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The glass transition, extensively studied in dense fluids, polymers, or colloids, corresponds to a dramatic evolution of equilibrium transport coefficients upon a modest change of control parameter, like temperature or pressure. A similar…

Statistical Mechanics · Physics 2013-05-06 Ludovic Berthier , Jorge Kurchan

We perform molecular dynamics simulations to study lithium dynamics in a model of LiPO$_3$ glass at temperatures below the glass transition. A straightforward analysis of the ionic trajectories shows that lithium diffusion results from…

Soft Condensed Matter · Physics 2009-11-10 Michael Vogel

By means of molecular dynamics simulations and the Voronoi tessellation, we study the influence of the history on the low temperature characteristics of soft sphere and silica glasses. The quench from the liquid is interrupted at an…

Soft Condensed Matter · Physics 2007-05-23 Philippe Jund , Remi Jullien

We present a simple mathematical framework for the description of the dynamics of glassy systems in terms of a random walk in a complex energy landscape pictured as a network of minima. We show how to use the tools developed for the study…

Statistical Mechanics · Physics 2015-03-17 Paolo Moretti , Andrea Baronchelli , Alain Barrat , Romualdo Pastor-Satorras

The slowing down of molecular dynamics when approaching the glass transition generally proceeds much stronger than expected for thermally activated motions. This strange phenomenon can be formally ascribed to a temperature-dependent…

Soft Condensed Matter · Physics 2013-11-28 Th. Bauer , P. Lunkenheimer , A. Loidl

We present the results of a large scale molecular dynamics computer simulation in which we investigated the static and dynamic properties of a silica melt in the temperature range in which the viscosity of the system changes from O(10^-2)…

Statistical Mechanics · Physics 2009-10-31 Jurgen Horbach , Walter Kob

Properties of water have been well elucidated for temperatures above $\sim$230 K and yet mysteries remain in the deeply supercooled region. By performing extensive molecular dynamics simulations on this supercooled region, we find that…

Soft Condensed Matter · Physics 2018-11-15 Shinji Saito , Biman Bagchi , Iwao Ohmine

Amorphous silica ($a-SiO_2$) is a widely used inorganic material. Interestingly, the relationship between the local atomic structures of $a-SiO_2$ and their effects on ductility and fracture is seldom explored. Here, we combine large-scale…

Mesoscale and Nanoscale Physics · Physics 2023-04-17 Jiahao Liu , Jingjie Yeo

The dynamical behavior of a kind of models with hierarchically constrained dynamics is investigated. The models exhibit many properties resembling real structural glasses. In particular, we focus on the study of time-dependent temperature…

Statistical Mechanics · Physics 2009-11-07 A. Prados , J. J. Brey

We image local structural rearrangements in soft colloidal glasses under small periodic perturbations induced by thermal cycling. Local structural entropy $S_{2}$ positively correlates with observed rearrangements in colloidal glasses. The…

Soft Condensed Matter · Physics 2016-06-13 Xiunan Yang , Rui Liu , Mingcheng Yang , Wei-Hua Wang , Ke Chen

Swap algorithms can shift the glass transition to lower temperatures, a recent unexplained observation constraining the nature of this phenomenon. Here we show that swap dynamic is governed by an effective potential describing both particle…

Soft Condensed Matter · Physics 2018-09-12 Carolina Brito , Edan Lerner , Matthieu Wyart

We report a molecular dynamics (MD) study of the collective dynamics of a simple monatomic liquid -interacting through a two body potential that mimics that of lithium- across the liquid-glass transition. In the glassy phase we find…

Disordered Systems and Neural Networks · Physics 2009-11-07 T. Scopigno , G. Ruocco , F. Sette , G. Viliani

Below the melting temperature $T_m$ crystals are the stable phase of typical elemental or molecular systems. However, cooling down a liquid below $T_m$, crystallization is anything but inevitable. The liquid can be supercooled, eventually…

Disordered Systems and Neural Networks · Physics 2017-03-07 M. Zanatta , L. Cormier , L. Hennet , C. Petrillo , F. Sacchetti

We give general topological rules which very accurately predict the chemical trends in glass transition temperature $T_g$ variation as a function of cross-linking. In multicomponent glasses, these chemical trends permit to distinguish…

Disordered Systems and Neural Networks · Physics 2009-10-31 Matthieu Micoulaut , Gerardo G. Naumis

With molecular dynamics simulations of a fluid mixture of classical particles interacting with pair-wise additive Weeks-Chandler-Andersen potentials, we consider the time series of particle displacements and thereby determine distributions…

Statistical Mechanics · Physics 2011-11-10 Lester O. Hedges , Lutz Maibaum , David Chandler , Juan P. Garrahan

In stark contrast with the conventional understanding of the glass transition, where the transition from glass to liquid appears as a dynamic process where atoms/molecules cooperatively relax into the equilibrium phase, we experimentally…

Disordered Systems and Neural Networks · Physics 2023-01-10 Ana Vila-Costa , Marta Gonzalez-Silveira , Cristian Rodríguez-Tinoco , Marta Rodríguez-López , Javier Rodríguez-Viejo

We study the glassy dynamics taking place in dense assemblies of athermal active particles that are driven solely by a nonequilibrium self-propulsion mechanism. Active forces are modeled as an Ornstein-Uhlenbeck stochastic process,…

Soft Condensed Matter · Physics 2016-09-28 Elijah Flenner , Grzegorz Szamel , Ludovic Berthier

In this paper, we review the general features of the out-of-equilibrium dynamics of spin glasses. We use this example as a guideline for a brief description of glassy dynamics in other disordered systems like structural and polymer glasses,…

Disordered Systems and Neural Networks · Physics 2009-11-03 Eric Vincent

Glass-forming liquids have only a modest tendency to crystallize and hence their dynamics can be studied even below the melting temperature. The relaxation dynamics of most of these liquids shows at a temperature $T_c$, somewhat above the…

Soft Condensed Matter · Physics 2025-01-17 Francesco Rusciano , Raffaele Pastore , Francesco Greco , Walter Kob

When a liquid freezes, a change in the local atomic structure marks the transition to the crystal. When a liquid is cooled to form a glass, however, no noticeable structural change marks the glass transition. Indeed, characteristic features…

Soft Condensed Matter · Physics 2015-11-24 Samuel S. Schoenholz , Ekin D. Cubuk , Daniel M. Sussman , Efthimios Kaxiras , Andrea J Liu