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We theoretically investigate the dynamic interaction of a quantum dot in a nanocavity with timesymmetric single photon pulses. The simulations, based on a wavefunction approach, reveal that almost perfect single photon absorption occurs for…

Quantum Physics · Physics 2012-07-23 Robert Johne , Andrea Fiore

We investigate the performance of a one-dimensional dimerized XY chain as a spin quantum battery. Such integrable model shows a rich quantum phase diagram that emerges through a mapping of the spins onto auxiliary fermionic degrees of…

The nature of excited states of open quantum systems produced by incoherent natural thermal light is analyzed based on a description of the generator of the dynamics. Natural thermal light is shown to generate long-lasting coherent dynamics…

Quantum Physics · Physics 2017-09-05 Leonardo A. Pachon , Juan D. Botero , Paul Brumer

We investigate the charge transfer characteristics of one and two excess charges in a DNA base-pair dimer using a model Hamiltonian approach. The electron part comprises diagonal and off-diagonal Coulomb matrix elements such a correlated…

Strongly Correlated Electrons · Physics 2015-05-14 Sabine Tornow , Ralf Bulla , Frithjof B. Anders , Gertrud Zwicknagl

Electron capture processes for low energy Ar9+ ions colliding on Ar2 dimer targets are investigated, focusing attention on charge sharing as a function of molecule orientation and impact parameter. A preference in charge-asymmetric…

Electron injection from an adsorbed molecule to the substrate (heterogeneous electron transfer) is studied. One reaction coordinate is used to model this process. The surface phonons and/or the electron-hole pairs together with the internal…

Chemical Physics · Physics 2009-11-07 Michael Schreiber , Ivan Kondov , Ulrich Kleinekathoefer

Ensembles of erbium dopants can realize quantum memories and frequency converters that operate in the minimal-loss wavelength band of fiber optical communication. Their operation requires the initialization, coherent control and readout of…

The long spin coherence times in ambient conditions of color centers in solids, such as nitrogen-vacancy (NV$^{-}$) centers in diamond, make these systems attractive candidates for quantum sensing. Quantum sensing provides remarkable…

Quantum Physics · Physics 2019-06-06 N. J. Harmon , M. E. Flatté

Plasmonic excitations decay within femtoseconds, leaving non-thermal (often referred to as "hot") charge carriers behind that can be injected into molecular structures to trigger chemical reactions that are otherwise out of reach -- a…

Materials Science · Physics 2025-01-28 Jakub Fojt , Paul Erhart , Christian Schäfer

This is the second of a series of papers devoted to develop a microscopical approach to the dipole emission process and its relation to coherent transport in random media. In this Letter, we deduce a relation between the transverse decay…

Optics · Physics 2009-03-12 M. Donaire

Absorption of electromagnetic energy by a dissipative material is one of the most fundamental electromagnetic processes that underlies a plethora of applied problems, including sensing and molecular detection, radar detection, wireless…

Optics · Physics 2020-03-31 Alexey Proskurin , Andrey Bogdanov , Denis G. Baranov

Most applications of metasurfaces require excitation and control of both electric and magnetic surface currents. For such purpose, the metasurface must have a finite thickness to handle magnetic surface currents. For metasurface sheets of…

Applied Physics · Physics 2022-02-28 F. S. Cuesta , A. D. Kuznetsov , G. A. Ptitcyn , X. Wang , S. A. Tretyakov

We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…

Atomic Physics · Physics 2015-06-19 Alexander Blättermann , Christian Ott , Andreas Kaldun , Thomas Ding , Thomas Pfeifer

The electron transfer in different solvents is investigated for systems consisting of donor, bridge and acceptor. It is assumed that vibrational relaxation is much faster than the electron transfer. Electron transfer rates and final…

Soft Condensed Matter · Physics 2016-09-28 D. Kilin , U. Kleinekathoefer , M. Schreiber

We consider two parallel layers of dipolar ultracold Fermi gases at different temperatures and calculate the heat transfer between them. The effective interactions describing screening and correlation effects between the dipoles in a single…

Atomic Physics · Physics 2016-03-09 B. Renklioglu , B. Tanatar , M. Ö. Oktel

Optical pump-probe signals can be viewed as work done by the matter while transferring the energy between two coherent baths (from pump to probe). In thermodynamics a heat engine, such as laser, is a device which performs similar work but…

Quantum Physics · Physics 2021-04-14 Md Qutubuddin , Konstantin E. Dorfman

It is shown that adsorption energy at semiconductor surfaces critically depends on the charge transfer to or from the adsorbed species. For the processes without the charge transfer, such as molecular adsorption of closed shell systems, the…

Materials Science · Physics 2013-08-23 Paweł Kempisty , Paweł Strak , Konrad Sakowski , Stanisław Krukowski

We study charge transfer between donor-acceptor molecules subject to a mirror symmetry constraint in the presence of a dissipative environment. The symmetry requirement leads to the breakdown of the standard single reaction coordinate…

Soft Condensed Matter · Physics 2007-05-23 M. R. D'Orsogna , R. Bruinsma

Interfacial ultrafast electron migration processes are simulated in finite cluster models of dye-sensitized solar cells within a single active electron approach. Initially, three different donor-acceptor $\pi$-conjugated dyes supported on…

Chemical Physics · Physics 2017-07-06 Gunter Hermann , Felix Witte , Jean Christophe Tremblay

The question of how quantum coherence facilitates energy transfer has been intensively debated in the scientific community. Since natural and artificial light-harvesting units operate under the stationary condition, we address this question…

Chemical Physics · Physics 2020-07-22 Pei-Yun Yang , Jianshu Cao