthier , Arnaud Lesaine , Daniel Bonamy , Cindy Rountree

We report an experimental study on the dynamics of a thin film of polymer solution coating a vertical fiber. The liquid film has first a constant thickness and then undergoes the Rayleigh-Plateau instability which leads to the formation of…

Fluid Dynamics · Physics 2013-05-21 François Boulogne , Ludovic Pauchard , Frédérique Giorgiutti-Dauphiné

Liquids in contact with solids are submitted to intermolecular forces making liquids heterogeneous and, in a mechanical model, the stress tensor is not any more spherical as in homogeneous bulks. The aim of this article is to show that a…

Soft Condensed Matter · Physics 2009-04-14 Henri Gouin

In the present contribution we review basic mathematical results for three physical systems involving self-organising solid or liquid films at solid surfaces. The films may undergo a structuring process by dewetting,…

Other Condensed Matter · Physics 2010-10-15 Uwe Thiele

Liquid films coating vertical cylinders can form annular liquid collars which translate downwards under gravity. We investigate the dynamics of a thin viscoplastic liquid film coating the interior or exterior of a vertical cylindrical tube,…

We investigate numerically the role of spatial arrangement of the patches on the irreversible adsorption of patchy colloids on a substrate. We consider spherical three-patch colloids and study the dependence of the kinetics on the opening…

Soft Condensed Matter · Physics 2014-10-01 C. S. Dias , N. A. M. Araújo , M. M. Telo da Gama

The ability to synthesize and control two-dimensional (2D) crystals creates numerous opportunities for studying emergent states of matter and their novel functionalities. Freestanding films provide a particularly versatile platform for…

Materials Science · Physics 2024-02-13 Yifan Su , Alfred Zong , Anshul Kogar , Di Lu , Seung Sae Hong , Byron Freelon , Timm Rohwer , Harold Y. Hwang , Nuh Gedik

We study the ultrafast structural dynamics, in response to electronic excitations, in heterostructures composed of Au$_{923}$ nanoclusters on thin-film substrates with the use of femtosecond electron diffraction. Various forms of atomic…

Recent experiments of thin films flowing down a vertical fiber with varying nozzle diameters present a wealth of new dynamics that illustrate the need for more advanced theory. We present a detailed analysis using a full lubrication model…

Fluid Dynamics · Physics 2019-01-03 H. Ji , C. Falcon , A. Sadeghpour , Z. Zeng , Y. S. Ju , A. L. Bertozzi