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The photon-ion merged-beams technique for the photoionization of mass/charge selected ionized atoms, molecules and clusters by x-rays from synchrotron radiation sources is introduced. Examples for photoionization of atomic ions are…

Atomic Physics · Physics 2017-02-22 S. Schippers , A. L. D. Kilcoyne , R. A. Phaneuf , A. Müller

The ionization of an atom by a high-frequency intense laser pulse, where the energy of a single-photon is sufficient to ionize the system, is investigated from first principles. It is shown that as a consequence of an AC Stark effect in the…

Atomic Physics · Physics 2012-06-26 Philipp V Demekhin , Lorenz S Cederbaum

Correctness of the model representing the fullerene shell C60 as a conducting sphere has been analyzed. The static and dynamical polarizabilities of the molecule C60 have been calculated on the basis of experimental data on the…

Atomic Physics · Physics 2009-11-11 M. Ya. Amusia , A. S. Baltenkov

The polarization-response spectrum of the fullerene C60 modeled as a homogeneous spherical plasma shell is calculated in the framework of the hydrodynamic approach allowing for the spatial dispersion caused by the Fermi-distributed valence…

Plasma Physics · Physics 2017-10-17 V. B. Gildenburg , I. A. Pavlichenko

We formulate a theory of low-temperature, stationary photoluminescence from a quantum-dot molecule composed of two spherical quantum dots whose electronic subsystems are resonantly coupled via the Coulomb interaction. We show that the…

Mesoscale and Nanoscale Physics · Physics 2016-08-05 S. Yu. Kruchinin , I. D. Rukhlenko , A. S. Baimuratov , M. Yu. Leonov , V. K. Turkov , Yu. K. Gun'ko , A. V. Baranov , A. V. Fedorov

A key question of quantum optics is how nonclassical bi-photon correlations at low power evolve into classical coherence at high-power. Direct observation of the crossover from quantum to classical behavior is desirable, but difficult due…

We study the interconnection between the results of two qualitatively different approximate calculations of photoionization cross sections, $\sigma_{n\ell}$, for neutral atoms ($A$) or their cations ($A^+$), centrally confined inside a…

Atomic Physics · Physics 2024-09-19 V. K. Dolmatov , L. V. Chernysheva , V. G. Yarzhemsky

We present the main features of the electronic structure of the heavy atoms that is best of all seen in photoionization. We acknowledge how important was and still is investigation of the interaction between low- and high frequency lasers…

Atomic Physics · Physics 2015-06-03 M. Ya. Amusia

The optical excitations in C$_{60}$ and higher fullerenes, including isomers of C$_{76}$, C$_{78}$, and C$_{84}$, are theoretically investigated. We use a tight binding model with long-range Coulomb interactions, treated by the Hartree-Fock…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya

With increasing energy the diamagnetic hydrogen atom undergoes a transition from regular to chaotic classical dynamics, and the closed orbits pass through various cascades of bifurcations. Closed orbit theory allows for the semiclassical…

Chaotic Dynamics · Physics 2007-05-23 T. Fabcic , J. Main , T. Bartsch , G. Wunner

An assessment is given as to the extent to which pure unitary evolution, as distinct from environmental decohering interaction, can provide the transition necessary for an observer to interpret perceived quantum dynamics as classical. This…

Quantum Physics · Physics 2021-10-05 John S. Briggs

Quantum plasmonics explores how light interacts with collective charge oscillations at metal-dielectric interfaces, enabling strong confinement and enhanced quantum effects at the nanoscale. While traditional quantum optics focuses on…

Quantum Physics · Physics 2025-04-03 Mingyuan Hong

We present an \emph{ab-initio} approach for computing the photoionization spectrum near autoionization resonances in multi-electron systems. While traditional (Hermitian) theories typically require computing the continuum states, which are…

The probability that photoionization of the caged atom in an endohedral system is accompanied by excitation of the fullerene shell is shown to be close to unity in broad intervals of the photoelectron energies. The result is obtained by…

Atomic Physics · Physics 2015-06-15 E. G. Drukarev , M. Ya. Amusia

In this work we study the first step in photosynthesis for the limiting case of a single photon interacting with photosystem II (PSII). We model our system using quantum trajectory theory, which allows us to consider not only the average…

Biological Physics · Physics 2022-08-10 Robert L. Cook , Liwen Ko , K. Birgitta Whaley

Quantum networks require flying qubits that transfer information between the nodes. This may be implemented by means of single atoms (the nodes) that emit and absorb single photons (the flying qubits) and requires full control of photon…

Quantum Physics · Physics 2017-09-20 Philipp Müller , Tristan Tentrup , Marc Bienert , Giovanna Morigi , Jürgen Eschner

We concentrate here on photon absorption as well as electron and positron scattering upon endohedrals that consist of a fullerenes shell and an inner atom A. The aim is to understand the effect of fullerene electron shell in formation of…

Atomic and Molecular Clusters · Physics 2018-02-12 M. Ya. Amusia , A. F. Ioffe

Ionization-excitation of an atom induced by the absorption of a single photon in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly…

Atomic Physics · Physics 2023-09-06 S. Kim , S. Steinhäuser , A. B. Voitkiv , C. Müller

We consider a fully quantized model of spontaneous emission, scattering, and absorption, and study propagation of a single photon from an emitting atom to a detector atom both with and without an intervening scatterer. We find an exact…

Quantum Physics · Physics 2009-11-07 Thomas Purdy , Daniel R. Taylor , Martin Ligare

The mechanism of the transition of a dynamical system from quantum to classical mechanics is of continuing interest. Practically it is of importance for the interpretation of multi-particle coincidence measurements performed at macroscopic…

Quantum Physics · Physics 2016-01-12 John S. Briggs , James M. Feagin