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We have made pressure and NMR measurements during the evolution of phase separation in solid helium isotopic mixtures. Our observations indicate clearly all three stages of the homogeneous nucleation - growth process: 1) creation of…

Other Condensed Matter · Physics 2009-11-13 M. Poole , J. Saunders , B. Cowan

We report a numerical study of the rate of crystal nucleation in a binary suspension of oppositely charged colloids. Two different crystal structures compete in the thermodynamic conditions under study. We find that the crystal phase that…

Soft Condensed Matter · Physics 2011-11-10 Eduardo Sanz , Chantal Valeriani , Daan Frenkel , Marjolein Dijkstra

Via hydrodynamics preserving molecular dynamics simulations we study growth phenomena in a phase separating symmetric binary mixture model. We quench high-temperature homogeneous configurations to state points inside the miscibility gap,…

Soft Condensed Matter · Physics 2021-07-23 Koyel Das , Subir K. Das

An exactly solvable reaction-diffusion model consisting of first-class particles in the presence of a single second-class particle is introduced on a one-dimensional lattice with periodic boundary condition. The number of first-class…

Statistical Mechanics · Physics 2009-11-13 F H Jafarpour , B Ghavami

When a system is brought to a metastable state, nuclei of the equilibrium phase form and grow. This is the well-known nucleation and growth of first-order phase transitions. Near a critical point of a continuous phase transition, critical…

Statistical Mechanics · Physics 2025-03-24 Fan Zhong

The treatment of nuclear effects in neutrino-nucleus interactions is one of the main sources of systematic uncertainty for the analysis and interpretation of data of neutrino oscillation experiments. Neutrinos interact with nuclei via…

High Energy Physics - Phenomenology · Physics 2020-01-29 Carlotta Giusti , Martin V. Ivanov

We review theoretical and simulational approaches to the description of equilibrium bulk crystal and interface properties as well as to the nonequilibrium processes of homogeneous and heterogeneous crystal nucleation for the simple model…

Soft Condensed Matter · Physics 2014-02-03 Francesco Turci , Tanja Schilling , Mohammad Hossein Yamani , Martin Oettel

Hard-sphere model systems are well-suited in both experiment and simulations to investigate fundamental aspects of the crystallization of fluids. In experiments on colloidal models of hard-sphere fluids, the uid is unavoidably at contact…

Soft Condensed Matter · Physics 2021-04-28 Jorge R. Espinosa , Carlos Vega , Chantal Valeriani , Daan Frenkel , Eduardo Sanz

Understanding the pathways to crystallization during the deposition of a vapor phase on a cold solid substrate is of great interest in industry, e.g., for the realization of electronic devices made of crystallites-free glassy materials, as…

Soft Condensed Matter · Physics 2023-10-03 Fabio Leoni , Hajime Tanaka , John Russo

A recently formulated description of homogeneous nucleation for Brownian particles in the over-damped limit based on fluctuating hydrodynamics is used to determine the nucleation pathway, characterized as the most likely path (MLP), for the…

Soft Condensed Matter · Physics 2012-10-18 James F. Lutsko

We use molecular dynamics to study the nucleation of cracks in a two dimensional material without pre-existing cracks. We study models with zero and non-zero shear modulus. In both situations the time required for crack formation obeys an…

Statistical Mechanics · Physics 2015-05-13 Cristiano L. Dias , Jens Kroger , Daniel Vernon , Martin Grant

Supercooled liquids give rise, by homogeneous nucleation, to solid superclusters acting as building blocks of glass, ultrastable glass, and glacial glass phases before being crystallized. Liquid-to-liquid phase transitions begin to be…

Disordered Systems and Neural Networks · Physics 2019-06-26 Robert F. Tournier

Bootstrap percolation on a graph iteratively enlarges a set of occupied sites by adjoining points with at least $\theta$ occupied neighbors. The initially occupied set is random, given by a uniform product measure, and we say that spanning…

Probability · Mathematics 2015-05-14 Janko Gravner , David Sivakoff

A system of a metastable phase with several sorts of the heterogeneous centers is considered. An analytical theory for the process of condensation in such a system is constructed in dynamic conditions. The free energy of formation of the…

Condensed Matter · Physics 2007-05-23 V. Kurasov

In many systems, nucleation of a stable solid may occur in the presence of other (often more than one) metastable phases. These may be polymorphic solids or even liquid phases. In such cases, nucleation of the solid phase from the melt may…

Materials Science · Physics 2013-04-08 Mantu Santra , Rakesh S. Singh , Biman Bagchi

We consider the liquid drop model for nuclei interacting with a neutralizing homogeneous background of electrons. The regime we are interested in is when the fraction between the electronic and the nuclear charge density is small. We show…

Mathematical Physics · Physics 2021-03-26 Lukas Emmert , Rupert L. Frank , Tobias König

Recently, it was shown that a theoretical description of nucleation based on fluctuating hydrodynamics and classical density functional theory can be used to determine non-classical nucleation pathways for crystallization (Lutsko, Sci. Adv.…

Chemical Physics · Physics 2024-06-26 James F. Lutsko , Cédric Schoonen

Nucleation phenomena are ubiquitous in nature and the presence of impurities in every real and experimental system is unavoidable. Yet numerical studies of nucleation are nearly always conducted for entirely pure systems. We have studied…

Statistical Mechanics · Physics 2021-08-11 Dipanjan Mandal , David Quigley

A hydrophilic liquid, such as water, forms hydrogen bonds with a hydrophilic substrate. The strength and locality of the hydrogen bonding interactions prohibit slip of the liquid over the substrate. The question then arises how the contact…

Fluid Dynamics · Physics 2018-07-11 Petter Johansson , Berk Hess
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