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Related papers: Polymer collapse and crystallization in bond fluct…

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Discovering novel emergent behavior in quantum many-body systems is a main objective of contemporary research. In this paper, we explore the effects on phases and phase transitions of the proximity to a Ruelle-Fisher instability, marking…

Statistical Mechanics · Physics 2024-09-12 Saverio Moroni , Fabio Cinti , Massimo Boninsegni , Giuseppe Pellicane , Santi Prestipino

We investigate the internal structure of a polymer during collapse from an expanded coil to a compact globule. Collapse is more probable in local regions of high curvature, so a smoothing of the fractal polymer structure occurs that…

Soft Condensed Matter · Physics 2008-11-07 G. E. Crooks , B. Ostrovsky , Y. Bar-Yam

We investigate the properties of highly compressible turbulence, the compressibility arising from a small effective polytropic exponent $\gamma_e$ due to cooling. In the limit of small $\gamma_e$, the density jump at shocks is shown to be…

Astrophysics · Physics 2009-10-28 E. Vazquez-Semadeni , T. Passot , A. Pouquet

The polymer systems are discussed in the framework of the Landau-Ginzburg model. The model is derived from the mesoscopic Edwards hamiltonian via the conditional partition function. We discuss flexible, semiflexible and rigid polymers. The…

Condensed Matter · Physics 2007-05-23 Robert Holyst , T. A. Vilgis

The conformations of interacting linear polymers on a dynamical planar random lattice are studied using a random two-matrix model. An exact expression for the partition function of self-avoiding chains subject to attractive contact…

Condensed Matter · Physics 2008-02-03 Simon Dalley

We study random copolymers consisted of two kinds of monomers with attraction between similar kinds. The mean field analysis of this system indicates a continuous phase transition into a phase with periodic microdomain structure. It is…

Condensed Matter · Physics 2009-10-22 A. M. Gutin , C. D. Sfatos , E. I. Shakhnovich

The collapse kinetics of strongly charged polyelectrolytes in poor solvents is investigated by Langevin simulations and scaling arguments. The rate of collapse increases sharply as the valence of counterions, z, increases from one to four.…

Soft Condensed Matter · Physics 2007-05-23 Namkyung Lee , D. Thirumalai

Collapse of the polymer chain upon the sharp decrease of solvent quality is studied. During collapse, any pair of polymer units appearing in a sufficiently close vicinity in space has the possibility with a certain probability to form an…

Soft Condensed Matter · Physics 2019-11-07 A. M. Astakhov , S. K. Nechaev , K. E. Polovnikov

We study energy relaxation in a phenomenological model for polymer built from rheological considerations: a one dimensional nonlinear lattice with dissipative couplings. These couplings are well known in polymer's community to be possibly…

Statistical Mechanics · Physics 2009-11-07 F. Gobet , S. Ciliberto , T. Dauxois

The nature of the glass transition is theoretically understood in the mean-field limit of infinite spatial dimensions, but the problem remains totally open in physical dimensions. Nontrivial finite-dimensional fluctuations are hard to…

Statistical Mechanics · Physics 2019-04-05 Ludovic Berthier , Patrick Charbonneau , Andrea Ninarello , Misaki Ozawa , Sho Yaida

The classic Kob-Andersen (KA) binary Lennard-Jones mixtures which are designed to prevent crystallization has been extensively studied in simulation of slow dynamics. Although crystallization can occur if a liquid system is cooled slowly,…

Soft Condensed Matter · Physics 2017-03-10 Penghui Cao

A directed polymer is considered on a flat substrate with randomly located parallel ridges. It prefers to lie inside wide regions between the ridges. When the transversel width $W=\exp(\lambda L^{1/3})$ is exponential in the longitudinal…

Disordered Systems and Neural Networks · Physics 2009-10-30 Th. M. Nieuwenhuizen

Fluid phase equilibrium depends on the external constraints imposed on a system. In a closed system with fixed volume, depending on the average density, a vapor bubble may be stable, metastable, or unstable, with respect to the homogeneous…

Soft Condensed Matter · Physics 2026-02-24 Frederic Caupin , Alberto Zaragoza , Miguel A. Gonzalez , Chantal Valeriani

We study the onset of rigidity near the glass transition (GT) in a short-chain polymer melt modelled by a bead-spring model, where all beads interact with Lennard-Jones potentials. The properties of the system are examined above and below…

Soft Condensed Matter · Physics 2009-11-10 Matthew L. Wallace , Bela Joos , Michael Plischke

Crystallization is a process of great practical relevance in which rare but crucial fluctuations lead to the formation of a solid phase starting from the liquid. Like in all first order first transitions there is an interplay between…

Statistical Mechanics · Physics 2017-07-12 Pablo M. Piaggi , Omar Valsson , Michele Parrinello

By Monte Carlo simulations of a variant of the bond-fluctuation model without topological constraints we examine the center-of-mass (COM) dynamics of polymer melts in $d=3$ dimensions. Our analysis focuses on the COM displacement…

Disordering of solids typically leads to amorphization, but polymorph transitions, facilitated by favorable atomic rearrangements, may temporarily help to maintain long-range periodicity in the solid state. In far-from-equilibrium…

Monte Carlo simulation on the crystallization of double crystalline diblock copolymer unravels an intrinsic relationship between block asymmetry and crystallization behaviour. We model crystalline A-B diblock copolymer, wherein the melting…

Soft Condensed Matter · Physics 2015-06-19 Chitrita Kundu , Ashok Kumar Dasmahapatra

Conformational transitions of a single macromolecule of finite size $N$ cannot be described within standard thermodynamic framework. Taking as a basis a simple model of homopolymer exhibiting a coil-globule transition, we show that a…

Statistical Mechanics · Physics 2007-05-23 Annick Lesne , Jean-Marc Victor

The interaction of polymers with small-scale velocity gradients can trigger a coil-stretch transition in the polymers. We analyze this transition within a direct numerical simulation of shear turbulence with an Oldroyd-B model for the…

Chaotic Dynamics · Physics 2009-11-07 Bruno Eckhardt , Jochen Kronjaeger , Joerg Schumacher