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Understanding and controlling spin relaxation in molecular qubits is essential for developing chemically tunable quantum information platforms. We present a fully first-principles framework for computing the spin relaxation tensor in a…

Quantum Physics · Physics 2025-07-25 Roman Dmitriev , Nosheen Younas , Yu Zhang , Andrei Piryatinski , Eric R. Bittner

The realisation of quantum computers based on molecular electronic spins requires the design of qubits with very long coherence times, T2. Dephasing can proceed over several different microscopic pathways, active at the same time and in…

Materials Science · Physics 2020-01-08 Alessandro Lunghi , Stefano Sanvito

We examine the effects of intra-environmental coupling on decoherence by constructing a low temperature spin--spin-bath model of an atomic impurity in a Debye crystal. The impurity interacts with phonons of the crystal through…

Quantum Physics · Physics 2009-11-07 L. Tessieri , J. Wilkie

Collectively-encoded qubits, involving ensembles of atomic or solid-state emitters, present many practical advantages for quantum technologies. However, they suffer from uncontrolled inhomogeneous dephasing which couples them to a…

Quantum Physics · Physics 2025-11-10 Antoine Covolo , Valentin Magro , Mathieu Girard , Sébastien Garcia , Alexei Ourjoumtsev

The coherence time of an electron spin decohered by the nuclear spin environment in a quantum dot can be substantially increased by subjecting the electron to suitable dynamical decoupling sequences. We analyze the performance of high-level…

Mesoscale and Nanoscale Physics · Physics 2008-03-27 Wenxian Zhang , N. P. Konstantinidis , V. V. Dobrovitski , B. N. Harmon , Lea F. Santos , Lorenza Viola

The inhomogeneity of an electron spin ensemble as well as fluctuating environment acting upon individual spins drastically shorten the spin coherence time $T_2$ and hinder coherent spin manipulation. We show that this problem can be solved…

Mesoscale and Nanoscale Physics · Physics 2021-10-13 V. V. Belykh , A. R. Korotneva , D. R. Yakovlev

The decay of Rabi oscillations provides direct information about coherence of electron spins. When observed in EPR experiments, it is often shortened by spatial inhomogeneity of the microwave field amplitude in a bulk sample. In order to…

Mesoscale and Nanoscale Physics · Physics 2018-09-03 A. P. Saiko , R. Fedaruk , S. A. Markevich

Quantum bits or qubits naturally decohere by becoming entangled with uncontrollable environments. Dynamical decoupling is thereby required to disentangle qubits from an environment by periodically reversing the qubit bases, but this causes…

Quantum Physics · Physics 2020-02-26 Yuhei Sekiguchi , Yusuke Komura , Hideo Kosaka

We demonstrate full suppression of dephasing tied to deformation potential coupling of confined electrons to longitunidal acoustic (LA) phonons in optical control experiments on large semiconductor quantum dots (QDs) with emission…

Mesoscale and Nanoscale Physics · Physics 2020-12-07 A. Ramachandran , G. R. Wilbur , S. O'Neal , D. G. Deppe , K. C. Hall

In a closed system, it is well known that the time-reversal symmetry can lead to Kramers degeneracy and protect nontrivial topological states such as quantum spin Hall insulator. In this letter we address the issue whether these effects are…

Mesoscale and Nanoscale Physics · Physics 2021-08-25 Tian-Shu Deng , Lei Pan , Yu Chen , Hui Zhai

Controlling decoherence is the most challenging task in realizing quantum information hardware. Single electron spins in gallium arsenide are a leading candidate among solid- state implementations, however strong coupling to nuclear spins…

Mesoscale and Nanoscale Physics · Physics 2012-07-12 Yongjie Hu , Ferdinand Kuemmeth , Charles M. Lieber , Charles M. Marcus

Temporal modes (TMs) of photons provide an appealing high-dimensional encoding basis for quantum information. While techniques to generate TM states have been established, high-dimensional decoding of single-photon TMs remains an open…

We show that the qubit decoherence due to zero-temperature energy relaxation can be almost completely suppressed by using the quantum uncollapsing procedure. To protect a qubit state, a partial quantum measurement moves it towards the…

Quantum Physics · Physics 2015-05-13 Alexander N. Korotkov , Kyle Keane

We experimentally demonstrate over two orders of magnitude increase in the coherence time of nitrogen vacancy centres in diamond by implementing decoupling techniques. We show that equal pulse spacing decoupling performs just as well as…

Quantum Physics · Physics 2010-12-08 C. A. Ryan , J. S. Hodges , D. G. Cory

In Si/SiGe quantum dots, the decoherence behavior of spin qubits usually comes from the non-Markovian effect of the charge noise. To improve the performance of using the coherent noise models in the decoherence simulation and tomography…

Quantum Physics · Physics 2025-10-28 Wei-en Chiu , Chia-Hsien Huang , Yi-Hsien Wu , Hsi-Sheng Goan

In this work the problem of characterizing matrix material structure from embedded electron spin decoherence is studied both theoretically and experimentally. Theoretical calculation using nuclear spin bath model and cluster correlation…

We study three-electron-spin decoherence in a semiconductor triple quantum dot with a linear geometry. The three electron spins are coupled by exchange interactions J_{12} and J_{23}, and we clarify inhomogeneous and homogeneous dephasing…

Mesoscale and Nanoscale Physics · Physics 2014-07-23 Jo-Tzu Hung , Jianjia Fei , Mark Friesen , Xuedong Hu

Spin relaxation in a quantum Hall ferromagnet, where filling is $\nu=1, 1/3, 1/5,...$, can be considered in terms of spin wave annihilation/creation processes. Hyperfine coupling with the nuclei of the GaAs matrix provides spin…

Strongly Correlated Electrons · Physics 2013-04-30 S. Dickmann , T. Ziman

We apply optimal control theory (OCT) to the design of refocusing pulses suitable for the CPMG sequence that are robust over a wide range of B0 and B1 offsets. We also introduce a model, based on recent progress in the analysis of unitary…

Quantum Physics · Physics 2011-01-24 Troy W. Borneman , Martin D. Hurlimann , David G. Cory

Addressing and mitigating decoherence sources plays an essential role in the development of a scalable quantum computing system, which requires low gate errors to be consistently maintained throughout the circuit execution. While nuclear…