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We analyze the two-dimensional photoelectrons momentum distribution of Ar atom ionized by midinfrared laser pulses and mainly concentrate on the energy range below 2Up. By using a generalized quantum trajectory Monte Carlo (GQTMC)…

Atomic Physics · Physics 2016-11-02 Weifeng Yang , Huatang Zhang , Cheng Lin , Jingwen Xu , Zhihao Sheng , Xiaohong Song , Shilin Hu , Jing Chen

Strong-field photoelectron momentum imaging of the prototypical biomolecule indole was disentangled in a combined experimental and computational approach. Experimentally, strong control over the molecules enabled the acquisition of…

Atomic Physics · Physics 2021-02-03 Joss Wiese , Jolijn Onvlee , Sebastian Trippel , Jochen Küpper

We investigate theoretically electron dynamics under a VUV attosecond pulse train which has a controlled phase delay with respect to an additional strong infrared laser field. Using the strong field approximation and the fact that the…

Atomic Physics · Physics 2015-05-13 P. Riviere , O. Uhden , U. Saalmann , J. M. Rost

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…

Photoelectron angular distributions (PADs) obtained from ionization of potassium atoms using moderately intense femtosecond IR fields ($\sim$10$^{12}$Wcm$^{-2}$) of various polarization states are shown to provide a route to "complete"…

Atomic Physics · Physics 2015-01-15 Paul Hockett , Matthias Wollenhaupt , Christian Lux , Thomas Baumert

Attosecond metrology with linearly polarized light pulses is the basis of a highly successful research area. An even broader impact can be expected from a generalized metrology that covers two-dimensional polarization states, enabling…

Optics · Physics 2023-12-29 Meng Han , Jia-bao Ji , Kiyoshi Ueda , Hans Jakob Wörner

We have proposed and developed a method to utilize attosecond pulses in diffraction imaging techniques applied to complex samples. In this study, the effects of the broadband properties of the wavefield owing to attosecond pulses are…

Optics · Physics 2023-12-01 G. N. Tran , Katsumi Midorikawa , Eiji J. Takahashi

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

Atomic Physics · Physics 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

We present techniques to perturb, measure and model the ion velocity distribution in an ultracold neutral plasma produced by photoionization of strontium atoms. By optical pumping with circularly polarized light we promote ions with certain…

Atomic Physics · Physics 2012-04-25 J. Castro , G. Bannasch , P. McQuillen , T. Pohl , T. C. Killian

We consider the time delay of electron detachment from a Coulomb center and two-center systems in the process of ionization. It is shown that the attosecond streaking, most usual method of time delay measure, can be formally described by…

Atomic Physics · Physics 2015-06-15 Vladislav V. Serov , Vladimir L. Derbov , Tatyana A. Sergeeva

We experimentally demonstrate spatiotemporal steering of photoelectron emission in multiphoton above-threshold single ionization of atoms exposed to a phase-controlled orthogonally polarized two-color (OTC) laser pulse. Spatial and energy…

Collective electron dynamics in plasmonic nanosystems can unfold on timescales in the attosec- ond regime and the direct measurements of plasmonic near-field oscillations is highly desirable. We report on numerical studies on the…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Frederik Süßmann , Matthias F. Kling

We report on the design and performance of a velocity map imaging (VMI) spectrometer optimized for experiments using high-intensity extreme ultraviolet (XUV) sources such as laser-driven high-order harmonic generation (HHG) sources and…

Half-cycle picosecond pulses have been produced from thin photo-conductors, when applying an electric field across the surface and switching on conduction by a short laser pulse. Then the transverse current in the wafer plane emits…

Optics · Physics 2015-06-03 H. -C. Wu , J. Meyer-ter-Vehn

The kinetic energy distribution of D$^+$ ions resulting from the interaction of a femtosecond laser pulse with D$_2$ molecules is calculated based on the rescattering model. From analyzing the molecular dynamics, it is shown that the…

Atomic Physics · Physics 2009-11-10 X. M. Tong , Z. X. Zhao , C. D. Lin

We investigate the possibility to monitor the dynamics of autoionizing states in real time and control the yields of different ionization channels in helium by simulating XUV-pump IR-probe experiments focused on the N=2 threshold. The XUV…

Atomic Physics · Physics 2015-05-18 Luca Argenti , Eva Lindroth

We present experimental data on the non-adiabatic strong field ionization of atomic hydrogen using elliptically polarized femtosecond laser pulses at a central wavelength of 390 nm. Our measured results are in very good agreement with a…

We describe the results of experiments and simulations performed with the aim of extending photoelectron spectroscopy with intense laser pulses to the case of molecular compounds. Dimer frame photoelectron angular distributions generated by…

Attosecond X-ray pulses are indispensable for exploring ultrafast phenomena in matter on Angstrom and attosecond scales. Here we propose a new method to realize spatiotemporal shaping of attosecond X-rays through temporal control of the…

Accelerator Physics · Physics 2026-01-13 Chenzhi Xu , Jiawei Yan , Gianluca Geloni , Christoph Lechner , Haixiao Deng

The measurement of tunneling times in strong-field ionization has been the topic of much controversy in recent years, with the attoclock and Larmor clock being two of the main contenders for correctly reproducing these times. By expressing…

Quantum Physics · Physics 2025-05-01 Pablo Martin Maier , Serguei Patchkovskii , Mikhail Ivanov , Olga Smirnova