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Phenomena involving electron transfer are ubiquitous in nature, photosynthesis and enzymes or protein activity being prominent examples. Their deep understanding thus represents a mandatory scientific goal. Moreover, controlling the…

Chemical Physics · Physics 2017-12-01 Carlo Andrea Rozzi , Filippo Troiani , Ivano Tavernelli

Nanoscale molecular-electronic devices and machines are emerging as promising functional elements, naturally flexible and efficient, for next generation technologies. A deeper understanding of carrier dynamics in molecular junctions is…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 K. Beltako , F. Michelini , N. Cavassilas , L. Raymond

Photosystem II (PSII) reaction center is a unique protein-chromophore complex that is capable of efficiently separating electronic charges across the membrane after photoexcitation. In the PSII reaction center, the primary energy- and…

For efficient photovoltaic conversion, it is important to understand how quantum entropy-related quantities evolve during the photovoltaic process. In this study, using a double quantum dot (DQD) photocell model, we explored the dynamic…

Mesoscale and Nanoscale Physics · Physics 2024-02-13 Lin-Jie Chen , Shun-Cai Zhao , Ya-Fang Tian

The theoretical and experimental study of energy transfer in photosynthesis has revealed an interesting transport regime, which lies at the borderline between classical transport dynamics and quantum-mechanical interference effects.…

Biological Physics · Physics 2014-02-13 Tobias Kramer , Christoph Kreisbeck

Generations of technologies with fundamentally new information processing capabilities will emerge if microscopic physical systems can be controlled to encode, transmit, and process quantum information, at scale and with high fidelity. In…

Quantum Physics · Physics 2020-05-06 Jianwei Wang , Fabio Sciarrino , Anthony Laing , Mark G. Thompson

Topological photonics is a rapidly emerging field of research in which geometrical and topological ideas are exploited to design and control the behavior of light. Drawing inspiration from the discovery of the quantum Hall effects and…

Recent evidence suggests that quantum effects may have functional importance in biological light-harvesting systems. Along with delocalized electronic excitations, it is now suspected that quantum coherent interactions with certain…

Chemical Physics · Physics 2015-10-22 Nathan Killoran , Susana F. Huelga , Martin B. Plenio

Natural and artificial light harvesting systems often operate in a regime where the flux of photons is relatively low. Besides absorbing as many photons as possible it is therefore paramount to prevent excitons from annihilation via photon…

Quantum Physics · Physics 2017-10-24 K. D. B. Higgins , B. W. Lovett , E. M. Gauger

There is a remarkable characteristic of photosynthesis in nature, that is, the energy transfer efficiency is close to 100%. Recently, due to the rapid progress made in the experimental techniques, quantum coherent effects have been…

Chemical Physics · Physics 2020-02-25 Ming-Jie Tao , Na-Na Zhang , Peng-Yu Wen , Fu-Guo Deng , Qing Ai , Gui-Lu Long

One of the important nonclassical effects in quantum optics is the anti-bunching, which has been observed in a large class of physical systems - including light-harvesting antennas with cyclic structures. The units of the ring couple with…

Chemical Physics · Physics 2017-03-09 Hui Dong , Sheng-Wen Li , Zhenhuan Yi , Girish S. Agarwal , Marlan O. Scully

Many advanced concepts for high-efficiency photovoltaic devices exploit the peculiar optoelectronic properties of semiconductor nanostructures such as quantum wells, wires and dots. While the optics of such devices is only modestly affected…

Mesoscale and Nanoscale Physics · Physics 2014-11-17 Urs Aeberhard

We report on the fabrication of two-dimensional periodic photonic nanostructures by nanoimprint lithography and dry etching, and their integration into a 1-{\mu}m-thin mono-crystalline silicon solar cell. Thanks to the periodic…

Mesoscale and Nanoscale Physics · Physics 2012-12-17 Christos Trompoukis , Ounsi El Daif , Valérie Depauw , Ivan Gordon , Jef Poortmans

Single photons constitute a main platform in quantum science and technology: they carry quantum information over extended distances in the future quantum internet and can be manipulated in advanced photonic circuits enabling scalable…

Recent developments in nanoscale experimental techniques made it possible to utilize single molecule junctions as devices for electronics and energy transfer with quantum coherence playing an important role in their thermoelectric…

Mesoscale and Nanoscale Physics · Physics 2018-03-12 Feng Chen , Yi Gao , Michael Galperin

Photon-mediated dipole-dipole interactions arise from atom-light interactions, which are universal and prevalent in a wide range of open quantum systems. This pairwise and long-range spin-exchange interaction results from multiple light…

Quantum Physics · Physics 2025-03-11 H. H. Jen

Obtaining the physical mechanism of photoelectric transfer in quantum-dot (QD) photocells may be one strategy to boost the photovoltaic conversion efficiency. In this work, we attempted to formulate a novel theoretical approach to evaluate…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Sheng-Nan Zhu , Shun-Cai Zhao , Lin-Jie Chen

The efficiency of photo-conductive switches, which continue to be used for the generation and detection of THz waves, has been overlooked for a long time. The so far 'optics-dominated' devices are making their way through to new and…

Applied Physics · Physics 2020-11-10 Giorgos Georgiou , Clément Geffroy , Christopher Bäuerle , Jean-François Roux

Micro/nanoscale single photon source is a building block of on-chip quantum information devices. Owing to possessing ultrasmall optical mode volume, plasmon structures can provide large Purcell enhancement, however scattering and absorption…

Optics · Physics 2021-01-20 Zhiyuan Qian , Zhichao Li , He Hao , Lingxiao Shan , Qihuang Gong , Ying Gu

In this paper we consider dynamics of a molecular system subjected to external pumping by a light source. Within a completely quantum mechanical treatment, we derive a general formula, which enables to asses effects of different light…

Biological Physics · Physics 2012-01-30 Tomas Mancal , Leonas Valkunas