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We perform systematic molecular dynamics simulations of water confined between two nanoscale plates at T=300 K. We investigate the effect of pressure (-0.15 GPa <= P <= 0.2 GPa) and plate separation (0.4 nm <= d <= 1.6 nm) on the phase…

Chemical Physics · Physics 2016-09-08 Nicolas Giovambattista , Peter J. Rossky , Pablo G. Debenedetti

Based on static and dynamical density functional theory, a phase-field-crystal model is derived which involves both the translational density and the orientational degree of ordering as well as a local director field. The model exhibits…

Soft Condensed Matter · Physics 2015-05-19 Hartmut Löwen

We study the kinetics of the nematic-isotropic transition in a two-dimensional liquid crystal by using a lattice Boltzmann scheme that couples the tensor order parameter and the flow consistently. Unlike in previous studies, we find the…

Soft Condensed Matter · Physics 2009-11-07 Colin Denniston , Enzo Orlandini , J. M. Yeomans

Bulk properties of ionic liquid crystals are investigated using density functional theory. The liquid crystal molecules are represented by ellipsoidal particles with charges located in their center or at their tails. Attractive interactions…

Soft Condensed Matter · Physics 2015-05-18 S. Kondrat , M. Bier , L. Harnau

Density-functional theory is used to investigate the phase behavior of colloidal binary hard-platelet and hard-rod fluids near a single hard wall or confined in a slit pore. The Zwanzig model, in which the orientations of the particles of…

Statistical Mechanics · Physics 2009-11-07 L. Harnau , S. Dietrich

Spherical particles confined to a sphere surface cannot pack densely into a hexagonal lattice without defects. In this study, we use hard particle Monte Carlo simulations to determine the effects of continuously deformable shape anisotropy…

Soft Condensed Matter · Physics 2026-01-01 Gabrielle N. Jones , Philipp W. A. Schönhöfer , Sharon C. Glotzer

Using classical density functional theory (DFT) in a modified mean-field approximation we investigate the fluid phase behavior of quasi-two dimensional dipolar fluids confined to a plane. The particles carry three-dimensional dipole moments…

Statistical Mechanics · Physics 2013-06-18 R. Geiger , S. H. Klapp

A cascade of phase transitions from square to hexagonal lattice is studied in 2D system of particles interacting via core-softened potential. Due to the presence of two length-scales of repulsion, different local configurations with four,…

Soft Condensed Matter · Physics 2017-12-14 N. P. Kryuchkov , S. O. Yurchenko , Yu. D. Fomin , E. N. Tsiok , V. N. Ryzhov

By using a phase-field crystal (PFC) model, the liquid-crystal growth of the plastic triangular phase is simulated with emphasis on crystal shape and topological defect formation. The equilibrium shape of a plastic triangular crystal (PTC)…

Soft Condensed Matter · Physics 2017-08-07 Sai Tang , Simon Praetorius , Rainer Backofen , Axel Voigt , Yan-Mei Yu , Jincheng Wang

The evaporation of a droplet induces variety of ordered patterns near the contact line between the droplet and a substrate. This pattern formation involves both the behavior of colloidal suspensions and interactions between a droplet and a…

Soft Condensed Matter · Physics 2024-08-05 Yusaku Abe , Yu Matsuda

We analytically and numerically characterize the structure of hard-sphere fluids in order to review various geometrical frustration scenarios of the glass transition. We find generalized polytetrahedral order to be correlated with…

Statistical Mechanics · Physics 2013-01-07 Benoit Charbonneau , Patrick Charbonneau , Gilles Tarjus

We use interface-resolved simulations to study finite-size effects in turbulent channel flow of neutrally-buoyant spheres. Two cases with particle sizes differing by a factor of 2, at the same solid volume fraction of 20% and bulk Reynolds…

Fluid Dynamics · Physics 2021-02-23 Pedro Costa , Francesco Picano , Luca Brandt , Wim-Paul Breugem

A model predicting the structure of repulsive, spherically symmetric, monodisperse particles confined between two walls is presented. We study the buckling transition of a single flat layer as the double layer state develops. Experimental…

Condensed Matter · Physics 2009-10-22 T Chou , David R. Nelson

We develop a perturbation theory to study the shape and the orientation of an initially spherical capsule of radius R with a viscosity contrast, a surface tension {\sigma} and a bending rigidity $\kappa$ in linear flows. The elastic…

Soft Condensed Matter · Physics 2026-02-18 Paul Regazzi , Marc Leonetti

We consider a simple model consisting of particles with four bonding sites ("patches"), two of type A and two of type B, on the square lattice, and investigate its global phase behavior by simulations and theory. We set the interaction…

Soft Condensed Matter · Physics 2011-11-24 N. G. Almarza , J. M. Tavares , M. Simões , M. M. Telo da Gama

We have employed molecular dynamics simulations based on the TIP4P/2005 water model to investigate the local structural, dynamical, and dielectric properties of the two recently reported body-centered-cubic and face-centered-cubic plastic…

Soft Condensed Matter · Physics 2019-04-03 Ioannis Skarmoutsos , Stefano Mossa , Elvira Guardia

When water is confined to nanocavities, its quantum-mechanical behavior can be revealed by terahertz spectroscopy. We place H2O molecules in the nanopores of a beryl crystal-lattice and observe a rich and highly anisotropic set of…

The search for local structures within a disordered medium has led to proposals of several methods for probing transient short-range symmetry in a homogeneous mono-atomic liquid. We offer a comparison of different characterizations of such…

Soft Condensed Matter · Physics 2020-05-04 Linsey Nowack , Stuart A. Rice

Liquid water can become metastable with respect to its vapor in hydrophobic confinement. The resulting dewetting transitions are often impeded by large kinetic barriers. According to macroscopic theory, such barriers arise from the free…

The generic square-gradient density-functional model with triple-parabolic free energy is used to study the stability of a cavity introduced into the stretched liquid. The various properties of the critical cavity, which is the largest…

Soft Condensed Matter · Physics 2015-05-13 Masao Iwamatsu